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Optics Communications

Polarization transfer between oriented metastable helium atoms and neon atoms: A comparison of even and odd isotopes

David M. Pepper, Harry T. M. Wang

Published Nov 1, 1983• 0 citations
Publisher
DOI
10.1016/0030-4018(83)90244-4

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Angular Momentum Transfer at the Chemo-ionization and Spin Exchange Processes. Interaction between Spin Polarized Metastable Helium Atoms

Victor A. Kartoshkin

In the collision of spin-polarized atoms, the transmission of electron polarization between colliding particles is possible. A similar situation occurs in a collision, for example, between alkali atoms in the ground state. If one of the colliding particles is in an excited state and its energy is sufficient for ionization of the collision partner, then along with the elastic process (spin exchange), an inelastic process (ionization) is also possible, as a result of these processes polarization can also be transferred to the partner. Simultaneously occurring elastic and inelastic processes at the collision between two helium atoms are possible if these atoms are in the metastable (23S1) state. The paper discusses the interaction between spin-polarized metastable atoms of helium-3 and helium-4 isotopes under conditions of optical pumping of atoms. Complex interaction potentials of the atoms under consideration were constructed and on their basis, the spin exchange and chemo-ionization cross-sections were calculated. Using these cross-sections, expressions for the transfer of orientation and alignment from one atom to another were obtained.

Mediterranean Journal of Chemistry•Oct 7, 2022•0 citations
A study of the physics of a nuclear magnetic resonance gyroscope is described. Experimental results in nuclear polarization and relaxation in 3He are obtained using an optical pumping apparatus and a high resolution rf spectroscopic technique. Polarization in the metastable states of the heavy noble gases (20, 21 Ne, 129, 132 Xe) was observed using a similar optical pumping apparatus. A sensitive detection method based on optical polarization of an excited state transition is developed and compared with the conventional method of monitoring optical transmission through the optical pumping cell. A new concept for the optical pumping of odd-mass-numbered heavy noble was isotopes to provide for ground-state nuclear polarization is discussed. Significant polarization in excited state neon was observed via collisional transfer from optically pumped helium in a cell filled with a mixture of helium and neon isotopes. The measured polarization was essentially independent of the isotopic composition. (Author)
In the collision of spin-polarized atoms, the transmission of electron polarization between colliding particles is possible. A similar situation occurs in a collision, for example, between alkali atoms in the ground state. If one of the colliding particles is in an excited state and its energy is sufficient for ionization of the collision partner, then along with the elastic process (spin exchange), an inelastic process (ionization) is also possible, as a result of these processes polarization can also be transferred to the partner. Simultaneously occurring elastic and inelastic processes at the collision between two helium atoms are possible if these atoms are in the metastable (23S1) state. The paper discusses the interaction between spin-polarized metastable atoms of helium-3 and helium-4 isotopes under conditions of optical pumping of atoms. Complex interaction potentials of the atoms under consideration were constructed and on their basis, the spin exchange and chemo-ionization cross-sections were calculated. Using these cross-sections, expressions for the transfer of orientation and alignment from one atom to another were obtained.