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arXiv:0804.3767 · Physical Review Letters

Dynamical Evolution of Correlated Spontaneous Emission of a Single Photon from a Uniformly Excited Cloud of N Atoms

Anatoly A. Svidzinsky, Juntao Chang, Marlan O. Scully

Published Apr 22, 2008• 157 citations
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Abstract

We study the correlated spontaneous emission from a dense spherical cloud of N atoms uniformly excited by absorption of a single photon. We find that the decay of such a state depends on the relation between an effective Rabi frequency Omega proportional square root N and the time of photon flight through the cloud R/c. If OmegaR/c<1 the state exponentially decays with rate Omega(2)R/c and the state lifetime is greater than R/c. In the opposite limit OmegaR/c>>1, the coupled atom-radiation system oscillates between the collective Dicke state (with no photons) and the atomic ground state (with one photon) with frequency Omega while decaying at a rate c/R.

DOI
10.1103/physrevlett.100.160504

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We study the correlated spontaneous emission from a dense spherical cloud of N atoms uniformly excited by absorption of a single photon. We find that the decay of such a state depends on the relation between an effective Rabi frequency Omega proportional square root N and the time of photon flight through the cloud R/c. If OmegaR/c<1 the state exponentially decays with rate Omega(2)R/c and the state lifetime is greater than R/c. In the opposite limit OmegaR/c>>1, the coupled atom-radiation system oscillates between the collective Dicke state (with no photons) and the atomic ground state (with one photon) with frequency Omega while decaying at a rate c/R.
We consider collective spontaneous emission from an ensemble of N identical two-level atoms prepared by absorption of a single photon–a.k.a. single photon Dicke superradiance. We discuss dynamical properties of superradiance for small (R ≪ λ) and large (R ≫ λ) atomic cloud. Moreover, we address the effects of virtual processes on collective decay rate and Lamb shift. It turns out that virtual processes lead to relatively small yet interesting effects on the time evolution of a rapidly decaying state. However, such processes substantially modify the dynamics of trapped states by bringing in new channels of decay.
We study emission of a single photon from a spherically symmetric cloud of NNN atoms (one atom is excited; $N\ensuremath{-}1$ are in the ground state) and present an exact analytical expression for eigenvalues and eigenstates of this many-body problem. We found that some states decay much faster than the single-atom decay rate, while other states are trapped and undergo very slow decay. When the size of the atomic cloud is small compared with the radiation wavelength, we found that the radiation frequency undergoes a large shift.
We consider collective emission of a single photon from a cloud of NNN two-level atoms (one excited, $N\ensuremath{-}1$ ground state). For a dense cloud the problem is reduced to finding eigenfunctions and eigenvalues of an integral equation. We discuss an exact analytical solution of this many-atom problem for a spherically symmetric atomic cloud. Some eigenstates decay much faster then the single atom decay rate, while the others undergo very slow decay. We show that virtual processes yield a small effect on the evolution of rapidly decaying states. However, they change the long time dynamics from exponential decay into a power-law behavior which can be observed experimentally. For trapped states virtual processes are much more important yielding additional decay channels which results in a slow decay of the otherwise trapped states. We also show that quantum mechanical treatment of spontaneous emission of weakly excited atomic ensemble is analogous to emission of NNN classical harmonic oscillators.
The collective Lamb shift and associated radiative decay of a large cloud of radius R containing N atoms uniformly excited by one photon of wavelength lambda is analyzed. It is shown that the time evolution of the symmetric state prepared by single photon absorption in the limit R>>lambda is similar to that encountered in the Dicke limit of small sample (R<<lambda) superradiance. The theory includes virtual (counterrotating) terms naturally and thus provides a simple calculation of the collective Lamb shift of a single Dicke state.
We study the collective spontaneous emission of a linear atomic chain excited by a single photon. The interaction between the atoms and the common vacuum field can significantly change the eigenenergy and the spontaneous emission rate of the system. Due to the dipole-dipole interactions, the system prepared in a single-photon timed Dicke state is the superposition of superradiant and subradiant eigenstates that can have a nonexponential decay dynamics. We can tune the frequency and linewidth of the superradiant and subradiant emission from a timed Dicke state by changing the direction of the atomic dipole moment or the atomic separation. In addition, the emission direction of the superradiant and subradiant photons also depends on the polarization of the atoms.
In this work we present a numerical and experimental investigation of the collective early-time decay rates of a strongly driven and optically dense cold atomic cloud. We prepare the atomic ensemble by driving the system to its steady state with varying Rabi frequencies ΩΩΩ that go from the weak Ω≪ΓΩ\ll ΓΩ≪Γ to the strong driving regime Ω≫ΓΩ\gg ΓΩ≫Γ, where ΓΓΓ is the single-atom decay rate. We investigate the early-time dynamics in the transition between the strong and weak driving regimes using: i) angular-dependent observables such as the light emitted by the cloud, and ii) global observables, i.e., the excited state population. When driving the cloud on-resonance, we find that as a function of the driving frequency, the behavior of the collected light at certain angles transitions from the single-photon subradiant regime to a superradiant regime while the behavior of the excited state population does not show superradiance. The experiment shows good agreement with numerical predictions in the regime of parameters under study.