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Open Systems & Information Dynamics

Spin-Based Quantum Information Processing in Magnetic Quantum Dots

Lucjan Jacak, J. Krasnyj, Dorota Jacak, R. Gonczarek, Mateusz Krzyżosiak, Paweł Machnikowski

Published May 31, 2005• 1 citation
Publisher

Abstract

We define the qubit as a pair of singlet and triplet states of two electrons in a He-type quantum dot (QD) placed in a diluted magnetic semiconductor (DMS) medium. The molecular field is here essential as it removes the degeneracy of the triplet state and strongly enhances the Zeeman splitting. Methods of qubit rotation as well as two-qubit operations are suggested. The system of a QD in a DMS is described in a way which allows an analysis of the decoherence due to spin waves in the DMS subsystem.

DOI
10.1007/s11080-005-5724-0

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We define the qubit as a pair of singlet and triplet states of two electrons in a He-type quantum dot (QD) placed in a diluted magnetic semiconductor (DMS) medium. The molecular field is here essential as it removes the degeneracy of the triplet state and strongly enhances the Zeeman splitting. Methods of qubit rotation as well as two-qubit operations are suggested. The system of a QD in a DMS is described in a way which allows an analysis of the decoherence due to spin waves in the DMS subsystem.
Abstract The spin degrees of freedom in quantum dot (QD) embedded in a diluted magnetic semiconductor (DMS) medium are considered in a model of a qubit and a gate for quantum information processing (QIP). The qubit is defined as a singlet and triplet pair of states of two electrons in a He‐type QD in the DMS medium with strongly enhanced gyromagnetic factor. Methods of qubit rotation (Rabi oscillations) as well as two‐qubit operations are suggested and analyzed. Moreover, decoherence related to spin waves (magnon‐induced dephasing) in this new system (QD in DMS) is studied, and the relevant time‐scale is estimated in accordance with preliminary experimental results. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
We present theoretically the Zeeman coupling and exchange induced swap action in spin-based quantum dot quantum computer models in the presence of magnetic field. We study the valence and conduction band states in a double quantum dots made in diluted magnetic semiconductor. The later have been proven to be very useful in building an all-semiconductor platform for spintronics. Due to a strong p–d exchange interaction in diluted magnetic semiconductor (Cd0.57Mn0.43Te), the relative contribution of this components is strongly affected by an external magnetic field, a feature that is absent in non magnetic double quantum dots. We determine the energy spectrum and the swap time as a function of magnetic field and the inter dot distance within the Hund–Mulliken molecular-orbit approach and by including the Coulomb interaction.
A Pauli spin blockade in quantum dot systems occurs when the charge transport is allowed only for some spin states, and it has been an efficient tool in spin-based qubit devices in semiconductors. We theoretically investigate a Pauli spin blockade in a triple quantum dot molecule consisting of three identical quantum dots in a semiconductor in the presence of an external magnetic field through the molecule. When the three-electron state is on resonance with two- or four-electron states, the Aharonov–Bohm oscillation and the Zeeman splitting lead to a periodic spin blockade effect. We focus on the spin blockade at a two- and three-electron resonance and show that we can tune the magnetic field to selectively allow only either a spin-singlet or spin-triplet state to add an additional electron from tunnel-coupled leads. This spin blockade maintains the three quantum dots at the optimal sweet spot against the charge noise, demonstrating its potential as an efficient readout scheme for the qubits in quantum dot systems.
We propose altermagnetic semiconductors as a platform for field-free, all-electrically controlled spin qubits in gate-defined quantum dots. The momentum-dependent spin splitting of an altermagnet produces a Zeeman-like qubit splitting whose magnitude and sign are set by the dot ellipticity, enabling local frequency tunability without external magnetic fields or micromagnets. Because the splitting is tied to a fixed altermagnetic quantization axis, electric-field noise is longitudinally suppressed at leading order, while quantization-axis fluctuations couple transversely and therefore cause relaxation rather than pure dephasing. The compensated magnetic order also avoids stray fields, making the platform naturally compatible with superconducting resonators and dispersive circuit-QED readout through the qubit's spin-dependent electric dipole. Starting from an effective quantum-dot model, supported by a microscopic lattice model, we derive the single- and two-dot Hamiltonian models. We show that electric-dipole spin resonance enables single-qubit control, while tunable exchange and electrically addressable qubit frequencies realize fSim two-qubit gates. The same double-dot architecture also supports singlet-triplet qubits with electrical control of both exchange and splitting gradients, removing the need for micromagnets or nuclear-polarization gradients. These results establish altermagnetic quantum dots as a route to field-free spin qubits with intrinsic electrical tunability and enhanced dephasing protection.
We investigate theoretically the hyperfine-induced dephasing of two-electron-spin states in a double quantum dot with a finite singlet-triplet splitting JJJ. In particular, we derive an effective pure dephasing Hamiltonian, which is valid when the hyperfine-induced mixing is suppressed due to the relatively large JJJ and the external magnetic field. Using both a quantum theory based on resummation of ring diagrams and semiclassical methods, we identify the dominant dephasing processes in regimes defined by values of the external magnetic field, the singlet-triplet splitting, and inhomogeneity in the total effective magnetic field. We address both free induction and Hahn echo decay of superposition of singlet and unpolarized triplet states (both cases are relevant for singlet-triplet qubits realized in double quantum dots). We also study hyperfine-induced exchange gate errors for two single-spin qubits. Results for III-V semiconductors as well as silicon-based quantum dots are presented.