A new scheme to observe saturated absorption resonances is presented. It is based on an active cavity with an amplifying medium. Experimental and theoretical comparisons with external and internal absorbing cell methods were carried out.
We present a new scheme of laser spectrometer based on an active optical cavity containing saturated absorbing and amplifying media. Such an active cavity may ensure enhancement in the amplitude of nonlinear optical resonances of saturated absorption at least by one order of magnitude as compared with similar passive system. The efficiency of the spectrometer was demonstrated by the observation of saturated absorption resonances in methane at a wavelength of 3.39 /spl mu/m under transit-time conditions. In these conditions, the contribution of fast molecules can be greatly reduced because of a finite interaction time of particles with the radiation field. In our work with a light beam 0.6 cm in diameter, we eliminated the transit-time broadening limit by using optical selection of slow methane molecules with a transverse velocity 20 times less than the mean thermal one, and obtained sub-DoppIer resonances with a homogeneous width less than 5 kHz.
Summary form only given. Results are presented of theoretical studies into the resonances of the saturated absorption and saturated dispersion in an external absorption cell. The theory has been worked out by means of combining methods of mathematical theory of diffraction and quantum mechanical method for computing the polarization of active media. This made it possible for the first time to find a self-consisting spatial solution of the density matrix equation for the two-level system and the Helmholtz equation for electromagnetic field and to solve the problem of propagation of two counterpropagating monochromatic waves though an absorbing nonlinear medium taking into consideration the transverse transit-time effect.
The behaviour of the amplitude of a saturated absorption resonance observed in laser radiation propagated through an active interferometer with nonlinear amplifying and absorbing media is studied experimentally for the first time. Upon variation of the gain in the amplifying medium and preserving a constant saturating field in the interferometer, a nonlinear increase in the amplitude of the saturated absorption resonance was observed. In this case, an increase in the detected signal exceeded an increase in the noise, i.e., the signal-to-noise ratio also increased.