The development of an easy-to-operate light source emitting single photons has become a major driving force in the emerging field of quantum information technology. Here, we report on the application of a compact and user-friendly Stirling cryocooler in the field of nanophotonics. The Stirling cryocooler is used to operate a single quantum emitter constituted of a semiconductor quantum dot (QD) at a base temperature below 30 K. Proper vibration decoupling of the cryocooler and its surrounding enables free-space micro-photoluminescence spectroscopy to identify and analyze different charge-carrier states within a single quantum dot. As an exemplary application in quantum optics, we perform a Hanbury-Brown and Twiss experiment demonstrating a strong suppression of multi-photon emission events with g((2))(0) < 0.04 from this Stirling-cooled single quantum emitter under continuous wave excitation. Comparative experiments performed on the same quantum dot in a liquid helium (LHe)-flow cryostat show almost identical values of g((2))(0) for both configurations at a given temperature. The results of this proof of principle experiment demonstrate that low-vibration Stirling cryocoolers that have so far been considered exotic to the field of nanophotonics are an attractive alternative to expensive closed-cycle cryostats or LHe-flow cryostats, which could pave the way for the development of high-quality table-top non-classical light sources.
The development of an easy-to-operate light source emitting single photons has become a major driving force in the emerging field of quantum information technology. Here, we report on the application of a compact and user-friendly Stirling cryocooler in the field of nanophotonics. The Stirling cryocooler is used to operate a single quantum emitter constituted of a semiconductor quantum dot (QD) at a base temperature below 30 K. Proper vibration decoupling of the cryocooler and its surrounding enables free-space micro-photoluminescence spectroscopy to identify and analyze different charge-carrier states within a single quantum dot. As an exemplary application in quantum optics, we perform a Hanbury-Brown and Twiss experiment demonstrating a strong suppression of multi-photon emission events with g((2))(0) < 0.04 from this Stirling-cooled single quantum emitter under continuous wave excitation. Comparative experiments performed on the same quantum dot in a liquid helium (LHe)-flow cryostat show almost identical values of g((2))(0) for both configurations at a given temperature. The results of this proof of principle experiment demonstrate that low-vibration Stirling cryocoolers that have so far been considered exotic to the field of nanophotonics are an attractive alternative to expensive closed-cycle cryostats or LHe-flow cryostats, which could pave the way for the development of high-quality table-top non-classical light sources.
Abstract In this work, we present a stand-alone and fiber-coupled quantum-light source. The plug-and-play device is based on an optically driven quantum dot delivering single photons via an optical fiber. The quantum dot is deterministically integrated in a monolithic microlens which is precisely coupled to the core of an optical fiber via active optical alignment and epoxide adhesive bonding. The rigidly coupled fiber-emitter assembly is integrated in a compact Stirling cryocooler with a base temperature of 35 K. We benchmark our practical quantum device via photon auto-correlation measurements revealing g(2)(0) = 0.07 ± 0.05 under continuous-wave excitation and we demonstrate triggered non-classical light at a repetition rate of 80 MHz. The long-term stability of our quantum light source is evaluated by endurance tests showing that the fiber-coupled quantum dot emission is stable within 4% over several successive cool-down/warm-up cycles. Additionally, we demonstrate non-classical photon emission for a user-intervention-free 100-hour test run and stable single-photon count rates up to 11.7 kHz with a standard deviation of 4%.
While nonclassical light sources are fundamental to quantum communication and computing, solid-state platforms like color centers and quantum dots require cryogenic temperatures to reach the performance levels necessary for practical applications. Over the past decade, low-temperature engineering has transitioned from manual handling of liquid cryogens to automated closed-cycle cryostats. This review details the principles behind modern cooling hardware ranging from flow cryostats to mechanical cryocoolers and dilution refrigerators, with a specific focus on the requirements of optical quantum devices. Aimed at the practicing scientist, this overview provides the technical insights and historical context needed to navigate the current cryogenic landscape and evaluate its role in the future of quantum technology deployment.
Single semiconductor quantum dots, which are considered as two-level systems in the artificial atom model, are promising structures for the realization of integrated devices such as single photon sources for quantum information applications. However, contrary to genuine atoms, they are condensed matter systems which suffer from the coupling to their solid environment, leading to a degradation of the coherence of the emitted photons. One possibility to avoid this coupling, thereby improving the coherence of the photons until the one imposed by the radiative limit T2 = 2T1, is to perform strictly resonant excitation of a quantum dot at low temperature. Using an experimental setup that spatially decouples the excitation and detection paths, we showed that a fine control of the electrostatic environment related to the nanostructures residual doping remains a major challenge to answer the widely encountered problem of the inhibition of the resonance fluorescence of a quantum dot. Meanwhile, thanks to quantum optics experiments and high resolution optical spectroscopy, we demonstrated that the resonant Rayleigh scattering regime where quantum dots emit single photons with the laser coherence time, paves the way to the development of "ultra-coherent" sources of single photons with high degrees of indistinguishability. In this regime where the laser tailors the coherence of the photons and where the radiative limit becomes a secondary requirement, two photons emitted successively by the same quantum dot are indistinguishable on time scales never obtained before for a solid nano-emitter (up to ten nanoseconds, comparing to the carriers lifetime and decoherence time of about a hundred of picoseconds).
Single-photon sources (SPS) are essential for secure quantum communication and quantum computing. Solid-state systems based on quantum dots (QDs) are particularly attractive for emitting pure, on-demand single photons, making them ideal candidates for flying qubits in quantum key distribution protocols. Integrating a SPS into photonic circuits is a key step toward scalable and "plug-and-play" quantum technologies. However, the SPS with the best performances (III-V QDs) operate only at cryogenic temperatures, a significant drawback for practical implementation. Alternatively, CdSe QDs (II-VI) are operational at 300 K and emit in the blue-green range, thus allowing for free-space long-distance communication in seawater and air.The thesis aims to develop an on-chip single-photon source that can operate at non-cryogenic temperatures. The SPS consists of a CdSe QD embedded within a ZnSe nanowire (NW) shell grown by molecular beam epitaxy on a patterned GaAs (111)B substrate. The NW geometry enhances light extraction by acting as a single-mode waveguide, while the conical ending of the shell improves emission control.We investigated the optical performance of the as-grown QD-NW emitter at room temperature, achieving a promising brightness of 0.17 photons per pulse and antibunching behavior with g(2)(0) < 0.3 within a reduced spectral window. However, the emission spectrum at 300 K features overlapping broad lines, leading to a trade-off between brightness and purity. At 6 K, we used a broadband filter to capture entirely the narrow exciton line and measured directly the photon count rate with an avalanche photodiode. In addition, we observed strong antibunching with a few percent purity through cathodoluminescence.Phonons impact the performance of the SPS at high temperatures, where broad lines overlap, and at cryogenic temperatures, where they reduce the photon indistinguishability. Understanding and controlling the influence of phonons has increased the need for high-accuracy temperature measurements at cryogenic temperatures. We present a calibration-free method to extract the local temperature from the emission spectrum, which we used to investigate the heating effects induced by non-resonant excitation. Additionally, we analysed the line-broadening mechanisms from cryogenic to room temperature. An extension of the Huang-Rhys model is developed to analytically describe the acoustic exciton-phonon interactions, accounting for multi-phonon processes. The model accurately fits emission spectra from 6 K to 300 K using parameters obtained from low-temperature data.The tapered nanowire shape is also an advantage for integration into a photonic device, enabling efficient evanescent coupling when the emitter is positioned next to a waveguide. The direct transfer using micromanipulators in a scanning electron microscope onto pre-fabricated waveguides is very challenging due to the tiny size of the waveguide at an emission wavelength of 550 nm. We developed a new approach, where the emitter is deposited within a large zone and then embedded within a resist, which serves as a mask during waveguide etching. This method significantly reduces the need for micro-manipulation and allows for promising prospects. We used finite-difference time-domain simulations to support the design and fabrication of the waveguides for optimal coupling.
Quantum light and in particular single photons have become essential resources for a growing number of quantum applications including quantum computing, quantum key distribution and quantum metrology. Solid-state atomlike systems such as semiconductor quantum dots and color defects in crystals have become the hallmark of highly pure single photon emitters in the past two decades. A particular interest has been developed in nanocrystal quantum dots (NQDs) and color centers in diamond as potential compact room-temperature emitters. There are however several challenges that inhibit the use of such sources in current technologies including low photon extraction efficiency, low emission rates and relatively low single photon purities. In this work we will review our efforts in overcoming these technical difficulties using several complementary methods including designing several nanoantenna devices that enhance the directionality and emission rate of the nanoemitter. In addition, we developed several temporal heralding techniques to overcome the hurdle of low single photon purity in NQDs in an effort to produce a highly pure, bright and efficient single photon source on-chip.
For photonic quantum technology applications, sources capable of emitting photons with indistinguishability close to unity are essential. Ideally, these sources should not require demanding cooling systems. Here, we present temperature-dependent two-photon-interference measurements on photons produced by the radiative decay of the negative trion in a low-noise GaAs quantum dot, which are in quantitative agreement with theoretical calculations accounting for carrier-phonon interactions and coupling to excited states. While at at the lowest explored temperatures the emission linewidth reaches values only 6(2) % above the Fourier limit and the indistinguishability I between subsequently emitted photons reaches 0.966(6), the latter drops to 0.05(4) at 55 K. We show that this loss can be explained with the coupling with energetically close excited trion states and suggest that the photon indistinguishability at elevated temperatures can be increased by employing Purcell enhancement of the emission rate or by increasing the energy separation of the excited states. Using cavity-enhanced emission, we experimentally verify the first route and demonstrate an improvement in photon indistinguishability from 0.314(25) to 0.80(3) at 32 K, which - to our knowledge - is the highest reported value at such temperature.