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Physical Review A

Wavelength dependence of coherently induced transparency in a Doppler-broadened cascade medium

Sara Shepherd, David J. Fulton, Malcolm H. Dunn

Published Dec 1, 1996• 81 citations
Publisher

Abstract

The effect of changing the coupling laser transition, and hence the wavelength, on the coherently induced transparency seen by a probe beam in a Doppler-broadened cascade electromagnetically induced transparency (EIT) configuration is studied experimentally and theoretically. The transparency of the vapor is shown to be an effect not just of EIT, but of the varying Autler-Townes splitting for each velocity group within the vapor. Consequently, the best overall transparency for Rabi splittings less than the Doppler width is not at the position of matched coupling and probe wavelengths, but for coupling wavelengths less than that of the probe. \textcopyright{} 1996 The American Physical Society.

DOI
10.1103/physreva.54.5394

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Recently it was predicted, and shown experimentally, that a cw coherently induced transparency feature could be observed in a Doppler-broadened cascade medium even when the probe and coupling fields had a wavelength mismatch of several hundred nanometers.1 This observation is significant since it removes the requirement for finding wavelength-matched systems to carry out cw atomic coherence experiments within an inhomogeneously broadened medium.2,3 The explanation of this transparency lies with the fact that both E.I.T. and Autler-Townes splitting4 are velocity group dependent. Each velocity group experiences its own Doppler-shift and hence detuning from the probe and coupling field transitions. Therefore, there exists a variation in the frequency position of maximum E.I.T. and of the Autler-Townes split components for each velocity groups. It is the integration of both of these effects over all of the velocity groups that produces the overall probe absorption.

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Comparison of wavelength dependence in cascade-, Λ-, and Vee-type schemes for electromagnetically induced transparency

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We present a theoretical study of the effects of mismatching wavelengths for the coupling and probe fields in Doppler-broadened media for the three basic energy level configurations commonly used to realize electromagnetically induced transparency (EIT). Three wavelength regimes are considered: mismatched wavelengths for which the coupling frequency is greater than the probe frequency, matched wavelengths for which the coupling and probe frequencies are equal, and mismatched wavelengths for which the probe frequency is greater than the coupling frequency. The transparency that may be induced in these regimes is compared for the cascade-, \ensuremath{\Lambda}-, and Vee-type systems. We show that in the first mismatched regime $({\ensuremath{\lambda}}_{c}<{\ensuremath{\lambda}}_{p})$ EIT is possible in all schemes and is in fact stronger than in the matched case. It is also demonstrated that for the second mismatched regime $({\ensuremath{\lambda}}_{c}>{\ensuremath{\lambda}}_{p})$ EIT can be realized most readily in the Vee-type configuration in the presence of Doppler broadening. These predictions are explained by considering the absorption as a function of both the probe field detuning and the atomic velocity.

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We study the relationship between electromagnetically-induced transparency(EIT) and Autler–Townes(AT) splitting in a cascade three-level Doppler-broadened system. By comparing the absorption spectrum with the fluorescence excitation spectrum, it is found that for a Doppler-broadened system, EIT resonance cannot be explained as the result of quantum interference, unlike the case of a homogeneously broadened system. Instead, the macroscopic polarization interference plays an important role in determining the spectra of EIT and AT splitting, which can be explained within the same framework when being detected by the absorption spectra.

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Influence of Doppler effect on the phenomenon of electromagnetically induced transparency

Qiyong Tao, Guiyin Zhang, Haiming Zheng

Electromagnetically induced transparency (EIT) is a significant nonlinear optical phenomenon. Based on the theory of density matrix equation, we presented the influence of Doppler effect on EIT. A cascade type three-level system and Na atomic vapor is adopted during the course. The results showed that EIT is determined by Rabi frequency of the couple and probing field. It is independent of temperature usually. But when we take Doppler effect into account, it is found that the full transparency appeared at the condition of ΩP=0.01GHz, ΩC=1GHz will vary with temperature. An obvious transparent window can be observed only when the temperature is less than 50K. With the increase of temperature, EIT phenomenon disappeared quickly. At room temperature, we can see that the double peaks of Aulter-Townes will instead of the EIT transparent window as Rabi frequency of the couple field is larger than 1.5GHz.

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Abstract We develop an analytical approach on electromagnetically induced transparency (EIT) in a Doppler broadened medium consisting of five-level cascade systems excited by a strong coupling and weak probe laser fields. In a weak field limit of the probe light, EIT spectrum is interpreted as functions of controllable parameters of the coupling light and temperature of the medium. The theoretical interpretation of EIT spectrum is applied to the case of 85 Rb atoms and compared with available experimental observation. Such an analytical interpretation provides quantitative parameters to control properties of the Doppler broadened EIT medium, and it is useful to find related applications.

Physica Scripta•Feb 1, 2016•28 citations
The effect of changing the coupling laser transition, and hence the wavelength, on the coherently induced transparency seen by a probe beam in a Doppler-broadened cascade electromagnetically induced transparency (EIT) configuration is studied experimentally and theoretically. The transparency of the vapor is shown to be an effect not just of EIT, but of the varying Autler-Townes splitting for each velocity group within the vapor. Consequently, the best overall transparency for Rabi splittings less than the Doppler width is not at the position of matched coupling and probe wavelengths, but for coupling wavelengths less than that of the probe. \textcopyright{} 1996 The American Physical Society.
Recently it was predicted, and shown experimentally, that a cw coherently induced transparency feature could be observed in a Doppler-broadened cascade medium even when the probe and coupling fields had a wavelength mismatch of several hundred nanometers.1 This observation is significant since it removes the requirement for finding wavelength-matched systems to carry out cw atomic coherence experiments within an inhomogeneously broadened medium.2,3 The explanation of this transparency lies with the fact that both E.I.T. and Autler-Townes splitting4 are velocity group dependent. Each velocity group experiences its own Doppler-shift and hence detuning from the probe and coupling field transitions. Therefore, there exists a variation in the frequency position of maximum E.I.T. and of the Autler-Townes split components for each velocity groups. It is the integration of both of these effects over all of the velocity groups that produces the overall probe absorption.
We present a theoretical study of the effects of mismatching wavelengths for the coupling and probe fields in Doppler-broadened media for the three basic energy level configurations commonly used to realize electromagnetically induced transparency (EIT). Three wavelength regimes are considered: mismatched wavelengths for which the coupling frequency is greater than the probe frequency, matched wavelengths for which the coupling and probe frequencies are equal, and mismatched wavelengths for which the probe frequency is greater than the coupling frequency. The transparency that may be induced in these regimes is compared for the cascade-, \ensuremath{\Lambda}-, and Vee-type systems. We show that in the first mismatched regime $({\ensuremath{\lambda}}_{c}<{\ensuremath{\lambda}}_{p})$ EIT is possible in all schemes and is in fact stronger than in the matched case. It is also demonstrated that for the second mismatched regime $({\ensuremath{\lambda}}_{c}>{\ensuremath{\lambda}}_{p})$ EIT can be realized most readily in the Vee-type configuration in the presence of Doppler broadening. These predictions are explained by considering the absorption as a function of both the probe field detuning and the atomic velocity.
We study the relationship between electromagnetically-induced transparency(EIT) and Autler–Townes(AT) splitting in a cascade three-level Doppler-broadened system. By comparing the absorption spectrum with the fluorescence excitation spectrum, it is found that for a Doppler-broadened system, EIT resonance cannot be explained as the result of quantum interference, unlike the case of a homogeneously broadened system. Instead, the macroscopic polarization interference plays an important role in determining the spectra of EIT and AT splitting, which can be explained within the same framework when being detected by the absorption spectra.
Electromagnetically induced transparency (EIT) is a significant nonlinear optical phenomenon. Based on the theory of density matrix equation, we presented the influence of Doppler effect on EIT. A cascade type three-level system and Na atomic vapor is adopted during the course. The results showed that EIT is determined by Rabi frequency of the couple and probing field. It is independent of temperature usually. But when we take Doppler effect into account, it is found that the full transparency appeared at the condition of ΩP=0.01GHz, ΩC=1GHz will vary with temperature. An obvious transparent window can be observed only when the temperature is less than 50K. With the increase of temperature, EIT phenomenon disappeared quickly. At room temperature, we can see that the double peaks of Aulter-Townes will instead of the EIT transparent window as Rabi frequency of the couple field is larger than 1.5GHz.
We describe in this Letter how inhomogeneous line broadening affects the Autler-Townes (AT) splitting in a three level open molecular cascade system. For moderate Rabi frequencies in the range of 300 to 500 MHz the fluorescence line shape from the uppermost level |3> in this system depends strongly on the frequency ratio of the two laser fields. However, the fluorescence spectrum of the intermediate level |2> appears as expected. We provide a description of the conditions for optimally resolved AT splitting in terms of the probe laser/coupling field frequency ratio and laser propagation geometry based on our theoretical analysis of the Doppler integral. This is important for applications such as molecular angular momentum alignment as well as for the measurement of the transition dipole moment matrix element.
Abstract We develop an analytical approach on electromagnetically induced transparency (EIT) in a Doppler broadened medium consisting of five-level cascade systems excited by a strong coupling and weak probe laser fields. In a weak field limit of the probe light, EIT spectrum is interpreted as functions of controllable parameters of the coupling light and temperature of the medium. The theoretical interpretation of EIT spectrum is applied to the case of 85 Rb atoms and compared with available experimental observation. Such an analytical interpretation provides quantitative parameters to control properties of the Doppler broadened EIT medium, and it is useful to find related applications.