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Conference on Lasers and Electro-Optics Pacific Rim (CLEO-PR)

Modulation transfer spectroscopy for D2 transition line of rubidium

Heung‐Ryoul Noh, Sang Eon Park

Published Jun 1, 2013• 0 citations
Publisher

Abstract

When a frequency-modulated pump beam overlaps with a probe beam, new modulated probe beams are generated via nonlinear interaction with atoms. We observed this phenomenon for D2line of87Rb and compared with calculated results.
DOI
10.1109/cleopr.2013.6600609

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We conducted a theoretical and experimental study of lineshape in modulation transfer spectroscopy for ⁸⁷Rb atoms. When a linearly polarized pump beam, modulated at an angular frequency of Ω, overlaps in parallel with an unmodulated linearly polarized probe beam, combined modulated probe beams are generated via nonlinear interaction with atoms. The detected modulation transfer signals are calculated by numerically solving the complete optical Bloch equations for the ⁸⁷Rb atoms without the use of any phenomenological parameters. We find that the calculated results are in good agreement with experimental results.
We report modulation transfer spectroscopy on the D2 transitions in 85 Rb and 87 Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87 Rb F = 2 → F ' = 3 and the 85 Rb F = 3 → F ' = 4 transitions, can be significantly enhanced by expanding the beams, improving the signals for laser frequency stabilization. The signal gradient for these transitions is increased by a factor of 3 and the peak to peak amplitude was increased by a factor of 2. The modulation transfer signal for the 85 Rb F = 2 → F ' transitions is also presented to highlight how this technique can generate a single, clear line for laser frequency stabilization even in cases where there are a number of closely spaced hyperfine transitions.
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An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and probe beams have been varied to explore line broadening effects and signal-to-noise of each technique. This humble setup will hopefully grow into a more robust experimental arrangement in which double resonance, two-laser excitations are used to explore hyperfine state changing collisions between rubidium atoms and noble gas atoms. Rb-noble gas collisions can transfer population between hyperfine levels, such as 5P3/2 (F ′ = 3) Collision ←− 5P3/2 (F ′ = 2), and the probe beam couples 7S1/2 (F ′′ = 2) ← 5P3/2 (F ′ = 3). Polarization spectroscopy signal depends on the rate of population transfer due to the collision as well as maintaining the orientation created by the pump laser. Fluorescence spectroscopy relies only on transfer of population due to the collision. Comparison of these techniques yields information regarding the change of the magnetic sublevels, mF , during hyperfine state changing collisions.
The D_1 line of ^{85}Rb exhibits non-cycling transitions; therefore, only weak modulation transfer spectroscopy (MTS) signals could be obtained \cite{Khan2024}. In this study, however, strong MTS spectra were obtained for the D_1 line via optical pumping (OP) of the D_2 line of 85^{85}85Rb. Four linear parallel (lin \parallel lin) and linear perpendicular (lin\perplin), \sigma^+ - \sigma^+, and \sigma^+ - \sigma^- polarization configurations were investigated using an OP laser with four different polarizations such as linear horizontal (P), linear vertical (S), \sigma^+, and \sigma^- polarizations. Under the linear perpendicular configuration, the MTS signal for the F_g=3 \rightarrow F_e=2 transition of the D_1 line exhibited approximately a 41-fold increase in the signal slope in the presence of a linearly-polarized OP beam, compared with the signal slope obtained without OP. The calculated MTS spectra for the \sigma^+ \sigma^- configuration in the presence of \sigma^+- or \sigma^--polarized OP beam as an example matched well with experimental observations.