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Physics Today

The Most Tenuous of Molecules

Daniel Kleppner

Published Jul 1, 1995• 2 citations
Publisher
DOI
10.1063/1.2808084

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Physical Review Letters•Sep 9, 2005•21 citations
Small weakly bound boson-fermion 4Hem3Hen^{4}\mathrm{He}_{m}^{3}\mathrm{He}_{n}4Hem3​Hen​ clusters formed in a free jet expansion are identified using nondestructive transmission grating diffraction. The observations confirm the existence of more than 11 very tenuous complexes including the three-body halo molecule 4He23He^{4}\mathrm{He}_{2}^{3}\mathrm{He}4He23​He and the pseudo-Borromean complex 4He23He2^{4}\mathrm{He}_{2}^{3}\mathrm{He}_{2}4He23​He2​. Effective cluster formation temperatures, extracted from a sudden freeze model for cluster growth using theoretical binding energies, increase smoothly with cluster size, thereby confirming the calculations with the possible exception of 4He23He2^{4}\mathrm{He}_{2}^{3}\mathrm{He}_{2}4He23​He2​.