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Physical Review A

Single-photon superradiance and radiation trapping by atomic shells

Anatoly A. Svidzinsky, Fu Li, Hongyuan Li, Xiwen Zhang, C. H. Raymond Ooi, Marlan O. Scully

Published Apr 18, 2016• 20 citations
Publisher

Abstract

The collective nature of light emission by atomic ensembles yields fascinating effects such as superradiance and radiation trapping even at the single-photon level. Light emission is influenced by virtual transitions and the collective Lamb shift which yields peculiar features in temporal evolution of the atomic system. We study how two-dimensional atomic structures collectively emit a single photon. Namely, we consider spherical, cylindrical, and spheroidal shells with two-level atoms continuously distributed on the shell surface and find exact analytical solutions for eigenstates of such systems and their collective decay rates and frequency shifts. We identify states which undergo superradiant decay and states which are trapped and investigate how size and shape of the shell affects collective light emission. Our findings could be useful for quantum information storage and the design of optical switches.

DOI
10.1103/physreva.93.043830

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The collective nature of light emission by atomic ensembles yields fascinating effects such as superradiance and radiation trapping even at the single-photon level. Light emission is influenced by virtual transitions and the collective Lamb shift which yields peculiar features in temporal evolution of the atomic system. We study how two-dimensional atomic structures collectively emit a single photon. Namely, we consider spherical, cylindrical, and spheroidal shells with two-level atoms continuously distributed on the shell surface and find exact analytical solutions for eigenstates of such systems and their collective decay rates and frequency shifts. We identify states which undergo superradiant decay and states which are trapped and investigate how size and shape of the shell affects collective light emission. Our findings could be useful for quantum information storage and the design of optical switches.
The collective nature of light emission by atomic ensembles yields fascinating effects such as superradiance and radiation trapping even at the single-photon level.Light emission is influenced by virtual transitions and the collective Lamb shift which yields peculiar features in temporal evolution of the atomic system.We study how two-dimensional atomic structures collectively emit a single photon.Namely, we consider spherical, cylindrical, and spheroidal shells with two-level atoms continuously distributed on the shell surface and find exact analytical solutions for eigenstates of such systems and their collective decay rates and frequency shifts.We identify states which undergo superradiant decay and states which are trapped and investigate how size and shape of the shell affects collective light emission.Our findings could be useful for quantum information storage and the design of optical switches.
Superradiance is one of the many fascinating phenomena predicted by quantum electrodynamics that have first been experimentally demonstrated in atomic systems and more recently in condensed matter systems like quantum dots, superconducting q-bits, cyclotron transitions and plasma oscillations in quantum wells (QWs). It occurs when a dense collection of N identical two-level emitters are phased via the exchange of photons, giving rise to enhanced light-matter interaction, hence to a faster emission rate. Of great interest is the regime where the ensemble interacts with one photon only and therefore all of the atoms, but one, are in the ground state. In this case the quantum superposition of all possible configurations produces a symmetric state that decays radiatively with a rate N times larger than that of the individual oscillators. This phenomenon, called single photon superradiance, results from the exchange of real photons among the N emitters. Yet, to single photon superradiance is also associated another collective effect that renormalizes the emission frequency, known as cooperative Lamb shift. In this work, we show that single photon superradiance and cooperative Lamb shift can be engineered in a semiconductor device by coupling spatially separated plasma resonances arising from the collective motion of confined electrons in QWs. These resonances hold a giant dipole along the growth direction z and have no mutual Coulomb coupling. They thus behave as a collection of macro-atoms on different positions along the z axis. Our device is therefore a test bench to simulate the low excitation regime of quantum electrodynamics.
Superradiance, the cooperative spontaneous emission of photons from an ensemble of identical atoms, provides valuable insights into the many-body physics of photons and atoms. We show that an ensemble of resonant atoms embedded in the center of a planar cavity can be collectively excited by synchrotron radiation into a purely superradiant state. The collective coupling of the atoms via the radiation field leads to a substantial radiative shift of the transition energy, the collective Lamb shift. We simultaneously measured the temporal evolution of the superradiant decay and the collective Lamb shift of resonant 57Fe nuclei excited with 14.4-kilo-electron volt synchrotron radiation. Our experimental technique provides a simple method for spectroscopic analysis of the superradiant emission.
We consider collective spontaneous emission from an ensemble of N identical two-level atoms prepared by absorption of a single photon–a.k.a. single photon Dicke superradiance. We discuss dynamical properties of superradiance for small (R ≪ λ) and large (R ≫ λ) atomic cloud. Moreover, we address the effects of virtual processes on collective decay rate and Lamb shift. It turns out that virtual processes lead to relatively small yet interesting effects on the time evolution of a rapidly decaying state. However, such processes substantially modify the dynamics of trapped states by bringing in new channels of decay.
In an ensemble of identical atoms, cooperative effects like sub- and superradiance may alter the decay rates and the energies of specific transitions may be shifted from the single-atom value by the so-called collective Lamb shift. While such effects in ensembles of two-level systems are by now well understood, realistic multilevel systems are more difficult to handle. In this work we show that in a system of atoms under the action of an external magnetic field, the collective contribution to the level shifts can amount to sizable quantitative and qualitative deviations from the single-atom Zeeman splitting picture. We develop a formalism to describe single-photon superradiance in multilevel systems and identify three-parameter regimes, two of which present measurable deviations in the radiation spectrum compared to the case of single-atom magnetic-field-induced splitting.
Ensembles of dipolar emitters which couple collectively to the radiation field display sub- and superradiance. These terms refer to a reduction or an enhancement of photon emission rates due to the interference of emission channels. Arrays of trapped neutral atoms constitute a promising platform for harnessing this phenomenon in technological applications, e.g., for excitation storage, single-photon switches, and mirrors. However, quantum and thermally induced vibrations of the atoms within their traps lead to position fluctuations that entangle the motion and the internal atomic degrees of freedom. We develop here a theory for collective atom-light coupling in the presence of this quantized motion within the Lamb-Dicke limit. We show the existence of sub- and superradiant states that are hybrids of electronic and vibrational excitations, investigate their properties for analytically and numerically efficiently solvable cases, and discuss how a finite temperature affects the collective photon emission.