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Physical Review B

Spin-dependent localization of electrons in quadruple quantum dots

A Kwaśniowski, Janusz Adamowski

Published Dec 7, 2010• 6 citations
Publisher

Abstract

An all electrical manipulation with singlet and triplet states of an electron pair in a quadruple quantum dot (QD) has been studied by a configuration interaction method. We have investigated two nanodevices that consist of four weakly coupled lateral QDs, in which the electron localization can be changed by tuning the external voltages: the gate voltage in the first nanodevice and the source-drain voltage in the second. The electrons that---in the initial state---singly occupy the two identical input QDs are transferred to the two asymmetric output QDs by the sufficiently high electric field. We have shown that---for the QDs with suitably chosen parameters---the localization of the electrons in the output QDs depends on the spin states of the electron pair and the final spin state can be uniquely determined by a single-shot measurement of the electric charge gathered in only one of the output QDs. This leads to a possibility of performing the controlled operations on the electron-spin qubits in the quadruple QDs. We have found that the classical exclusive OR (XOR) logic gate can be performed with the electric field-induced transitions and the output read out by the spin-to-charge conversion.

DOI
10.1103/physrevb.82.245306

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An all electrical manipulation with singlet and triplet states of an electron pair in a quadruple quantum dot (QD) has been studied by a configuration interaction method. We have investigated two nanodevices that consist of four weakly coupled lateral QDs, in which the electron localization can be changed by tuning the external voltages: the gate voltage in the first nanodevice and the source-drain voltage in the second. The electrons that---in the initial state---singly occupy the two identical input QDs are transferred to the two asymmetric output QDs by the sufficiently high electric field. We have shown that---for the QDs with suitably chosen parameters---the localization of the electrons in the output QDs depends on the spin states of the electron pair and the final spin state can be uniquely determined by a single-shot measurement of the electric charge gathered in only one of the output QDs. This leads to a possibility of performing the controlled operations on the electron-spin qubits in the quadruple QDs. We have found that the classical exclusive OR (XOR) logic gate can be performed with the electric field-induced transitions and the output read out by the spin-to-charge conversion.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
We present a method of changing the effective spin-spin interactions of electrons localized in quantum dot molecules from antiferromagnetic to ferromagnetic using electrical means. We show that starting with antiferromagnetic interaction of two electrons localized in two quantum dots, the effective spin-spin interaction can change to ferromagnetic by allowing interaction with a third dot containing two spin singlet electrons. The total spin of this four-electron complex can be tuned by changing the third dot potential from singlet to triplet. This is demonstrated using the linear combination of harmonic orbitals combined with the configuration-interaction method mapped onto the Hubbard and an effective $t\text{\ensuremath{-}}J$ model for the triple dot system. All three approaches predict singlet-triplet spin transition, i.e., a mechanism for changing the magnitude and sign of the effective Heisenberg interaction between two localized spins.
We study the two-qubit controlled-NOT gate operating on qubits encoded in the spin state of a pair of electrons in a double quantum dot. We assume that the electrons can tunnel between the two quantum dots encoding a single qubit, while tunneling between the quantum dots that belong to different qubits is forbidden. Therefore, the two qubits interact exclusively through the direct Coulomb repulsion of the electrons. We find that entangling two-qubit gates can be performed by the electrical biasing of quantum dots and/or tuning of the tunneling matrix elements between the quantum dots within the qubits. The entangling interaction can be controlled by tuning the bias through the resonance between the singly occupied and doubly occupied singlet ground states of a double quantum dot.
A pair of self-assembled InGaAs quantum dots filled with two electrons can act as a singlet-triplet spin qubit that is robust against nuclear spin fluctuations as well as charge noise. This results in a T2* coherence time two orders of magnitude longer than that of a single electron, provided the qubit is operated at a particular "sweet spot" in gate voltage. However, at this fixed operating point the ground-state splitting can no longer be tuned into resonance with e.g. another qubit, limiting the options for coupling multiple qubits. Here, we propose using a four-electron coupled quantum dot to implement a singlet-triplet qubit that features a magnetically tunable level splitting. As a first step towards full experimental realization of this qubit design, we use optical spectroscopy to demonstrate the tunability of the four-electron singlet-triplet splitting in a moderate magnetic field.
The effect of an external electric field on the exchange interaction has been studied by an exact diagonalization method for two electrons in laterally coupled quantum dots (QDs). We have performed a systematic study of several nanodevices that contain two gate-defined QDs with different shapes and sizes located between source and drain contacts. The confinement potential is modeled by two potential wells with a variable range and softness. In all the considered nanodevices, the overall dependence of exchange energy J on electric field F is similar, i.e. for low fields J increases with increasing F, while for intermediate fields J reaches a maximum and then abruptly falls to zero if F exceeds a certain critical value. However, the J(F) dependence also shows certain characteristic properties that depend on the nanodevice geometry. We have found that the low- and intermediate-field behavior can be accurately parameterized by a linear function J(F) = αF+β, where α is independent of the nanodevice geometry and softness of the confinement potential. We have shown that the linear J(F) relation appears only if the tunnel coupling between the QDs is weak, i.e. the interdot separation is sufficiently large. This relation becomes nonlinear for the strong interdot coupling. For specific nanodevices we have found that the J(F) dependence exhibits a plateau in a broad electric-field regime. The properties of the exchange energy found in the present paper can be applied to all electrical manipulation of electron spin qubits.