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Conference on Lasers and Electro-Optics

Cs vapour cells: absorption and fluorescence may vary by several orders of magnitude

David G. Sarkisyan, Yu. P. Malakyan, A. Papoyan, G. Bison, Antoine Weis

Published Aug 29, 2005• 1 citation
Publisher

Abstract

Summary form only given. We have studied the absorption and fluorescence of the D/sub 2/ line [6S/sub 1/2/(F=3,4)-6P/sub 3/2/(F=2,3,4.5)] in dilute Cs atomic vapour for 3 vapour cells: an extremely thin cell with a column length of 8 /spl mu/m, a 16.5 mm-long cell with pure Cs vapour, and a 10.4 mm-long Cs cell containing 40 Torr of Ne. A laser diode with a 20 MHz-linewidth and the maximum intensity of 40 mW/cm/sup 2/ was used. In order to have a comparable peak absorption (for the case of low laser intensity), the extremely thin cell was heated to /spl sim/100/spl deg/C. The effective absorption cross-sections of these cells versus laser intensity are shown. It is important to note that the same behaviour was observed for the resonance fluorescence. The effect of optical pumping of Zeeman sublevels, leads to a dramatically different behaviour of absorption for the /spl nu//sub 3/ and the /spl nu//sub 4/ transitions at a laser intensity /spl ges/0.1 mW/cm/sup 3/ and the absorption of /spl nu//sub 3/ is very sensitive to the presence of a weak external magnetic field. Meanwhile, there is no hint for this effect both for the extremely thin and the buffer gas-filled cells.

DOI
10.1109/iqec.2000.907907

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The absorption and fluorescence spectra of a submicron Cs vapour layer under resonant excitation on the D2 line are measured. Sub-Doppler features centered at the resonance frequency of the hyperfine (hf) transitions have been observed. Substantial changes in the amplitude and width of the sub-Doppler resonances for individual hf transitions were recorded in dependence on the intensity of the incident laser radiation. In the fluorescence spectra narrow dips due to the effects of saturation have been observed. We also report about the observation of coherence resonances in Hanle configuration obtained at cell thickness of the order of the wavelength of the laser light.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Apr 22, 2005•6 citations
Summary form only given. We have studied the absorption and fluorescence of the D/sub 2/ line [6S/sub 1/2/(F=3,4)-6P/sub 3/2/(F=2,3,4.5)] in dilute Cs atomic vapour for 3 vapour cells: an extremely thin cell with a column length of 8 /spl mu/m, a 16.5 mm-long cell with pure Cs vapour, and a 10.4 mm-long Cs cell containing 40 Torr of Ne. A laser diode with a 20 MHz-linewidth and the maximum intensity of 40 mW/cm/sup 2/ was used. In order to have a comparable peak absorption (for the case of low laser intensity), the extremely thin cell was heated to /spl sim/100/spl deg/C. The effective absorption cross-sections of these cells versus laser intensity are shown. It is important to note that the same behaviour was observed for the resonance fluorescence. The effect of optical pumping of Zeeman sublevels, leads to a dramatically different behaviour of absorption for the /spl nu//sub 3/ and the /spl nu//sub 4/ transitions at a laser intensity /spl ges/0.1 mW/cm/sup 3/ and the absorption of /spl nu//sub 3/ is very sensitive to the presence of a weak external magnetic field. Meanwhile, there is no hint for this effect both for the extremely thin and the buffer gas-filled cells.
Recently unique extremely thin cells (ETC) containing atomic vapour of alkali metals with the column thickness L of an order and much less than optical light wavelength λ have been developed. It has been demonstrated that these ETC are a very promising tool for a fundamental study of atom-light, atom-atom, atom-surface and atom-external magnetic field interactions. Particularly, a dramatically different behaviour of resonant absorption, fluorescence and resonant magneto-optical processes compared to that obtained with the help of cm-long ordinary cells has been demonstrated. Possible applications based on ETC are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references. For the study of buffer gas influence, a multi-region cell (MRC) has been developed. MRC consists of an ETC cell having a wedged thickness of the gap between the windows that allows one to form atomic vapour column thickness in the range of 0.1 ÷ 4 μm. The ETC is connected through a sapphire tube with a 1cm-long sapphire tube having sapphire windows. The 1cm-long cell has a sapphire side-arm containing Rb metal. MRC's are filled with 6 Torr and 20 Torr Neon gas, thus there is Rb vapour and buffer gas inside the MRC. The construction of the MRC allows one to compare absorption and fluorescence processes simultaneously in the case of the ETC use as well as in the case of 1cm-long ordinary cell use. The comparison of the resonant absorption and fluorescence in the extremely thin cell (ETC) filled with pure Rb with another one filled with Rb and Neon gas with the pressures of 6 Torr and 20 Torr is provided. The effect of the collapse and revival of Dicke-type narrowing is still observable for the thicknesses L = λ/2, and L = λ, with λ being the resonant laser wavelength 794 nm (D1 line of Rb), i.e. the spectra of the resonant absorption and fluorescence demonstrate strong sub-Doppler narrowing for the thickness L = λ/2 and broadening for the thickness L = λ. It is important to note that in an ordinary Rb cell with the thickness L in the range of 1mm - 10 cm filled with buffer gas, with the pressure higher than 1 Torr, in the well-known Saturation Absorption scheme, any sub-Doppler features are absent. For L = λ the so called velocity selective optical pumping/saturating resonance (VSOP) located at the atomic transition is still observable when Ne pressure is 6 Torr, while the linewidth is increased by 4 times in comparison with that obtained in a pure Rb ETC. It is also demonstrated that the use of the fluorescence spectra at L = λ/2 allows one to use ETC for the buffer gas pressure measurements. Comparison with the theory will be presented.
A new nano-cell with smoothly varying longitudinal thickness of the atomic vapour layer L in the range of 350 - 5100 nm allowing to study the resonant absorption of D1 and D2 lines of Cs atoms for thicknesses changing from L = Lambda/2 to L = 6 Lambda with the step of Lambda/2 (Lambda = 852 nm or 894 nm are the resonant laser wavelengths) and for different intensities is developed. It is revealed that for low laser intensities there is narrowing of the resonant absorption spectrum for the thicknesses L = (2n + 1)Lambda/2 (where n is an integer) up to L = 7Lambda /2 and broadening of the spectrum for L = n Lambda. For relatively high laser intensity (>1 mW/cm2), velocity selective optical pumping/saturated resonances of a reduced absorption (with the line-width close to the natural one), and centred on the hyperfine transitions occur when L = n Lambda. The possible application of these resonance peaks is given. The developed theoretical model describes well the experiment.
Comparison of the absorption and fluorescence in the nanocell (or so called extremely thin cell) filled with pure Rb with another one filled with Rb and Neon gas is provided. The effect of the collapse and revival of Dicke-type narrowing is still observable for thickness L=lambda/2, and lambda, where lambda , is a resonant laser wavelength either 780 nm, or 795 nm (for Rb, D2 or D1 line). For L=  so called velocity selective optical pumping (VSOP) resonance located at the atomic transition is still observable, while the linewidth is increased by 4 times in comparison with that obtained in the pure Rb nanocell. Comparison with the theory is presented. Electromagnetically Induced Transparency effect detected in the nanocell filled with Rb and Neon gas is presented. The EIT resonance linewidth is of 12 MHz when L~ 1 µm, while for the nanocell filled with pure Rb linewidth is ~9 MHz.
Comparison of the resonant absorption and fluorescence in the extremely thin cell (ETC) filled with pure Rb with another one filled with Rb and Neon gas with the pressures 6 Torr and 20 Torr is provided. The effect of the collapse and revival of Dicke-type narrowing is still observable for the thickness L=λ/2, and L=λ, where λ is a resonant laser wavelength 794 nm (D1 line of the Rb), i.e. the spectra of the resonant absorption and fluorescence demonstrate the sub-Doppler narrowing for the thickness L=λ/2 and broadening for the thickness L=λ. It is important to note, that in an ordinary Rb cell with the thickness L in the range of 1mm- 10 cm filled with buffer gas, with a pressure higher than 1 Torr in the Saturation Absorption scheme, any sub-Doppler features are absent. For L= λ the so called velocity selective optical pumping (VSOP) resonance located at the atomic transition is still observable when Ne pressure is 6 Torr , while the linewidth is increased by 4 times in comparison with that obtained in the pure Rb ETC. This VSOP resonance is wash out when Ne pressure is 20 Torr. It is demonstrated that use of the fluorescence spectra at L=λ/2 allows one to use the ETC for the buffer gas pressure measurement. Comparison with the theory is presented.
Absorption and fluorescence in Rb sub-micron cell on D2 line have been studied when the thickness L varies in the range of 0.5 λ - 3.5 λ, and the laser intensity is 0.1 - 1 W/cm2 (λ = 780 nm, λL ~ 5 MHz). When L = (2n +1) λ/2 (n-integer) and I ~ 0.1 W/cm2, revival of peaks of Dicke-type coherent narrowing effect with some modification of the spectra (as compared with low intensity regime) are still observable. The experimental results obtained at I ~ 1 W/cm2 for L = λ/2 show that there are no "dips" of a reduced absorption in the spectra, though there is a strong spectral broadening of the absorption (and fluorescence), as well as a reduction of the absorption (in contrast, I ~ 1 mW/cm2 is sufficient to create the dips when L = λ). Probably, this is caused by a strong Dicke narrowing regime when L = λ/2. Several additional differences of fluorescence and absorption spectra behaviour at high intensities are revealed.
The absorption and fluorescence spectra of a submicron Cs vapour layer under resonant excitation on the D2 line are measured. Sub-Doppler features centered at the resonance frequency of the hyperfine (hf) transitions have been observed. Substantial changes in the amplitude and width of the sub-Doppler resonances for individual hf transitions were recorded in dependence on the intensity of the incident laser radiation. In the fluorescence spectra narrow dips due to the effects of saturation have been observed. We also report about the observation of coherence resonances in Hanle configuration obtained at cell thickness of the order of the wavelength of the laser light.