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Applied Physics Letters

Few-photon-level two-dimensional infrared imaging by coincidence frequency upconversion

Kun Huang, Xiaorong Gu, Haifeng Pan, E Wu, Heping Zeng

Published Apr 9, 2012• 45 citations
Publisher
DOI
10.1063/1.3703610

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Applied Physics Letters•Jun 17, 2013•43 citations
Single-photon frequency upconversion is an effective method of infrared single-photon detection and imaging by converting the long-wavelength photons to shorter wavelengths to match the detector’s spectral response. We realized few-photon level 2D infrared imaging with a coincidence frequency upconversion system in a bulk periodically poled lithium niobate crystal. Moreover, the infrared photons carrying orbital angular momentum were converted to the visible regime with high efficiency, while the orbital angular momentum of the photons was well conserved during the frequency upconversion process. The single-photon frequency upconversion method was also used for mid-infrared imaging at 3.39 µm with high efficiency and low noise.
Mid-infrared (MIR) imaging plays a pivotal role in chemical sensing, biomedicine, and material analysis, yet its further development is fundamentally constrained by limited room-temperature sensitivity and the lack of efficient multidimensional light-field control. In recent years, frequency upconversion imaging has emerged as a rapidly advancing approach that translates MIR signals to the visible or near-infrared domain, enabling high-sensitivity detection with mature, low-noise photonic platforms. More importantly, by engineering the pump field in nonlinear frequency conversion processes, a multidimensional imaging framework has been established, enabling indirect, all-optical encoding and retrieval of multiple degrees of freedom—including amplitude, phase, spectrum, time, and polarization—of MIR light fields. This paradigm shifts complex light-field manipulation from the MIR to technologically mature short-wavelength regimes, overcoming intrinsic limitations of conventional approaches. In this review, we systematically summarize the principles, architectures, and representative methodologies of MIR upconversion multidimensional imaging, and outline future directions toward high-sensitivity, high-dimensional, and integrated imaging systems, with implications extending to broader photonic and information processing domains.
We demonstrated few-photon-level mid-infrared imaging at 3.39 μm by efficient frequency up-conversion. The quantum frequency up-conversion efficiency of mid-infrared photons was high to 32.9%, while mid-infrared images were up-converted with the quantum efficiency of 12.5%. The mid-infrared imaging sensitivity was improved by counting the frequency up-conversion photons temporally confined within the time-window of the pump pulse. The frequency up-conversion system induced a background noise of 1.1 × 103 counts per second.