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Optics Letters

Subkilohertz linewidths measured by heterodyne-detected coherent population trapping in sodium vapor

Koji Motomura, 隆典 越水, Ken-ichi Harada, Hirotaka Ueno, Masaharu Mitsunaga

Published May 14, 2004• 10 citations
Publisher

Abstract

Subkilohertz spectroscopy by coherent population trapping (CPT) has been performed in Na atomic vapor. The system employs a frequency-swept acousto-optic modulator for bichromatic excitation as well as a heterodyne-lock-in detection technique that permits the direct measurement of the CPT dispersion curves at a good signal-to-noise ratio. A CPT linewidth of -400 Hz was measured as well as a steep refractive-index dispersion of as much as 3.3 x 10(-10) Hz(-1), corresponding to a group velocity of 1800 m/s.

DOI
10.1364/ol.29.001141

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Subkilohertz spectroscopy by coherent population trapping (CPT) has been performed in Na atomic vapor. The system employs a frequency-swept acousto-optic modulator for bichromatic excitation as well as a heterodyne-lock-in detection technique that permits the direct measurement of the CPT dispersion curves at a good signal-to-noise ratio. A CPT linewidth of -400 Hz was measured as well as a steep refractive-index dispersion of as much as 3.3 x 10(-10) Hz(-1), corresponding to a group velocity of 1800 m/s.
We report a phase-sensitive microwave detection setup for spectroscopy of coherent population trapping (CPT) resonance in a Cs vapor cell. In this scheme, the optically carried microwave interrogation signal that interacts with atoms is detected by a fast photodiode at the cell output and is then mixed with the local oscillator microwave signal itself. This detection scheme produces at the output of the microwave mixer a dispersive CPT signal that can be directly used for correction of the local oscillator frequency onto the atomic resonance. The evolution of the dispersive CPT resonance signal with the laser power is briefly reported. With this detection scheme, we demonstrate the operation of a CPT atomic clock with a short-term fractional frequency stability of 1 × 10 − 11 at 1 s, which is in good agreement with the slope of the frequency discriminator and the residual microwave phase noise of the setup.
An all-optical microwave frequency standard based on coherent population trapping (CPT) in 85Rb is developed. The CPT resonances are detected by an ordinary edge-emitting diode laser in a simple optical setup. A buffer-gas mixture is carefully optimized to yield a narrow linewidth and a reduced temperature dependence of the resonance frequency. With the developed system we are able to measure ultranarrow optically induced hyperfine CPT resonances at <20 Hz, which is in good agreement with the linewidth calculated from experimental parameters. The frequency of an RF-signal generator has been stabilized to the CPT resonance between the two mF=0 magnetic sublevels. The relative frequency stability (square root of Allan variance) follows a slope of 3.5×10-11 τ-1/2(1 s<τ<2000 s). The best stability of 6.4×10-13 is reached at an integration time of τ=2000 s. This stability is sufficient for many high-precision applications. Frequency-shift measurements were made to evaluate the frequency dependencies on the operation parameters.
Summary form only given. We report on recent experiments to use dark line coherent population trapping (CPT) resonances in cesium vapor as the basis for a compact frequency reference. The resonance is excited by directly modulating the injection current of a VCSEL at one-half the ground state hyperfine transition of Cs (4.6 GHz) to produce RF sidebands on the optical carrier. The laser output is then passed through a room-temperature cell containing Cs at its vapor pressure together with 8.7 kPa of Neon buffer gas and the transmitted optical power is detected in a photodiode. When the laser carrier is tuned half way between the two hyperfine components of the D/sub 2/ line at 852 nm, and the RF modulation frequency is adjusted to be equal to one-half the hyperfine splitting, the absorption of the sidebands through the cell is slightly reduced due to the CPT effect. As the RF frequency is scanned over the resonance, lock-in detection is used to produce a /spl sim/1 kHz wide dispersive error signal which is in turn used to stabilize the modulation frequency. The narrow signal is the result of the buffer gas, which reduces the time-of-flight broadening of the transition.
We report our measurement of coherent-population-trapping (CPT) signal linewidths in small vapor cells, which are desirable for chip scale atomic clock (CSAC) applications. The linewidths are measured in both rubidium vapor cells and cesium vapor cells. Using a micro-machined silicon absorption cell (diameter = 1.7 mm, length = 2 mm), we demonstrate a sub-kHz linewidth (FWHM) of the clock transition in the /sup 133/Cs atom (|F = 3, m/sub F/ = 0>/spl harr/|F = 4, m/sub F/ = 0>). The measured intrinsic linewidths (FWHM = 777 Hz for Cs and FWHM = 1496 Hz for Rb) of the cells agree with the calculated results.