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Chinese Physics

Saturation effects on Ba 6pnl(l=0,2) and 6pnk(|M| =0,1) autoionization spectra

Shiben Li, Dai Chang-Jian

Published Jan 24, 2007• 8 citations
Publisher

Abstract

Using a three-step laser saturation excitation technique, the saturation effects on the Ba 6p n s ( J = 1) and 6p n d ( J = 1, 3) autoionization spectra are observed systemically in zero field. These saturation spectra are introduced to determine the high n members of 6p nl ( l = 0, 2) autoionizing series and are used to analyse the channel interactions among the autoionizing series in zero field. Furthermore, the saturation excitation technique is applied to the electric field case, in which the saturation spectra of Ba 6p nk (| M | = 0, 1) autoionizing Stark states are measured. Most of these saturation spectra are observed for the first time so far as we know, which indicate the mixing of the autoionizing states in the electric fields.

DOI
10.1088/1009-1963/16/2/018

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Using a three-step laser saturation excitation technique, the saturation effects on the Ba 6p n s ( J = 1) and 6p n d ( J = 1, 3) autoionization spectra are observed systemically in zero field. These saturation spectra are introduced to determine the high n members of 6p nl ( l = 0, 2) autoionizing series and are used to analyse the channel interactions among the autoionizing series in zero field. Furthermore, the saturation excitation technique is applied to the electric field case, in which the saturation spectra of Ba 6p nk (| M | = 0, 1) autoionizing Stark states are measured. Most of these saturation spectra are observed for the first time so far as we know, which indicate the mixing of the autoionizing states in the electric fields.
In the study of Yb atomic Rydberg states, new members of 6sns 1 S 0 series for n=23, 24, 66-116 and 6snd 1 D 2 series for n=81-114 were observed. The data are in excellent agreement with the MQDT analysing results. The autoionizing Rydberg series 6p 1 2 /n's ( 1/2 , 1/2 ) 1 0 were investigated by three-step laser excitation. The ICE model was used to explain the experimental spectrum, and it has been proved to be suitable for describing the excitation of the autoionizing Rydberg states with a weakly-excited core.
The first detailed observation of the perturbations by an electric field of the Rydberg autoionizing resonances of a rare-gas atom is reported. The Stark spectroscopy of autoionizing Rydberg states converging to the second ionization limit $4{p}^{5}^{2}P_{\frac{1}{2}}^{o}$ in Kr I is performed in an atomic beam with the use of a two-step laser excitation from the 4p55s[32]204{p}^{5}5s{[\frac{3}{2}]}_{2}^{0}4p55s[23​]20​ metastable state. In addition to the verification of the ${({n}^{*})}^{\ensuremath{-}3}$ dependence of the zero-field width of two autoionizing series and of the linear dependence of the Stark-manifold splittings with the electric field, we have observed an (n)0.7{(n)}^{0.7}(n)0.7 law for the dependence of the Stark-manifold splitting along the series, an important narrowing and dissymmetrization of the $n{d}^{\ensuremath{'}}$ resonances, and a nonlinear-field behavior of Stark-manifold components in the vicinity of the first anticrossing. Discussions are carried out with the use of the recent work on Rydberg-Stark spectroscopy and on autoionizing states in two-electron atoms.
We report the effects of static electric fields on the doubly excited 6p12nl6{p}_{\frac{1}{2}}\mathrm{nl}6p21​​nl states of barium in the region n∗=12{n}^{*}=12n∗=12. Using a three-step laser excitation scheme we have measured the electric-field dependence of the positions and autoionization widths of the $6{p}_{\frac{1}{2}}\ensuremath{-}17s,16p,15d,12l (l=4\ensuremath{-}10),12f, \mathrm{and} 16s$ states at field values of up to 4.92 kV/cm. The photoexcitation spectra of the autoionizing states exhibit interference effects which are well understood and provide a better understanding of the character of these states in electric fields. The systematic study of the spectra and positions allows us to explain the field dependence of the autoionization widths in terms of electric-field mixing of the discrete portions of the auoionizing states. The relationship of these effects to dielectronic recombination rates of ions and electrons in plasma microfields is discussed.