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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

New nonlinear phenomena under conditions of strong selective reflection

Ya. A. Fofanov

Published Sep 10, 2010• 6 citations
Publisher

Abstract

This work is devoted to study of the strong selective reflection of obliquely incident laser beam (inclined geometry) from the interface "glass-rubidium vapour". It is shown that the contrast of the strongest refection resonances exceeds 500% at the moderate heating of reflecting cells. The new nonlinear properties of selective reflection resonances have been investigated - asymmetry of saturation of resonant total internal reflection (TIR) and nonlinear structures that appear under conditions close to resonant TIR. The observed structures can not be associated with well-known sub-Doppler resonances in selective reflection. The nonlinear structures described here do not have saturation properties in usual sense. They exist only in the inclined geometry and in a narrow range of saturating values of the surface power density at the interface. The transformation of the fluctuations of reflected light was also investigated at the optical saturation of selective reflection resonances. For this purpose the intensity of incident light was slightly modulated. The reduction of the corresponding intensity modulation was registered in the reflected light. This reduction of the intensity fluctuations ("classical squeezing") and the relatively high selective reflection coefficient offer good possibilities for the squeezing of quantum fluctuations in the reflected light. In the process of appropriate studies it was found that the reduction (squeezing) of photons (quantum) fluctuations in the reflected light beam is about of 5% in compare with the coherent light.

DOI
10.1117/12.882693

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Soviet Journal of Quantum Electronics•Mar 31, 1989•13 citations
This work is devoted to study of the strong selective reflection of obliquely incident laser beam (inclined geometry) from the interface "glass-rubidium vapour". It is shown that the contrast of the strongest refection resonances exceeds 500% at the moderate heating of reflecting cells. The new nonlinear properties of selective reflection resonances have been investigated - asymmetry of saturation of resonant total internal reflection (TIR) and nonlinear structures that appear under conditions close to resonant TIR. The observed structures can not be associated with well-known sub-Doppler resonances in selective reflection. The nonlinear structures described here do not have saturation properties in usual sense. They exist only in the inclined geometry and in a narrow range of saturating values of the surface power density at the interface. The transformation of the fluctuations of reflected light was also investigated at the optical saturation of selective reflection resonances. For this purpose the intensity of incident light was slightly modulated. The reduction of the corresponding intensity modulation was registered in the reflected light. This reduction of the intensity fluctuations ("classical squeezing") and the relatively high selective reflection coefficient offer good possibilities for the squeezing of quantum fluctuations in the reflected light. In the process of appropriate studies it was found that the reduction (squeezing) of photons (quantum) fluctuations in the reflected light beam is about of 5% in compare with the coherent light.
Nonlinear selective reflection of obliquely incident laser beam (inclined geometry) has been investigated. The new structures were detected on the tops of strong reflection resonances under conditions of optical saturation of the D2-lines in the natural mixture of rubidium isotopes. The detected nonlinear structures have not saturation properties in usual sense and exist only in the close area of saturating power density values. This phenomenon can be useful for the amplification the nonlinear characteristics of the optical interface in order to reduce the fluctuations of selective reflected light.
The transformation of intensity fluctuations accompanying the nonlinear resonance reflection of light from a glass-resonant gas interface is discussed. The illumination of the interface at angles close to the critical angle for total internal reflection is found to have certain advantages over orthogonal incidence. At the maximum of the strongest resonance, the reflected light intensity amounts to more than 50% of the incident light. In these conditions, a squeezing of the amplitude (photon) fluctuations is observed in the radiation generated by a semiconductor laser-nonlinear selective reflector system. A simple semiclassical theory adequately describes some important characteristics of this system: the shape of the reflection resonances, the strength of the saturation fields, and so on.
Nonlinear selective reflection from the interface YAG window-high density rubidium vapor in the high-temperature cell is studied at the transition 5S1/2_{1/2}1/2​-5P3/2_{3/2}3/2​. In the experiment tunable pump and probe lasers are used. The selective reflection spectra for the laser probe beam are investigated at four different rubidium atomic densities and five different pump beam intensities. The estimated dipole-dipole interaction-induced line broadening varies from 13.213.213.2 to 39.639.639.6 GHz, the measured pumped intensities change from 1.21.21.2 to 8.88.88.8 kW⋅\cdot⋅cm−2^{-2}−2. Growth of the pump intensity causes reduction of the magnitude and the width of the recorded selective reflection resonance. We suggest developing all-optical modulators on the basis of nonlinear selective reflection.
A series of reflection resonances formed by the hyperfine components of the D 2 -lines in the spectrum of the natural mixture of rubidium isotopes is studied. Passages from resonantly frustrated total internal reflection to resonance Brewster reflection caused by the frequency tuning of the incident light are demonstrated experimentally. The contrast of the strongest refection resonances exceeds 500% at the moderate heating of reflecting cells. The intensity of the reflected light changes in this case by more than 20 times. A theory is developed which is based on a two-level model for resonance atoms and Fresnel formulas for reflection coefficients. Numerical calculations based on the proposed theory confirm main experimental results.
We present an experimental study of nonlinear selective reflection at a dielectric--Cs-vapor interface, in a three-level cascade-up scheme. The nonlinear reflection at the Cs D2{\mathit{D}}_{2}D2​ resonance line is monitored in the presence of resonant irradiation at 621 nm or 658 nm (6P3/2{\mathit{P}}_{3/2}P3/2​\ensuremath{\rightarrow}8D5/2{\mathit{D}}_{5/2}D5/2​,9S1/2{\mathit{S}}_{1/2}S1/2​). Experimental reflection spectra with either counterpropagating or copropagating light beams are analyzed and compared with the theoretical predictions of F. Schuller et al. [Phys. Rev. A 47, 519 (1993)]. For a blue-detuned pump and copropagating geometry an alternative type of three-level coherent reflection resonances, specifically associated with desorbing atoms, is observed. Also observed is the nonlinear reflection associated with the off-resonant, two-photon dispersion of atoms moving parallel to the window surface. Probe beam saturation is responsible for the appearance of additional resonant features in reflection spectra. Finally we analyze crossover spectral resonances which arise from nondegenerate, four-wave-mixing processes induced by the combined influence of counterpropagating pump and probe beams, and the pump beam being partially reflected by the window.
Resonance lines of rubidium and cesium and injection lasers were used in a study of selective reflection from an interface between a transparent dielectric and an absorbing gas as a function of the angle of incidence of radiation and of its polarization, and of the concentration of atoms in a cell. Selective reflection resonances were observed against zero background when radiation was incident on the cell at the Brewster angle. The conditions for observation of selective frustrated total internal reflection (FTIR) were determined analytically and experimentally. The maximum reflection coefficient obtained was 95 ± 2%, which was 10 times greater than the nonresonant reflection coefficient. The spectral width of the region where FTIR was observed ranged from 0.1 to 1.5 cm − 1, depending on the concentration of atoms and the angle of incidence. The FTIR eifect was used to construct a selective component which made it possible to ensure narrow-band cw operation of an injection laser with an external resonator. Other potential applications of the FTIR effect in quantum electronics were also considered.