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arXiv:cond-mat/9906180 · Physical review. B, Condensed matter

Pair excitations, collective modes, and gauge invariance in the BCS–Bose-Einstein crossover scenario

Ioan Kosztin, Qijin Chen, Ying-Jer Kao, Kathryn Levin

Published May 1, 2000• 74 citations
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Abstract

In this paper we study the BCS Bose-Einstein condensation (BEC) crossover scenario within the superconducting state, using a T-matrix approach which yields the ground state proposed by Leggett. Here we extend this ground state analysis to finite temperatures T and interpret the resulting physics. We find two types of bosoniclike excitations of the system: long lived, incoherent pair excitations and collective modes of the superconducting order parameter, which have different dynamics. Using a gauge invariant formalism, this paper addresses their contrasting behavior as a function of T and superconducting coupling constant g. At a more physical level, our paper emphasizes how, at finite T, BCS-BEC approaches introduce an important parameter ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2}={\ensuremath{\Delta}}^{2}\ensuremath{-}{\ensuremath{\Delta}}_{\mathrm{sc}}^{2}$ into the description of superconductivity. This parameter is governed by the pair excitations and is associated with particle-hole asymmetry effects that are significant for sufficiently large g. In the fermionic regime, ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2}$ represents the difference between the square of the excitation gap ${\ensuremath{\Delta}}^{2}$ and that of the superconducting order parameter ${\ensuremath{\Delta}}_{\mathrm{sc}}^{2}.$ The parameter ${\ensuremath{\Delta}}_{\mathrm{pg}}^{2},$ which is necessarily zero in the BCS (mean field) limit increases monotonically with the strength of the attractive interaction g. It follows that there is a significant physical distinction between this BCS-BEC crossover approach (in which g is the essential variable which determines ${\ensuremath{\Delta}}_{\mathrm{pg}})$ and the widely discussed phase fluctuation scenario in which the plasma frequency is the tuning parameter. Finally, we emphasize that in the strong coupling limit, there are important differences between the composite bosons that arise in crossover theories and the usual bosons of the (interacting) Bose liquid. Because of constraints imposed on the fermionic excitation gap and chemical potential, in crossover theories, the fermionic degrees of freedom can never be fully removed from consideration.

DOI
10.1103/physrevb.61.11662

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In this paper we study the BCS Bose-Einstein condensation (BEC) crossover scenario within the superconducting state, using a T-matrix approach which yields the ground state proposed by Leggett. Here we extend this ground state analysis to finite temperatures T and interpret the resulting physics. We find two types of bosoniclike excitations of the system: long lived, incoherent pair excitations and collective modes of the superconducting order parameter, which have different dynamics. Using a gauge invariant formalism, this paper addresses their contrasting behavior as a function of T and superconducting coupling constant g. At a more physical level, our paper emphasizes how, at finite T, BCS-BEC approaches introduce an important parameter \ensuremathΔpg2=\ensuremathΔ2\ensuremath−\ensuremathΔsc2{\ensuremath{\Delta}}_{\mathrm{pg}}^{2}={\ensuremath{\Delta}}^{2}\ensuremath{-}{\ensuremath{\Delta}}_{\mathrm{sc}}^{2}\ensuremathΔpg2​=\ensuremathΔ2\ensuremath−\ensuremathΔsc2​ into the description of superconductivity. This parameter is governed by the pair excitations and is associated with particle-hole asymmetry effects that are significant for sufficiently large g. In the fermionic regime, \ensuremathΔpg2{\ensuremath{\Delta}}_{\mathrm{pg}}^{2}\ensuremathΔpg2​ represents the difference between the square of the excitation gap \ensuremathΔ2{\ensuremath{\Delta}}^{2}\ensuremathΔ2 and that of the superconducting order parameter \ensuremathΔsc2.{\ensuremath{\Delta}}_{\mathrm{sc}}^{2}.\ensuremathΔsc2​. The parameter \ensuremathΔpg2,{\ensuremath{\Delta}}_{\mathrm{pg}}^{2},\ensuremathΔpg2​, which is necessarily zero in the BCS (mean field) limit increases monotonically with the strength of the attractive interaction g. It follows that there is a significant physical distinction between this BCS-BEC crossover approach (in which g is the essential variable which determines \ensuremathΔpg){\ensuremath{\Delta}}_{\mathrm{pg}})\ensuremathΔpg​) and the widely discussed phase fluctuation scenario in which the plasma frequency is the tuning parameter. Finally, we emphasize that in the strong coupling limit, there are important differences between the composite bosons that arise in crossover theories and the usual bosons of the (interacting) Bose liquid. Because of constraints imposed on the fermionic excitation gap and chemical potential, in crossover theories, the fermionic degrees of freedom can never be fully removed from consideration.
The (mean field based) BCS theory is considered one of the most successful theories in condensed matter physics. It is justified in ordinary metal superconductors the coherence length ξξξ is large, with two important features: the order parameter (OP) and excitation gap (EG) are identical, and the pair formation and their Bose condensation take place at the same temperature Tc. It fails to explain the underdoped cuprate superconductivity: EG is finite at Tc and thus distinct from OP. Since these superconductors belong to a large class of small ξξξ materials, this failure has the potential for widespread impact. Here we have extended BCS theory in a natural way to short ξξξ superconductors, based on a BCS--BEC crossover scenario, and arrived at a simple physical picture in which incoherent, finite momentum pairs become progressively more important as the pairing interaction becomes stronger, leading to the distinction between EG and OP. The superconductivity from the fermionic perspective and BEC from the bosonic perspective are just two sides of the same coin. Our theory is capable of making verifiable quantitative predictions. We obtain a cuprate phase diagram (with one free parameter) , in (semi-)quantitative agreement with experiment. The mutually compensating contributions from fermionic quasiparticles and bosonic pair excitations provides a natural explanation for the quasi-universal behavior of the in-plane superfluid density versus T. Our bosonic pair excitations also provide an intrinsic mechanism for the long mysterious linear T terms in the specific heat. Incoherent pair contributions lead to new low T power laws, consistent with existing experiments. Finally, we demonstrated that the onset of superconducting long range order leads to sharp features in the specific heat at Tc, consistent with experiment.
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We consider a lattice version of the ``negative-U′′U''U′′ Hubbard model in three dimensions, to study the crossover from a superconducting phase transition (dominated by phase fluctuation) to a regime where the amplitude of the superconducting order parameter controls the critical temperature. Starting from a fermionic Hamiltonian, we give a microscopic derivation of the effective action in terms of the relevant physical fields: the modulus and phase of the superconducting order parameter. Furthermore, by employing to the resulting coarse--grained quantum XY\mathrm{XY}XY model the phase fluctuation algebra between number and phase operators (given by the Euclidean group E2),{E}_{2}),E2​), we map the ``phase-only'' action onto a solvable quantum spherical model. We establish the self--consistent theory (involving both fermionic and bosonic degrees of freedom), and calculate the superconducting phase coherence transition temperature Tc{T}_{c}Tc​ as a function of the coupling strength ∣U∣,|U|,∣U∣, exhibiting a maximum where the behavior crosses over from BCS to Bose-Einstein (BE) condensation. We examine a pseudogap in the normal state which emerges naturally as a precursor of superconductivity at the second characteristic temperature Tg{T}_{g}Tg​ due to a state with bound pairs but without long--range phase coherence. Furthermore, we demonstrate that the reduced gaps of the model $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{g}\ensuremath{\sim}4$ is almost independent on the pairing strength ∣U∣/t,|U|/t,∣U∣/t, whereas $2{\ensuremath{\Delta}}_{0}{/k}_{B}{T}_{c}$ increases with increasing ∣U∣|U|∣U∣---in striking analogy with the phenomenology of the high--temperature cuprate superconductors when interpreted in terms of the BCS-BC crossover scenario.
The BCS-BEC crossover is studied in a systematic way in the broken-symmetry phase between zero temperature\nand the critical temperature. This study bridges two regimes where quantum and thermal fluctuations\nare, respectively, important. The theory is implemented on physical grounds, by adopting a fermionic selfenergy\nin the broken-symmetry phase that represents fermions coupled to superconducting fluctuations in weak\ncoupling and to bosons described by the Bogoliubov theory in strong coupling. This extension of the theory\nbeyond mean field proves important at finite temperature, to connect with the results in the normal phase. The\norder parameter, the chemical potential, and the single-particle spectral function are calculated numerically for\na wide range of coupling and temperature. This enables us to assess the quantitative importance of superconducting\nfluctuations in the broken-symmetry phase over the whole BCS-BEC crossover. Our results are relevant\nto the possible realizations of this crossover with high-temperature cuprate superconductors and with\nultracold fermionic atoms in a trap.
We investigate here the BCS-BEC crossover in relativistic systems using a variational construct for the ground state and the minimization of the thermodynamic potential. This is first studied in a four-fermion point interaction model and with a BCS type ansatz for the ground state with fermion pairs. It is shown that the antiparticle degrees of freedom play an important role in the BCS-BEC crossover physics, even when the ratio of Fermi momentum to the mass of the fermion is small. We also consider the phase structure for the case of fermion pairing with imbalanced populations. Within the ansatz, thermodynamically stable gapless modes for both fermions and antifermions are seen for strong coupling in the Bose-Einstein condensation (BEC) regime. We further investigate the effect of fluctuations of the condensate field by treating it as a dynamical field and generalize the BCS ansatz to include quanta of the condensate field also in a boson-fermion model with quartic self-interaction of the condensate field. It is seen that the critical temperature decreases with inclusion of fluctuations.
In this paper we present a very general theoretical framework for addressing fermionic superfluids over the entire range of BCS to Bose Einstein condensation (BEC) crossover in the presence of population imbalance or spin polarization. Our emphasis is on providing a theory which reduces to the standard zero temperature mean-field theories in the literature, but necessarily includes pairing fluctuation effects at nonzero temperature within a consistent framework. Physically, these effects are associated with the presence of preformed pairs (or a fermionic pseudogap) in the normal phase, and pair excitations of the condensate, in the superfluid phase. We show how this finite TTT theory of fermionic pair condensates bears many similarities to the condensation of point bosons. In the process we examine three different types of condensate: the usual breached pair or Sarma phase and both the one- and two-plane-wave Larkin-Ovchinnikov-Fulde-Ferrell (LOFF) states. The last of these has been discussed in the literature albeit only within a Landau-Ginzburg formalism, generally valid near Tc{T}_{c}Tc​. Here we show how to arrive at the two-plane-wave LOFF state in the ground state as well as at general temperature TTT.