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Journal of Physics A Mathematical and General

Conservative dynamics, phase ordering and stretched exponential decays

Chuck Yeung, David Jasnow

Published Dec 21, 1990• 4 citations
Publisher

Abstract

The authors discuss the dynamics of an observable field related to a locally conserved field. They show that for a model of phase ordering dynamics and for a variation of model C critical dynamics, that the two-time momentum space correlation function decays asymptotically as a stretched exponential. They show that under some conditions the asymptotic behaviour is experimentally observable and argue that the non-exponential behaviour is not a feature specific to these models but should rather apply for any observable coupled to a locally conserved field.

DOI
10.1088/0305-4470/23/24/005

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Physical Review E•Sep 17, 2009•2 citations
The authors discuss the dynamics of an observable field related to a locally conserved field. They show that for a model of phase ordering dynamics and for a variation of model C critical dynamics, that the two-time momentum space correlation function decays asymptotically as a stretched exponential. They show that under some conditions the asymptotic behaviour is experimentally observable and argue that the non-exponential behaviour is not a feature specific to these models but should rather apply for any observable coupled to a locally conserved field.
Abstract Time evolution, near a phase transition in the critical domain of critical systems not far from equilibrium, using a Langevin-type evolution is studied. Typical quantities of interest are relaxation rates towards equilibrium, time-dependent correlation functions and transport coefficients. The main motivation for such a study is that, in systems in which the dynamics is local (on short time-scales, a modification of a dynamic variable has an influence only locally in space) when the correlation length becomes large, a large time-scale emerges, which characterizes the rate of time evolution. This phenomenon called critical slowing down leads to universal behaviour and scaling laws for time-dependent quantities. In contrast with the situation in static critical phenomena, there is no clean and systematic derivation of the dynamical equations governing the time evolution in the critical domain, because often the time evolution is influenced by conservation laws involving the order parameter, or other variables like energy, momentum, angular momentum, currents and so on. Indeed, the equilibrium distribution does not determine the driving force in the Langevin equation, but only the dissipative couplings are generated by the derivative of the equilibrium Hamiltonian, and directly related to the static properties. The purely dissipative Langevin equation specifically discussed, corresponding to static models like the f4 field theory and two-dimensional models. Renormalization group (RG) equations are derived, and dynamical scaling relations established.
We review the progress made in dynamic bulk critical behaviour in equilibrium in the last 25 years since the review of Halperin and Hohenberg. We unify the presentation of the theoretical background by restricting ourselves to the field-theoretic renormalization group method. The main results obtained in the different universality classes are presented. This contains the critical dynamics near the gas–liquid transition in pure fluids (model H), the plait point and consolute point in mixtures (model H � ), the superfluid transition in 4 He (model F) and 4 He– 3 He mixtures (model F � ), the Curie point (model J) and Neel point (model G) in Heisenberg magnets and the superconducting transition. In comparison with experimental results, it became clear that in most cases one has to consider apart from the universal asymptotic critical behaviour also the non-universal effective behaviour. Either because it turned out to be inevitable due to a small dynamical transient exponent inhibiting the system to reach the asymptotics (e.g., at the superfluid transition) or because one is interested in the region further away from the phase transition like in pure fluids and mixtures at their gas–liquid or demixing transition. The calculation of the critical dynamics is adequate in most cases only in two-loop order. We review these results and present the solution to unreasonable features found for some models. Thus, we consider model C where relaxational and diffusive dynamics are coupled and the scaling properties and the limit to a purely relaxational model (model A) have not been understood. In general for models where the order parameter couples to other conserved densities time scale ratios between the kinetic coefficients of the order parameter and the conserved densities play an important role. Their fixed-point values and the approach to the fixed point are changed considerably in two-loop order compared to their values in one-loop order. These considerations are relevant for the explanation of the dynamical critical shape functions of systems such as superfluid helium (model F) and the isotropic antiferromagnet (model G). As far as possible, the comparison of results obtained by the renormalization group theory with numerical simulations has been made.
We now begin our exposition of universal dynamic scaling behavior that emerges under non-equilibrium conditions. We are mainly concerned with the relaxational models A and B here, but also touch on other dynamic universality classes. First, we consider non-equilibrium critical relaxation from a disordered initial state, and compute the associated universal scaling exponents within the dynamic renormalization group framework. Related phenomena in the early-time regime, prior to reaching temporally translationally invariant asymptotics, are ‘aging’ and a non-equilibrium fluctuation-dissipation ratio, both of which have enjoyed prominence in the literature on ‘glassy’ kinetics. In this context, we derive the critical initial slip exponent for the order parameter, and briefly discuss interesting persistence properties. Second, we explore the long-time scaling laws in phase ordering kinetics and coarsening for the relaxational models, following a fast temperature ‘quench’ into the ordered phase, in systems with either non-conserved or conserved order parameters. Aside from a few explicit computations in the spherical model limit (wherein the number of order parameter components n → ∞), we largely employ phenomenological considerations and scaling theory, stressing the importance of topological defects for energy dissipation during coarsening. Next we address the question how violations of Einstein's relation that links relaxation coefficients and noise correlations might affect the asymptotic dynamic critical scaling behavior. Whereas in systems with non-conserved order parameter typically the equilibrium scaling laws are recovered in the vicinity of the critical point, in contrast genuinely novel universality classes may emerge in the case of a conserved parameter, provided it is driven out of equilibrium in a spatially anisotropic fashion.
Simulations show that the autocorrelation function C(t) in the d=3 Ising model with a plaquette interaction has a stretched-exponential decay in a supercooled liquid phase. Such a decay characterizes also some ground-state probability distributions obtained from the numerically exact counting of up to 10^450 configurations. A related model with a strongly degenerate ground state but lacking glassy features does not exhibit such a decay. Tensionless modification of the droplet model might explain stretched-exponential decay of C(t) even in three-dimensional systems.
Dynamical scaling functions above Tc for the characteristic frequencies and the dynamical correlation functions of the order parameter and the conserved density of model C are calculated in one loop order. By a proper exponentiation procedure these results can be extended in order to consider the changes in these functions using the fixed point values and exponents in two loop order. The dynamical amplitude ratio R of the characteristic frequencies is generalized to the critical region. Surprisingly the decay of the shape functions at large scaled frequency does not behave as expected from applying scaling arguments. The exponent upsilon of the decay does not change when going from the critical to the hydrodynamic region although the shape functions change. The value of upsilon for the order parameter is in agreement with its value in the critical region, whereas for the conserved density it is equal to 2, the value in the hydrodynamic region.