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Physical Review A

Atom-atom correlations via radiation-field coupling

Yves Gontier

Published Mar 1, 1997• 1 citation
Publisher

Abstract

It is shown that two identical systems, not interacting with each other but resonantly coupled with the same intense radiation field, can be correlated. The case of a pair of two-level atoms is quantitatively investigated by calculating the probability for the emission of a photon by one of the two atoms. One finds that the presence of the other atom strongly affects the shape of the resonance curve. It is concluded that this effect, called signal transmission by means of optical correlations, if observable, could be the way for transmitting information between the atoms without resorting to any modulation of the field amplitude.

DOI
10.1103/physreva.55.2397

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It is shown that two identical systems, not interacting with each other but resonantly coupled with the same intense radiation field, can be correlated. The case of a pair of two-level atoms is quantitatively investigated by calculating the probability for the emission of a photon by one of the two atoms. One finds that the presence of the other atom strongly affects the shape of the resonance curve. It is concluded that this effect, called signal transmission by means of optical correlations, if observable, could be the way for transmitting information between the atoms without resorting to any modulation of the field amplitude.
The correlations arising between identical atoms resonantly coupled with the same radiation field are studied within a fully quantized theory. The atoms do not interact with each other and may be widely separated. We study how a modulation of the atom-field parameter of any one atom is transmitted to the others. This exchange of informations between remote systems was predicted in a previous account in the case of two atoms (signal transmission by optical correlations). In this paper, the theory is generalized to more than two atoms in order to model the effect of onlooker atoms. Outlines of experiments enabling investigation of the observability of these correlations and the applications that can be made are presented.
The normalised intensity correlation function of resonance fluorescence radiation from two-level atoms is studied in various respects. In the first part of the paper the author discusses only interference effects for several uncoupled, linearly arranged, atoms. It is shown that, depending on the distance between the atoms, the direction of observation and the strength of the driving field, an antibunching effect as well as a very big bunching effect may be observed. In the second part of the paper he studies for the case of two atoms and weak external fields the influence of the interaction between the atoms by means of a perturbation theory. It is shown that the coupling between the atoms strongly modifies the normalised intensity correlation function in comparison with the case of uncoupled atoms. He takes as the driving field a coherent external field as well as laser light and thermal light.
The interaction between electromagnetic radiation and two three-level atoms is investigated. The atom-atom separation is assumed to be smaller than the corresponding mean resonance wavelength. The total radiance rate of the atomic system is calculated as a function of time. Explicit results are given for several different initial states of the atomic system. Some of them exhibit superradiance, and some act as photon-trapping states. Instead of exponential decay, the oscillations appear in the time evolution of the radiation rate due to the correlation between atoms. The decay constants and coupling decay constants show strong effects on the emission rates. Completely differing from two identical double-level atoms, the cooperative effects always exist in the three-level atomic system except for the case in which the coupling decay constants ${\ensuremath{\gamma}}_{12}$ and ${\ensuremath{\gamma}}_{21}$ are zero.
A simple theoretical model is formulated which describes dynamical features of the interaction of two-level atoms with a continuum of radiation oscillators. In particular, this paper is concerned with resonance scattering by single atoms in the presence of an external classical field, and spontaneous emission by a system of identical atoms. In the case of resonance scattering, the response of an atom to rapid changes of the amplitude of the external field is studied. The model for spontaneous emission by a system of atoms is based on the assumptions that all atoms have the same resonance frequency, and that the atoms are contained in a volume whose extension is small compared with the wavelength of the emitted radiation. The complete evolution of a system of mmm atoms is determined by a set of coupled first-order linear differential equations, and explicit solutions are presented for the values m=1,2,3,4,and8m=1,2,3,4, \mathrm{and} 8m=1,2,3,4,and8. Pair correlations of the atoms and photon-number fluctuations are discussed. An approximation for resonance fluorescence by a system of atoms with a broad distribution of resonance frequencies is included in an Appendix.
The frequency distribution of resonant radiation emitted by a system of two identical interacting atoms is calculated. The separation between the atoms is assumed to be much larger than the size of their charge distributions. Initially one atom is excited while the second one is in the ground state. The two atoms are coupled through the radiation field and the electrostatic interaction. For not too large internuclear separations the line shape of the emitted radiation exhibits two distinct peaks, and the general features are identical with the result obtained from resonance fluorescence scattering. In the decay process, however, there is equal probability of scattering through the symmetric and antisymmetric states, and thus the peak heights of the emitted radiation are different from the ones in the resonance fluorescent case. For large internuclear separations the two peaks merge into the one characteristic of the line shape of a single isolated atom.
It is shown how certain classes of problems dealing with the interaction of radiation with atoms can be formulated in terms of four-operator perturbation series. The case of an isolated atom coupled to a single-mode field is discussed in detail within the resolvent formalism. The process where no photon is effectively absorbed by the atom is described, to all orders, in terms of a series involving four operators which simultaneously increase and/or decrease the photon number and the orbital quantum number. This series is exactly summed and the summation technique is generalized to single-atom, two-field and to two-atom, single-field systems exhibiting zero, one, and two net photon absorptions or emissions. The theory is applied to induced emission of a single photon from a pair of two-level atoms coupled to a monomode radiation field. The energy diagrams, the time dependence of the probability, and the resonance curves are discussed for systems where (i) both atoms are in the upper state and (ii) atom 1 is in the upper state and atom 2 is in the lower state at t=0. In comparing these results to the ones obtained with a single atom, we find that the important intensity-dependent correlations give rise to trapping effects even when the atoms are initially in the upper state.