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Physical Review A

Cooperative spontaneous emission of N atoms: Many-body eigenstates, the effect of virtual Lamb shift processes, and analogy with radiation of N classical oscillators

Anatoly A. Svidzinsky, Juntao Chang, Marlan O. Scully

Published May 13, 2010• 239 citations
Publisher

Abstract

We consider collective emission of a single photon from a cloud of $N$ two-level atoms (one excited, $N\ensuremath{-}1$ ground state). For a dense cloud the problem is reduced to finding eigenfunctions and eigenvalues of an integral equation. We discuss an exact analytical solution of this many-atom problem for a spherically symmetric atomic cloud. Some eigenstates decay much faster then the single atom decay rate, while the others undergo very slow decay. We show that virtual processes yield a small effect on the evolution of rapidly decaying states. However, they change the long time dynamics from exponential decay into a power-law behavior which can be observed experimentally. For trapped states virtual processes are much more important yielding additional decay channels which results in a slow decay of the otherwise trapped states. We also show that quantum mechanical treatment of spontaneous emission of weakly excited atomic ensemble is analogous to emission of $N$ classical harmonic oscillators.

DOI
10.1103/physreva.81.053821

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We consider collective emission of a single photon from a cloud of NNN two-level atoms (one excited, N\ensuremath−1N\ensuremath{-}1N\ensuremath−1 ground state). For a dense cloud the problem is reduced to finding eigenfunctions and eigenvalues of an integral equation. We discuss an exact analytical solution of this many-atom problem for a spherically symmetric atomic cloud. Some eigenstates decay much faster then the single atom decay rate, while the others undergo very slow decay. We show that virtual processes yield a small effect on the evolution of rapidly decaying states. However, they change the long time dynamics from exponential decay into a power-law behavior which can be observed experimentally. For trapped states virtual processes are much more important yielding additional decay channels which results in a slow decay of the otherwise trapped states. We also show that quantum mechanical treatment of spontaneous emission of weakly excited atomic ensemble is analogous to emission of NNN classical harmonic oscillators.
We study emission of a single photon from a spherically symmetric cloud of NNN atoms (one atom is excited; $N\ensuremath{-}1$ are in the ground state) and present an exact analytical expression for eigenvalues and eigenstates of this many-body problem. We found that some states decay much faster than the single-atom decay rate, while other states are trapped and undergo very slow decay. When the size of the atomic cloud is small compared with the radiation wavelength, we found that the radiation frequency undergoes a large shift.
We consider collective spontaneous emission from an ensemble of N identical two-level atoms prepared by absorption of a single photon–a.k.a. single photon Dicke superradiance. We discuss dynamical properties of superradiance for small (R ≪ λ) and large (R ≫ λ) atomic cloud. Moreover, we address the effects of virtual processes on collective decay rate and Lamb shift. It turns out that virtual processes lead to relatively small yet interesting effects on the time evolution of a rapidly decaying state. However, such processes substantially modify the dynamics of trapped states by bringing in new channels of decay.
We present analytical solutions for the evolution of collective states of N atoms. On the one hand is a (timed) Dicke state prepared by absorption of a single photon and exhibiting superradiant decay. This is in strong contrast to evolution of a symmetric Dicke state which is trapped for large atomic clouds. We show that virtual processes yield a small effect on the evolution of the rapidly decaying timed Dicke state. However, they change the long time dynamics from exponential decay into a power-law behavior which can be observed experimentally. For trapped states virtual processes are much more important and provide new decay channels resulting in a slow decay of the otherwise trapped state.
A landmark in the development of quantum electrodynamics was the discovery that emission–reabsorption of virtual photons modifies the value of energy levels in an atom from those computed by using Dirac’s equation (Lamb shift). An early result of statistical quantum electrodynamics was that the exchange of virtual photons in an ensemble of identical atoms leads as well to a change in the frequency of the radiation emitted from this system (cooperative Lamb shift). Dicke’s discovery that coherence effects lead to the shortening of the emission lifetime from a small sample by a factor equal to the number of atoms in the ensemble (superradiance or cooperative decay rate) was an early landmark in quantum optics. Both cooperative decay rate and cooperative Lamb shift were shown to have the same physical origin—the exchange of virtual photons, a process described by the Lienard–Wiechert dipole–dipole interaction. This effective potential is the kernel of the integral equation describing the dynamics of the system. This complex long-range kernel gives, for both cooperative quantities, strong dependence on the geometry of the atomic cloud. I summarize the known expressions for the initial cooperative decay rate and the cooperative Lamb shift in different geometries. The results for both the scalar photon and the vector photon (electrodynamics) theories for experimentally realizable systems of either uniform or phased polarization are given.
We study the correlated spontaneous emission from a dense spherical cloud of N atoms uniformly excited by absorption of a single photon. We find that the decay of such a state depends on the relation between an effective Rabi frequency Omega proportional square root N and the time of photon flight through the cloud R/c. If OmegaR/c<1 the state exponentially decays with rate Omega(2)R/c and the state lifetime is greater than R/c. In the opposite limit OmegaR/c>>1, the coupled atom-radiation system oscillates between the collective Dicke state (with no photons) and the atomic ground state (with one photon) with frequency Omega while decaying at a rate c/R.
The collective nature of light emission by atomic ensembles yields fascinating effects such as superradiance and radiation trapping even at the single-photon level. Light emission is influenced by virtual transitions and the collective Lamb shift which yields peculiar features in temporal evolution of the atomic system. We study how two-dimensional atomic structures collectively emit a single photon. Namely, we consider spherical, cylindrical, and spheroidal shells with two-level atoms continuously distributed on the shell surface and find exact analytical solutions for eigenstates of such systems and their collective decay rates and frequency shifts. We identify states which undergo superradiant decay and states which are trapped and investigate how size and shape of the shell affects collective light emission. Our findings could be useful for quantum information storage and the design of optical switches.