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Optics Letters

Spectral technique for measuring hyperfine structure of atoms

Wang Yuzhu, Zhou Ru-fang, Zhou Zhiyiao, Ni Guo-Quan, Cai Weiquan

Published Jul 1, 1984• 2 citations
Publisher

Abstract

A new spectral technique for measuring the hyperfine structure of atoms is reported. A divergent atomic beam and a divergent laser beam are crossed. Because of the Doppler effect, the hyperfine structure of atomic levels will be directly displayed in the interaction region in the form of spatially resolved fluorescence arc hands. By measuring the spatial-fluorescence intensity distribution, it is possible to obtain the hyperfine splittings of atomic levels. Basic principles and experimental results are given.

DOI
10.1364/ol.9.000276

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A new spectral technique for measuring the hyperfine structure of atoms is reported. A divergent atomic beam and a divergent laser beam are crossed. Because of the Doppler effect, the hyperfine structure of atomic levels will be directly displayed in the interaction region in the form of spatially resolved fluorescence arc hands. By measuring the spatial-fluorescence intensity distribution, it is possible to obtain the hyperfine splittings of atomic levels. Basic principles and experimental results are given.
Abstract Resonance scattering techniques are very useful for high-resolution atomic spectroscopy. The applicability of these techniques has been much extended, particularly through the rapid development of tunable-laser technology. The use of a narrow-band tunable laser, acting on a collimated atomic beam, gives a direct method enabling, for example, hyperfine structure and isotope shift studies. The intensity of lasers allows stepwise excitations to be performed, and with the two-photon absorption technique, Doppler-free measurements on thermal gases are also possible. By using pulsed lasers, time-resolved measurements yielding radiative life-times and structural information can be performed. The basic resonance scattering methods can be combined with radiofrequency and coherence techniques to yield a resolution, limited only by the uncertainty relation. Optical double resonance and level-crossing techniques, not requiring a narrow-band light source, have been extensively used. Several examples of the application of resonance scattering methods are given.
Summary form only given. A Doppler free measurement of the hyperfine structure splitting (HFS) of 5S/sub 1/2/ level is performed using trapped sodium atoms. We employed two techniques: 1) trap loss enhancement, which consists in the observation of the trapped atom fluorescence when an extra loss channel is created by single photon ionization of the 5S state. This method was not very precise because the lack of absolute reference. 2) Photoionization out of 5S/sub 1/2/ after a two photon excitation from the 3S/sub 1/2/ state.
We have performed an analysis of the effect of hyperfine structure in an experiment in which an aligned excited state is probed using linearly polarized light. The state is born with a given electronic alignment resulting from a collisional process. It is probed after a time which is short in comparison to its radiative lifetime but much longer than ω−1hfs, where ℏωhfs is the hyperfine splitting. This means that hyperfine structure has ample time to ‘‘develop.’’ It is therefore essential to take into account both the hyperfine structure of the level and the manner in which the alignment is affected by recoupling to the new basis. Ratios of fluorescent intensities for different laser polarization configurations contain information on the alignment of the system. We show how these may be calculated for a system with several isotopes, some of which have hyperfine structure, and where many components are probed with appreciable strength. A comparison is made with our experimental results for the Hg(6 3P1) level probed on the 6 3P1–7 3S1 transition. The presence of hyperfine structure has a considerable influence on the measurements. It is important to understand such effects if one is to obtain information on the nascent electronic alignment by observation of the fluorescent intensities.
We have developed a rubidium atomic-beam light source that emits Rb lines with a Doppler width of only 0.0015 cm−1. When the light from this source was measured with a scanning Fabry–Perot interferometer and the data were reduced by digital computer utilizing numerical deconvolution techniques, we were able to determine a hyperfine level splitting in natural rubidium as small as 0.0014 cm−1 with an uncertainty of 0.0001 cm−1. We have measured the relative intensities and positions of 19 of the 20 hfs components of the two resonance lines, 7800 and 7974 Å, of natural Rb. From these data, we calculate isotope shifts σ87−σ85 = 0.00268 cm−1 for 52P32 and σ87′−σ85′ = 0.00259 cm−1 for 52P12.
An extremely thin cell with a wedge gap was developed that makes it possible to form a column of Rb atom vapor with thickness in the range from 100 to 600 nm. It is experimentally shown that the use of this cell, along with commercially available diode lasers, allows one to spectrally resolve individual transitions between the Zeeman sublevels of the hyperfine structure of the 87Rb D 1 line (transitions F g =1, 2→F e =1, 2) in the resonance fluorescence spectrum in the presence of an external magnetic field (B≈200 G). This makes it possible to realize systems consisting of nondegenerate atomic levels. For comparison, it is shown that transitions between the Zeeman sublevels in the fluorescence spectrum obtained with the aid of a conventional cell (1–10 cm long) in an external magnetic field with B∼200 G remain completely masked by the Doppler-broadened profile. The results obtained can be used for the creation of a simple magnetometer based on an extremely thin cell with Rb vapor for the measurement of magnetic fields with a submicron local spatial resolution.