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Physical Review Letters

Atomic Transitions in Finite-Bandwidth Squeezed Light

Helmut Ritsch, P. Zoller

Published Aug 29, 1988• 62 citations
Publisher

Abstract

A stochastic density-matrix equation for an atom strongly driven by finite-bandwidth squeezed light is derived. The quantum properties of the light are accounted for by a doubling of dimensions of the stochastic process for $c$-number electric field amplitudes. The possibility of obtaining reduced atomic linewidths in the absorption spectrum of the atom embedded in colored squeezed light is discussed, based on nonperturbative solutions of stochastic optical Bloch equations.

DOI
10.1103/physrevlett.61.1097

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A stochastic density-matrix equation for an atom strongly driven by finite-bandwidth squeezed light is derived. The quantum properties of the light are accounted for by a doubling of dimensions of the stochastic process for ccc-number electric field amplitudes. The possibility of obtaining reduced atomic linewidths in the absorption spectrum of the atom embedded in colored squeezed light is discussed, based on nonperturbative solutions of stochastic optical Bloch equations.
We derive stochastic density-matrix equations for an atom strongly driven by finite-bandwidth squeezed light. The quantum properties of the light are accounted for by a doubling of dimensions of the stochastic process for c-number electric field amplitudes. Saturation properties and the weak-field absorption spectrum of a two-level atom embedded in finite-bandwidth squeezed light and driven by a coherent field are calculated. We discuss the effect of finite bandwidth of the squeezed light in obtaining subnatural linewidth in the atomic absorption spectra, based on nonperturbative solutions of the stochastic optical Bloch equations.
The atomic Bloch equations driven by a quantum noise are investigated in the framework of c-number multiplicative stochastic Rabi amplitudes. It is shown that the stochastic broad-band vacuum fluctuations can be incorporated in such a way that spontaneous absorption is removed. It is shown that the multiplicative stochastic noise with no spontaneous absorption is equivalent to the quantum vacuum noise. A stochastic model of the broad-band squeezed vacuum is introduced and investigated. From such a stochastic description the fast and the slow damping rates of the Bloch polarizations are obtained. The strong-field resonance fluorescence spectrum and the steady-state atomic inversion for the stochastic model of squeezed vacuum fluctuations are derived.
In this paper, the optical Bloch equations of a two-level atom ensemble driven by squeezed light field are derived. Based on these equations, we calculate the atomic absorption and dispersion. The results show that for different squeezing conditions of the field fluctuations, atomic absorption-lineshape exhibits sub-or super-natural linewidth phenomenon. Atomic dispersion depends on the squeezing direction and coherent excitation direction of the driving field. When these two directions are not parallel or perpendicular to each other, the dispersion zero-point shows a shift to the transition frequency of the atom.
We present an analytical technique for investigating the behaviour of a coherently driven atom damped by a squeezed vacuum with finite squeezing bandwidth. A master equation and analytic expressions for the fluorescent spectrum are derived for the simple case of a two-level atom exactly resonant with the frequencies of both the squeezed field and the driving field. Suitable choices of driving strength, phase and squeezing source lead to either sub-natural lincwidths of the Rabi sidebands or a sub-natural linewidth of the central spectral peak or indeed sub-natural linewidths of all three spectral peaks when squeezing bandwidths are taken into account. We also establish the remarkable result that in the strong driving regime, the width of the central peak of the fluorescent spectrum depends solely on the squeezing found at the Rabi sideband frequencies.
The inhibition of atomic-phase decays by squeezed light, and consequent line narrowing, is reexamined for the case of finite-bandwidth squeezing, as produced in the output of a degenerate parametric amplifier. The extension of previous work to incorporate the effect of nonwhite, or colored, noise is accomplished via an adjoint equation, which gives the time evolution of a matrix functional of the incoming field. Simple equations for atomic variables are derived in which noise operators are defined so as to commute with each other and with all other quantities. This facilitates the reduction of a purely quantum-mechanical problem to a classical problem, solvable by classical stochastic-approximation methods. In particular, small-noise-approximation methods and simulations are carried out for a wide range of parameters describing the squeezed-field input. The method of simulation is extended to the computation of correlation functions and spectra for a realistically achievable set of parameters, with consideration given to reflections of the input in the emitted light. The fundamental effect is confirmed, and modifications to previous results are given.
The resonance fluorescence of a two-level atom driven by a coherent laser field and damped by a finite bandwidth squeezed vacuum is analysed. We extend the Yeoman and Barnett technique to a non-zero detuning of the driving field from the atomic resonance and discuss the role of squeezing bandwidth and the detuning in the level shifts, widths and intensities of the spectral lines. The approach is valid for arbitrary values of the Rabi frequency and detuning but for the squeezing bandwidths larger than the natural line-width in order to satisfy the Markoff approximation. The narrowing of the spectral lines is interpreted in terms of the quadrature-noise spectrum. We find that, depending on the Rabi frequency, detuning and the squeezing phase, different factors contribute to the line narrowing. For a strong resonant driving field there is no squeezing in the emitted field and the fluorescence spectrum exactly reveals the noise spectrum. In this case the narrowing of the spectral lines arises from the noise reduction in the input squeezed vacuum. For a weak or detuned driving field the fluorescence exhibits a large squeezing and, as a consequence, the spectral lines have narrowed linewidths. Moreover, the fluorescence spectrum can be asymmetric about the central frequency despite the symmetrical distribution of the noise. The asymmetry arises from the absorption of photons by the squeezed vacuum which reduces the spontaneous emission. For an appropriate choice of the detuning some of the spectral lines can vanish despite that there is no population trapping. Again this process can be interpreted as arising from the absorption of photons by the squeezed vacuum. When the absorption is large it may compensate the spontaneous emission resulting in the vanishing of the fluorescence lines.