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Physical review. B, Condensed matter

BCS to Bose crossover: Broken-symmetry state

Jan R. Engelbrecht, Mohit Randeria, C.A.R. Sáde Melo

Published Jun 1, 1997• 400 citations
Publisher

Abstract

A functional integral formulation, used previously to calculate ${\mathrm{T}}_{\mathrm{c}}$ and describe normal state properties of the BCS-Bose crossover, is extended to T${\mathrm{T}}_{\mathrm{c}}$. The saddle point approximation is shown to be qualitatively correct for T\ensuremath{\ll}${\mathrm{T}}_{\mathrm{c}}$ for all couplings, in contrast to the situation above ${\mathrm{T}}_{\mathrm{c}}$. Several features of the crossover are described. The difference between the T=0 ``pair size'' and the (prefactor of the T dependent) Ginzburg-Landau coherence length is pointed out: the two quantities are the same only in the BCS limit. The evolution of the collective modes from the BCS to the Bose regime is discussed together with the mixing of the amplitude and phase in the absence of a particle-hole symmetry.

DOI
10.1103/physrevb.55.15153

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A functional integral formulation, used previously to calculate Tc{\mathrm{T}}_{\mathrm{c}}Tc​ and describe normal state properties of the BCS-Bose crossover, is extended to TTc{\mathrm{T}}_{\mathrm{c}}Tc​. The saddle point approximation is shown to be qualitatively correct for T\ensuremath{\ll}Tc{\mathrm{T}}_{\mathrm{c}}Tc​ for all couplings, in contrast to the situation above Tc{\mathrm{T}}_{\mathrm{c}}Tc​. Several features of the crossover are described. The difference between the T=0 ``pair size'' and the (prefactor of the T dependent) Ginzburg-Landau coherence length is pointed out: the two quantities are the same only in the BCS limit. The evolution of the collective modes from the BCS to the Bose regime is discussed together with the mixing of the amplitude and phase in the absence of a particle-hole symmetry.
We use a functional integral formulation to study the crossover from cooperative Cooper pairing to the formation and condensation of tightly bound pairs in a 3D continuum model of fermions with attractive interactions. The inadequacy of a saddle point approximation with increasing coupling is pointed out, and the importance of temporal (quantum) fluctuations for normal state properties at intermediate and strong coupling is emphasized. In addition to recovering the Nozieres-Schmitt-Pink interpolation scheme for T{sub c}, and the Leggett variational results for T = 0, we also present results for evolution of the time-dependent Ginzburg-Landau equation and collective mode spectrum as a function of the coupling.
We use a functional integral formulation to study the finite temperature crossover from cooperative Cooper pairing to independent bound state formation and condensation. We show the inadequacy of mean field results for normal state properties obtained at the saddle point level as the coupling increases. The importance of quantum (temporal) fluctuations is pointed out and an interpolation scheme for Tc{\mathit{T}}_{\mathit{c}}Tc​ is derived from this point of view. The time-dependent Ginzburg-Landau (TDGL) equation near Tc{\mathit{T}}_{\mathit{c}}Tc​ is shown to describe a damped mode in the BCS limit, and a propagating one in the Bose limit. A singular point is identified at intermediate coupling where a simple TDGL description fails.
The problem of the evolution from BCS theory with cooperative Cooper pairing to the formation and condensation of composite bosons has attracted considerable attention for the past several decades. It has gained renewed impetus in the mid-eighties with the discovery of the high-Tc superconductors, which have a coherence length comparable to the interparticle spacing. More recently, this subject has spurred a great deal of research activity in connection with experiments involving dilute atomic gases of fermionic atoms. The initial objective of this work will be to use functional integral techniques to analyze the low-temperature BCS-to-BEC evolution of d-wave superconductors within the saddle point (mean field) approximation for a continuum model. Then, the same mathematical formalism will be applied to the problem of the BCS-to-BEC evolution of fully spin-polarized p-wave Fermi gases in two dimensions. We find that a quantum phase transition occurs for both systems as they are driven from the BCS-like regime of weakly interacting fermionic pairs to the opposite BEC-like regime of strongly interacting bosonic molecules. This is in contrast to the smooth crossover predicted and observed in systems that exhibit s-wave pairing symmetry. We calculate several spectroscopic and thermodynamic properties that signal the occurrence of this phase transition, and suggest some possible experimental realizations. Finally, fluctuations about the saddle point solution are included in the calculations, and the effects of such correction are analyzed in the low (T~0) and high (T~Tc) temperature limits. We conclude that, at high temperatures, the bosonic degrees of freedom that arise from two-particle bound states become essential to describe the strong coupling limit,\nas the saddle point approximation alone becomes unreliable.
In this paper we study the BCS Bose-Einstein condensation (BEC) crossover scenario within the superconducting state, using a T-matrix approach which yields the ground state proposed by Leggett. Here we extend this ground state analysis to finite temperatures T and interpret the resulting physics. We find two types of bosoniclike excitations of the system: long lived, incoherent pair excitations and collective modes of the superconducting order parameter, which have different dynamics. Using a gauge invariant formalism, this paper addresses their contrasting behavior as a function of T and superconducting coupling constant g. At a more physical level, our paper emphasizes how, at finite T, BCS-BEC approaches introduce an important parameter ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2}={\ensuremath{\Delta}}^{2}\ensuremath{-}{\ensuremath{\Delta}}_{\mathrm{sc}}^{2}$ into the description of superconductivity. This parameter is governed by the pair excitations and is associated with particle-hole asymmetry effects that are significant for sufficiently large g. In the fermionic regime, ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2}$ represents the difference between the square of the excitation gap ${\ensuremath{\Delta}}^{2}$ and that of the superconducting order parameter ${\ensuremath{\Delta}}_{\mathrm{sc}}^{2}.$ The parameter ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2},$ which is necessarily zero in the BCS (mean field) limit increases monotonically with the strength of the attractive interaction g. It follows that there is a significant physical distinction between this BCS-BEC crossover approach (in which g is the essential variable which determines ${\ensuremath{\Delta}}_{\mathrm{pg}})$ and the widely discussed phase fluctuation scenario in which the plasma frequency is the tuning parameter. Finally, we emphasize that in the strong coupling limit, there are important differences between the composite bosons that arise in crossover theories and the usual bosons of the (interacting) Bose liquid. Because of constraints imposed on the fermionic excitation gap and chemical potential, in crossover theories, the fermionic degrees of freedom can never be fully removed from consideration.
The BCS-BEC crossover is studied in a systematic way in the broken-symmetry phase between zero temperature\nand the critical temperature. This study bridges two regimes where quantum and thermal fluctuations\nare, respectively, important. The theory is implemented on physical grounds, by adopting a fermionic selfenergy\nin the broken-symmetry phase that represents fermions coupled to superconducting fluctuations in weak\ncoupling and to bosons described by the Bogoliubov theory in strong coupling. This extension of the theory\nbeyond mean field proves important at finite temperature, to connect with the results in the normal phase. The\norder parameter, the chemical potential, and the single-particle spectral function are calculated numerically for\na wide range of coupling and temperature. This enables us to assess the quantitative importance of superconducting\nfluctuations in the broken-symmetry phase over the whole BCS-BEC crossover. Our results are relevant\nto the possible realizations of this crossover with high-temperature cuprate superconductors and with\nultracold fermionic atoms in a trap.
We present a self-consistent theory for the thermodynamics of the BCS-BEC crossover in the normal and superfluid phase which is both conserving and gapless. It is based on the variational many-body formalism developed by Luttinger and Ward and by DeDominicis and Martin. Truncating the exact functional for the entropy to that obtained within a ladder approximation, the resulting self-consistent integral equations for the normal and anomalous Green functions are solved numerically for arbitrary coupling. The critical temperature, the equation of state, and the entropy are determined as a function of the dimensionless parameter 1∕kFa1∕{k}_{F}a1∕kF​a, which controls the crossover from the BCS regime of extended pairs to the BEC regime of tightly bound molecules. The tightly bound pairs turn out to be described by a Popov-type approximation for a dilute, repulsive Bose gas. Even though our approximation does not capture the critical behavior near the continuous superfluid transition, our results provide a consistent picture for the complete crossover thermodynamics which compares well with recent numerical and field-theoretic approaches at the unitarity point.