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Physical Review Letters

Control of Localization and Suppression of Tunneling by Adiabatic Passage

Nicolas Sangouard, S. Guérin, M. Amniat-Talab, Hans Rudolf Jauslin

Published Nov 24, 2004• 18 citations
Publisher

Abstract

We show that a field of frequency omega combined with its second harmonic 2omega driving a double-well potential allows us to localize the wave packet by adiabatic passage, starting from the delocalized ground state. The relative phase of the fields allows us to choose the well of localization. We can suppress (and restore) the tunneling subsequently by switching on (and off) abruptly the fields at well-defined times. The mechanism relies on the fact that the dynamics is driven to an eigenstate of the Floquet Hamiltonian which is a localized state.

DOI
10.1103/physrevlett.93.223602

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We show that a field of frequency omega combined with its second harmonic 2omega driving a double-well potential allows us to localize the wave packet by adiabatic passage, starting from the delocalized ground state. The relative phase of the fields allows us to choose the well of localization. We can suppress (and restore) the tunneling subsequently by switching on (and off) abruptly the fields at well-defined times. The mechanism relies on the fact that the dynamics is driven to an eigenstate of the Floquet Hamiltonian which is a localized state.
The second-order perturbation theory in the framework of the Kramers-Henneberger oscillating frame representation of the Hamiltonian [H. A. Kramers, Quantum Mechanics (North-Holland, Amsterdam, 1956); W. C. Henneberger, Phys. Rev. Lett. 21, 838 (1968)] is used to study the tunneling process in a periodically driven double-well potential. The eigenstates of the Floquet Hamiltonian are efficiently approximated when a field frequency is larger than a classical frequency of the time-averaged Hamiltonian. The conditions for coherent enhancement and suppression of tunneling are obtained when the standard perturbation theory fails. It is shown that the enhancement and suppression of tunneling is due to field-induced coupling between states of a one-period averaged effective potential.
The effect of a periodic driving force on coherent tunneling of a driven double square-well system, especially when its central potential barrier is very tall and very thin, is investigated. The suppression or enhancement of the tunneling of a wave packet properly chosen in the double-well system may be achieved by a judicious choice of the period of a driving force, i.e., by a particular choice of the generating condition of a nonlinear resonance exhibiting a desirable property. We analyze this mechanism by exploiting both the properties of a dynamical symmetry of the Hamiltonian and the localized properties of Floquet states induced by the nonlinear resonance. \textcopyright{} 1996 The American Physical Society.
A periodically driven two-state dynamics, being analysed within the Floquet formalism, exhibits localization of the amplitude dynamics in an infinite frequency range, extending from the bare tunnel splitting up to infinity. In contrast, the suppression of tunnelling in a driven symmetric double well is restricted to a limited frequency regime, extending from the bare tunnel splitting up to the first resonance frequency with higher-lying states. With the amplitude dynamics of a periodically driven two-level system not being restricted to describe coherent tunnelling transport only, the localization phenomenon within the infinite frequency range does allow for novel applications for systems in strong laser fields.
The roles of spatial symmetry and strength of external time-dependent perturbation on the dynamics of a quantum particle, initially localized in one of the wells of an asymmetric double-well potential are studied using the recently developed techniques incorporating quantum theory of motion and time-dependent Fourier grid Hamiltonian methods. The model used here includes a mimic of the related experimental situations which is considered as a perturbation to the static double-well potential. Analysis of localized and delocalized phase space structures and corresponding time-profile of tunneling probability reveal the recipe toward controlling the tunneling oscillations by modulating the parameters of applied perturbation. A study on a stochastic pulsating potential also reveals the root to the quantum localization, even in moderate field strength.
Control of tunneling in a symmetric double well coupled to a bath via an external field is demonstrated. Optimal control theory is employed to design a laser field which couples to the reaction coordinate and drives a localized wave packet on the reactant side to the product side at a specified target time τ. Both a very quantumlike system (high barrier) and a low barrier double well are examined; excellent results are obtained for a range of reduced bath viscosities. Analysis of the control fields and corresponding localization dynamics shows that the frequency components of the control field are more or less in resonance with eigenstates of the double well and that the laser field enhances the natural dynamics of the individual wells. Future extension to more complicated models where the field couples to the bath is discussed.