Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Dynamic hologram magnification with incoherent optical pumping

Omar A. Ormachea, Alexei L. Tolstik

Published Jul 1, 2003• 1 citation
Publisher

Abstract

In the present work consideration is given to theoretical and experimental analysis of the possibilities for improving the efficiency of multiwave mixing in the process of dynamic hologram recording in solutions of complex organic compounds with additional irradiation of resonant medium at a frequency falling within the absorption band from the excited level. Three- and seven-fold increase in the diffraction efficiency has been realized in Rhodamine 6G dye for four- and six-wave missing, respectively.

DOI
10.1117/12.498464

Related papers

Amplification of multiwave mixing in lasing dyes and polarization recording of dynamic holograms

Omar A. Ormachea, Alexei L. Tolstik

This work presents theoretical and experimental studies of the energy efficiency of multiwave mixing in complex molecular media (dye solutions) exhibiting higher order nonlinearities. There is a great variety of such media, including the resonance ones revealing nonlinearities of higher orders due to the absorption saturation effect and transitions between different excited states of the molecules. However, the majority of previous studies of multiwave mixing have been performed in the resonant medium approximation disregarding the induced anisotropy effect. A new method for enhancement of multiwave mixing in solutions of laser dyes has been proposed and substantiated with the use of lasing as an additional light beam, whose absorption by the molecules in the excited states leads to the formation of thermal dynamic gratings resultant in the improved efficiency of the energy exchange. The theoretical models for the formation of nonlinear dynamic holograms adequately describing the control process over multiwave mixing by an independent light beam, the frequency of which is tuned into the induced absorption band from the molecules in the excited state, have been developed. Polarization multiwave mixing has been realized in Rhodamine-6G dye solution using nonlinearities up to the ninth order inclusive. It has been demonstrated that on orthogonal polarization of the hologram recording waves the diffraction efficiency is lowered by one-two orders, the diffracted wave polarization being dependent on the diffraction order (the polarization plane alignment is identical within the orders of the same evenness).

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Sep 16, 2005•0 citations

Nonlinear hologram recording and multiwave mixing in resonant media

Alexei L. Tolstik

The schemes of light beam transformations by volume dynamic holograms in resonant media revealing the fifth- or higher- order nonlinearities have been theoretically analyzed. N- wave mixing has been realized by changing of the propagation direction or read-out wave frequency in the solution of Rhodamine-6J dye and polymethine dye 3274U. It has been demonstrated that the experimental result are in good agreement with the theoretical data obtained for a three- level medium model with due regard to absorption form the excited singlet level.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Dec 29, 1999•0 citations

Polarization recording of dynamic holograms in saturable absorbers

José Luis Arce Diego, Félix Fanjul-Vélez, David Pereda Cubián +3 more

The potentialities of diffraction methods for wavefront transformations may be considerably widened due to the use of nonlinear recording of dynamic holograms enabling multiwave mixing in media with the fifth and higher order nonlinearities. There is a great variety of such media including the resonant ones for which the presence of higher order nonlinearities is conditioned by the absorption saturation effect and transitions between different excited states of the molecules. However, in the majority of previous studies of multiwave mixing the resonant medium approximation has been used disregarding the induced anisotropy effect. This work presents a theoretical model and experimental studies of the energy efficiency of multiwave mixing in complex molecular media exhibiting higher order nonlinearities, in two cases: when the nonlinear cavity is introduced in the Fabry-Perot interferometer (IFP), and without it. Owing to the use of different combinations of mutually aligning polarizations for interacting waves, one is enabled to determine the contribution into the interaction efficiency by various dynamic gratings and nonlinearity mechanisms. The role of polarization gratings resultant from spatial modulation of the light field polarization state at the orthogonal polarization of the hologram recording waves has been established. Comparisons between the contributions of the above gratings and “normal” gratings recorded by identically polarized light beams into the process of multiwave mixing have demonstrated that the relation of these contributions is dependent on the intensity of interacting waves, and also it has been found that polarization of the diffracted wave is dependent on the diffraction order.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Mar 23, 2005•2 citations

Frequency conversion of coherent images by thin and volume dynamic holograms

Omar A. Ormachea, O. G. Romanov, Alexei L. Tolstik +3 more

One of the main advances of dynamical holography is the possibility to operate with coherent images in real-time experimental situation. Non-degenerate four-wave mixing has some advantages among different holographic methods because it gives the possibility to perform visualization of infra-red images or to convert visible radiation into ultra-violet region. In the work we study different schemes of frequency conversion of coherent images by thin and volume dynamic holograms nonlinearly formed in multilevel resonance media in conditions of non-degenerate four-wave mixing. The theoretical model of dynamic gratings formation in dye solutions based on coupled-wave equations has been developed. Experimental realization of frequency conversion of coherent images from infra-red to the visible and between different wavelengths of visible region has been performed. It has been shown that the criterion of hologram thickness is dependent on the optical density of medium and intensity of input radiation. The diffraction efficiency of dynamic gratings has been measured in conditions of optical bleaching and in the mode of strong absorption, enabling recording of thin gratings.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Feb 7, 2006•0 citations

Four-wave mixing in multilevel media at spatially homogenous irradiation

S. M. Karpuck, Alexander S. Rubanov, Alexei L. Tolstik +1 more

Theoretical analysis of nonconventional schemes of four-wave mixing (FWM) using additional irradiation of resonance medium, which enables the realization of noncoherent optical control of the process efficiency, has been carried out. The possibility of significant increase in the phase conjugate reflectivity and decrease in the pump wave intensity, required for realization of optical bistability, has been shown. Optical control and intensification of FWM in Rhodamine 6G solution have been experimentally accomplished

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Dec 16, 1992•1 citation

Nonlinear hologram recording in resonant media and optical control of diffraction efficiency

Alexei L. Tolstik, Omar A. Ormachea

The schemes for nonlinear recording of dynamic holograms in multilevel resonant media, in conditions when the fifth- and higher-order nonlinearities are exhibited, have been studied both theoretically and experimentally. The optical methods to control the diffraction efficiency of nonlinear dynamic holograms with the use of an additional light beam tuned out into the absorption band from the ground or excited state of the molecules have been considered.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•May 20, 2006•0 citations
In the present work consideration is given to theoretical and experimental analysis of the possibilities for improving the efficiency of multiwave mixing in the process of dynamic hologram recording in solutions of complex organic compounds with additional irradiation of resonant medium at a frequency falling within the absorption band from the excited level. Three- and seven-fold increase in the diffraction efficiency has been realized in Rhodamine 6G dye for four- and six-wave missing, respectively.
This work presents theoretical and experimental studies of the energy efficiency of multiwave mixing in complex molecular media (dye solutions) exhibiting higher order nonlinearities. There is a great variety of such media, including the resonance ones revealing nonlinearities of higher orders due to the absorption saturation effect and transitions between different excited states of the molecules. However, the majority of previous studies of multiwave mixing have been performed in the resonant medium approximation disregarding the induced anisotropy effect. A new method for enhancement of multiwave mixing in solutions of laser dyes has been proposed and substantiated with the use of lasing as an additional light beam, whose absorption by the molecules in the excited states leads to the formation of thermal dynamic gratings resultant in the improved efficiency of the energy exchange. The theoretical models for the formation of nonlinear dynamic holograms adequately describing the control process over multiwave mixing by an independent light beam, the frequency of which is tuned into the induced absorption band from the molecules in the excited state, have been developed. Polarization multiwave mixing has been realized in Rhodamine-6G dye solution using nonlinearities up to the ninth order inclusive. It has been demonstrated that on orthogonal polarization of the hologram recording waves the diffraction efficiency is lowered by one-two orders, the diffracted wave polarization being dependent on the diffraction order (the polarization plane alignment is identical within the orders of the same evenness).
The schemes of light beam transformations by volume dynamic holograms in resonant media revealing the fifth- or higher- order nonlinearities have been theoretically analyzed. N- wave mixing has been realized by changing of the propagation direction or read-out wave frequency in the solution of Rhodamine-6J dye and polymethine dye 3274U. It has been demonstrated that the experimental result are in good agreement with the theoretical data obtained for a three- level medium model with due regard to absorption form the excited singlet level.
The potentialities of diffraction methods for wavefront transformations may be considerably widened due to the use of nonlinear recording of dynamic holograms enabling multiwave mixing in media with the fifth and higher order nonlinearities. There is a great variety of such media including the resonant ones for which the presence of higher order nonlinearities is conditioned by the absorption saturation effect and transitions between different excited states of the molecules. However, in the majority of previous studies of multiwave mixing the resonant medium approximation has been used disregarding the induced anisotropy effect. This work presents a theoretical model and experimental studies of the energy efficiency of multiwave mixing in complex molecular media exhibiting higher order nonlinearities, in two cases: when the nonlinear cavity is introduced in the Fabry-Perot interferometer (IFP), and without it. Owing to the use of different combinations of mutually aligning polarizations for interacting waves, one is enabled to determine the contribution into the interaction efficiency by various dynamic gratings and nonlinearity mechanisms. The role of polarization gratings resultant from spatial modulation of the light field polarization state at the orthogonal polarization of the hologram recording waves has been established. Comparisons between the contributions of the above gratings and “normal” gratings recorded by identically polarized light beams into the process of multiwave mixing have demonstrated that the relation of these contributions is dependent on the intensity of interacting waves, and also it has been found that polarization of the diffracted wave is dependent on the diffraction order.
One of the main advances of dynamical holography is the possibility to operate with coherent images in real-time experimental situation. Non-degenerate four-wave mixing has some advantages among different holographic methods because it gives the possibility to perform visualization of infra-red images or to convert visible radiation into ultra-violet region. In the work we study different schemes of frequency conversion of coherent images by thin and volume dynamic holograms nonlinearly formed in multilevel resonance media in conditions of non-degenerate four-wave mixing. The theoretical model of dynamic gratings formation in dye solutions based on coupled-wave equations has been developed. Experimental realization of frequency conversion of coherent images from infra-red to the visible and between different wavelengths of visible region has been performed. It has been shown that the criterion of hologram thickness is dependent on the optical density of medium and intensity of input radiation. The diffraction efficiency of dynamic gratings has been measured in conditions of optical bleaching and in the mode of strong absorption, enabling recording of thin gratings.
Theoretical analysis of nonconventional schemes of four-wave mixing (FWM) using additional irradiation of resonance medium, which enables the realization of noncoherent optical control of the process efficiency, has been carried out. The possibility of significant increase in the phase conjugate reflectivity and decrease in the pump wave intensity, required for realization of optical bistability, has been shown. Optical control and intensification of FWM in Rhodamine 6G solution have been experimentally accomplished