Dynamics of the elementary photoelectric conversion upon interaction of a single-photon mode with a bound electron in a one-dimensional rectangular potential well is considered. The spatial and temporal dynamics of the wave packet corresponding to a free photoelectron is investigated.
The interaction of a single-photon wave packet with an initially excited two-level atom in free space is studied in semiclassical and quantum approaches. It is shown that the final state of the field does not contain doubly occupied modes. The process of the atom's transition to the ground state may be accelerated, decelerated, or even reversed by the incoming photon, depending on parameters. The spectrum of emitted radiation is close to the sum of the spectrum of the incoming single-photon wave packet and the natural line shape, with small and complicated deviations.
We propose a two-dimensional interferometry based on the electron wave-packet interference by using a cycle-shaped orthogonally polarized two-color laser field. With such a method, the subcycle and intercycle interferences can be disentangled into different directions in the measured photoelectron momentum spectra. The Coulomb influence can be minimized and the overlapping of interference fringes with the complicated low-energy structures can be avoided as well. The contributions of the excitation effect and the long-range Coulomb potential can be traced in the Fourier domain of the photoelectron distribution. Because of these advantages, precise information on valence electron dynamics of atoms or molecules with attosecond temporal resolution and additional spatial information with angstrom resolution can be obtained with the two-dimensional electron wave-packet interferometry.
We are developing a semi-classical model to explain the physical processes behind the origin of the statistical variations in the photoelectron current pulses that we register for different kinds of light. They are: super-Poissonian thermal light, Poissonian laser light and sub-Poissonian nonlinearly generated light. Einstein’s photoelectron equation is an energy balancing equation. It does not incorporate the E-vector stimulation process before the quantum mechanically bound electrons can be released, which constitutes a key objective of physics. To introduce physics, we postulate that the photons are hybrid entities. They are discrete packets of energy hνmn at the moment of emission. Then they immediately evolve into spatially spreading diffractive wave packets to accommodate Huygens-Fresnel principle. HF principle has been behind the sustained progress in classical optics and photonics engineering. Thus a spatially spread out single wave-packet cannot any more deliver the necessary quantum cupful of energy hνmn to Angstrom-size detecting atoms. We need simultaneous stimulation of the same quantum entity by multiple wave packets. This model of physical interaction process naturally brings into play the significance of the degree of mutual coherence between different photon wave packets, along with their time varying amplitudes that are simultaneously stimulating the detecting quantum entities during any time-interval selected for the detection system. The superposition effects on the detector due to these phase and amplitude fluctuations are the physics-reasons behind the generation of different statistical variations in the photoelectron counts due to different kinds of sources even though the original photons are released randomly by all quantum sources.