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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Bright magneto-optical resonance sign reversal in Cs vapour confined in an extremely thin cell

Aigars Atvars, Marcis P. Auzinsh, Kristaps Bluss, C. Andreeva, S. Cartaleva, L. Petrov, David G. Sarkisyan, T. Varzhapetyan

Published Jun 1, 2007• 0 citations
Publisher

Abstract

An extremely thin cell (ETC) was used to analyse ground state effects of Cs atoms excited by laser light and placed in a magnetic field that was scanned around zero. The advantage of using the ETC is the possibility to separate the hf transitions, which are overlapped in ordinary cells, as a result of the spatial anisotropy of the atom-light interaction. Cs atoms were irradiated by circularly/linearly polarized light at lambda~852 nm, and the dependence of absorption on the external magnetic field was measured.

DOI
10.1109/cleoe-iqec.2007.4386933

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arXiv:0909.5081•Physical Review A•Mar 17, 2010•10 citations
An extremely thin cell (ETC) was used to analyse ground state effects of Cs atoms excited by laser light and placed in a magnetic field that was scanned around zero. The advantage of using the ETC is the possibility to separate the hf transitions, which are overlapped in ordinary cells, as a result of the spatial anisotropy of the atom-light interaction. Cs atoms were irradiated by circularly/linearly polarized light at lambda~852 nm, and the dependence of absorption on the external magnetic field was measured.
Experimental and theoretical studies are presented related to the ground-state magneto-optical resonance observed in cesium vapor confined in an extremely thin cell (ETC), with thickness equal to the wavelength of the irradiating light. It is shown that utilization of the ETC allows one to examine the formation of a magneto-optical resonance on the individual hyperfine transitions, thus distinguishing processes resulting in dark (reduced absorption) or bright (enhanced absorption) resonance formation. We report experimental evidence of bright magneto-optical resonance sign reversal in Cs atoms confined in an ETC. A theoretical model is proposed based on the optical Bloch equations that involves the elastic interaction processes of atoms in the ETC with its walls, resulting in depolarization of the Cs excited state, which is polarized by the exciting radiation. This depolarization leads to the sign reversal of the bright resonance. Using the proposed model, the magneto-optical resonance amplitude and width as a function of laser power are calculated and compared with the experimental ones. The numerical results are in good agreement with those of experiment.
Recently unique extremely thin cells (ETC) containing atomic vapour of alkali metals with the column thickness L of an order and much less than optical light wavelength λ have been developed. It has been demonstrated that these ETC are a very promising tool for a fundamental study of atom-light, atom-atom, atom-surface and atom-external magnetic field interactions. Particularly, a dramatically different behaviour of resonant absorption, fluorescence and resonant magneto-optical processes compared to that obtained with the help of cm-long ordinary cells has been demonstrated. Possible applications based on ETC are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references. For the study of buffer gas influence, a multi-region cell (MRC) has been developed. MRC consists of an ETC cell having a wedged thickness of the gap between the windows that allows one to form atomic vapour column thickness in the range of 0.1 ÷ 4 μm. The ETC is connected through a sapphire tube with a 1cm-long sapphire tube having sapphire windows. The 1cm-long cell has a sapphire side-arm containing Rb metal. MRC's are filled with 6 Torr and 20 Torr Neon gas, thus there is Rb vapour and buffer gas inside the MRC. The construction of the MRC allows one to compare absorption and fluorescence processes simultaneously in the case of the ETC use as well as in the case of 1cm-long ordinary cell use. The comparison of the resonant absorption and fluorescence in the extremely thin cell (ETC) filled with pure Rb with another one filled with Rb and Neon gas with the pressures of 6 Torr and 20 Torr is provided. The effect of the collapse and revival of Dicke-type narrowing is still observable for the thicknesses L = λ/2, and L = λ, with λ being the resonant laser wavelength 794 nm (D1 line of Rb), i.e. the spectra of the resonant absorption and fluorescence demonstrate strong sub-Doppler narrowing for the thickness L = λ/2 and broadening for the thickness L = λ. It is important to note that in an ordinary Rb cell with the thickness L in the range of 1mm - 10 cm filled with buffer gas, with the pressure higher than 1 Torr, in the well-known Saturation Absorption scheme, any sub-Doppler features are absent. For L = λ the so called velocity selective optical pumping/saturating resonance (VSOP) located at the atomic transition is still observable when Ne pressure is 6 Torr, while the linewidth is increased by 4 times in comparison with that obtained in a pure Rb ETC. It is also demonstrated that the use of the fluorescence spectra at L = λ/2 allows one to use ETC for the buffer gas pressure measurements. Comparison with the theory will be presented.
The nonlinear absorption and fluorescence spectra of 133 Cs vapours confined to the extremely thin cell are computed in the framework of perturbation theory regarding to the intensity of the laser light illumination. The amplitude as well as the sign of the longitudinal alignment of the ground state is shown to be defined by the spontaneous decay of the upper level. The sign and the magnitude of the nonlinear absorption resonance on the closed optical transition are shown to be defined by this process as well.
Summary form only given. We have studied the absorption and fluorescence of the D/sub 2/ line [6S/sub 1/2/(F=3,4)-6P/sub 3/2/(F=2,3,4.5)] in dilute Cs atomic vapour for 3 vapour cells: an extremely thin cell with a column length of 8 /spl mu/m, a 16.5 mm-long cell with pure Cs vapour, and a 10.4 mm-long Cs cell containing 40 Torr of Ne. A laser diode with a 20 MHz-linewidth and the maximum intensity of 40 mW/cm/sup 2/ was used. In order to have a comparable peak absorption (for the case of low laser intensity), the extremely thin cell was heated to /spl sim/100/spl deg/C. The effective absorption cross-sections of these cells versus laser intensity are shown. It is important to note that the same behaviour was observed for the resonance fluorescence. The effect of optical pumping of Zeeman sublevels, leads to a dramatically different behaviour of absorption for the /spl nu//sub 3/ and the /spl nu//sub 4/ transitions at a laser intensity /spl ges/0.1 mW/cm/sup 3/ and the absorption of /spl nu//sub 3/ is very sensitive to the presence of a weak external magnetic field. Meanwhile, there is no hint for this effect both for the extremely thin and the buffer gas-filled cells.
We have measured magneto-optical signals obtained by exciting the D1{D}_{1}D1​ line of cesium atoms confined to an extremely thin cell (ETC), whose walls are separated by less than $1\ensuremath{\mu}\text{m}$, and developed an improved theoretical model to describe these signals with experimental precision. The theoretical model was based on the optical Bloch equations and included all neighboring hyperfine transitions, the mixing of the magnetic sublevels in an external magnetic field, and the Doppler effect, as in previous studies. However, in order to model the extreme conditions in the ETC more realistically, the model was extended to include a unified treatment of transit relaxation and wall collisions with relaxation rates that were obtained directly from the thermal velocities of the atoms and the length scales involved. Furthermore, the interactions of the atoms with different regions of the laser beam were modeled separately to account for the varying laser beam intensity over the beam profile as well as saturation effects that become important near the center of the beam at the relatively high laser intensities used during the experiments in order to obtain measurable signals. The model described the experimentally measured signals for laser intensities for magnetic fields up to 55 G and laser intensities up to 1W/cm21{\text{W/cm}}^{2}1W/cm2 with excellent agreement.
Nonlinear magneto-optical resonances have been measured in an extremely thin cell (ETC) for the D1{D}_{1}D1​ transition of rubidium in an atomic vapor of natural isotopic composition. All hyperfine transitions of both isotopes have been studied for a wide range of laser power densities, laser detunings, and ETC wall separations. Dark resonances in the laser induced fluorescence (LIF) were observed as expected when the ground-state total angular momentum Fg{F}_{g}Fg​ was greater than or equal to the excited-state total angular momentum Fe{F}_{e}Fe​. Unlike the case of ordinary cells, the width and contrast of dark resonances formed in the ETC dramatically depended on the detuning of the laser from the exact atomic transition. A theoretical model based on the optical Bloch equations was applied to calculate the shapes of the resonance curves. The model, which had been developed previously for ordinary vapor cells, averaged over the contributions from different atomic velocity groups, considered all neighboring hyperfine transitions, took into account the splitting and mixing of magnetic sublevels in an external magnetic field, and included a detailed treatment of the coherence properties of the laser radiation. Such a theoretical approach had successfully described nonlinear magneto-optical resonances in ordinary vapor cells. However, to describe the resonances in the ETC, key parameters such as the ground-state relaxation rate, excited-state relaxation rate, Doppler width, and Rabi frequency had to be modified significantly in accordance with the ETC's unique features. The level of agreement between the measured and calculated resonance curves achieved for the ETC was similar to what could be accomplished for ordinary cells. However, in the case of the ETC, it was necessary to fine-tune parameters such as the background and the Rabi frequency for different transitions, whereas for the ordinary cells, these parameters were identical for all transitions.