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Physica status solidi. C, Conferences and critical reviews/Physica status solidi. C, Current topics in solid state physics

Zeeman coupling and Swap action in spin‐based diluted magnetic semiconductor quantum dot quantum computer

A. Hichri, S. Jaziri

Published Mar 29, 2004• 0 citations
Publisher

Abstract

We present theoretically the Zeeman coupling and exchange induced swap action in spin-based quantum dot quantum computer models in the presence of magnetic field. We study the valence and conduction band states in a double quantum dots made in diluted magnetic semiconductor. The later have been proven to be very useful in building an all-semiconductor platform for spintronics. Due to a strong p–d exchange interaction in diluted magnetic semiconductor (Cd0.57Mn0.43Te), the relative contribution of this components is strongly affected by an external magnetic field, a feature that is absent in non magnetic double quantum dots. We determine the energy spectrum and the swap time as a function of magnetic field and the inter dot distance within the Hund–Mulliken molecular-orbit approach and by including the Coulomb interaction.

DOI
10.1002/pssc.200304413

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We present theoretically the Zeeman coupling and exchange induced swap action in spin-based quantum dot quantum computer models in the presence of magnetic field. We study the valence and conduction band states in a double quantum dots made in diluted magnetic semiconductor. The later have been proven to be very useful in building an all-semiconductor platform for spintronics. Due to a strong p–d exchange interaction in diluted magnetic semiconductor (Cd0.57Mn0.43Te), the relative contribution of this components is strongly affected by an external magnetic field, a feature that is absent in non magnetic double quantum dots. We determine the energy spectrum and the swap time as a function of magnetic field and the inter dot distance within the Hund–Mulliken molecular-orbit approach and by including the Coulomb interaction.
We consider a quantum-gate mechanism based on electron spins in coupled semiconductor quantum dots. Such gates provide a general source of spin entanglement and can be used for quantum computers. We determine the exchange coupling JJJ in the effective Heisenberg model as a function of magnetic (B)(B)(B) and electric fields, and of the interdot distance aaa within the Heitler-London approximation of molecular physics. This result is refined by using sp\mathrm{sp}sp hybridization, and by the Hund-Mulliken molecular-orbit approach, which leads to an extended Hubbard description for the two-dot system that shows a remarkable dependence on BBB and aaa due to the long-range Coulomb interaction. We find that the exchange JJJ changes sign at a finite field (leading to a pronounced jump in the magnetization) and then decays exponentially. The magnetization and the spin susceptibilities of the coupled dots are calculated. We show that the dephasing due to nuclear spins in GaAs can be strongly suppressed by dynamical nuclear-spin polarization and/or by magnetic fields.
We perform time-dependent simulations of spin exchange for an electron pair in laterally coupled quantum dots. The calculation is based on configuration interaction scheme accounting for spin-orbit (SO) coupling and electron-electron interaction in a numerically exact way. Noninteracting electrons exchange orientations of their spins in a manner that can be understood by interdot tunneling associated with spin precession in an effective SO magnetic field that results in anisotropy of the spin swap. The Coulomb interaction blocks the electron transfer between the dots but the spin transfer and spin precession due to SO coupling is still observed. The electron-electron interaction additionally induces an appearance of spin components in the direction of the effective SO magnetic field which are opposite in both dots. Simulations indicate that the isotropy of the spin swap is restored for equal Dresselhaus and Rashba constants and properly oriented dots.
We calculate the effect of an inhomogeneous magnetic field, which is invariably present in an experimental environment, on the exchange energy of a double-quantum-dot artificial molecule, projected to be used as a two-qubit quantum gate in the proposed quantum-dot quantum computer. We use two different theoretical methods to calculate the Hilbert space structure in the presence of the inhomogeneous field: the Heitler-London method, which is carried out analytically, and the molecular orbital method, which is done computationally. Within these approximations we show that the exchange energy J changes slowly when the coupled dots are subject to a magnetic field with a wide range of inhomogeneity, suggesting that swap operations can be performed in such an environment as long as quantum error correction is applied to account for the Zeeman term. We also point out the quantum interference nature of this slow variation in exchange.
We determine the spin-exchange coupling J between two electrons located in two vertically tunnel-coupled quantum dots, and its variation when magnetic (B) and electric (E) fields (both in-plane and perpendicular) are applied. We predict a strong decrease of J as the in-plane B field is increased, mainly due to orbital compression. Combined with the Zeeman splitting, this leads to a singlet-triplet crossing, which can be observed as a pronounced jump in the magnetization at in-plane fields of a few T, and perpendicular fields of the order of 10 T for typical self-assembled dots. We use harmonic potentials to model the confining of electrons, and calculate the exchange J using the Heitler-London and Hund-Mulliken techniques, including the long-range Coulomb interaction. With our results we provide experimental criteria for the distinction of singlet and triplet states, and therefore for microscopic spin measurements. In the case where dots of different sizes are coupled, we present a simple method to switch the spin coupling on and off with exponential sensitivity using an in-plane electric field. Switching the spin coupling is essential for quantum computation using electronic spins as qubits.
We report on our recent progress in applying semiconductor quantum dots for spin-based quantum computation, as proposed by Loss and DiVincenzo (1998 Phys. Rev. A 57 120). For the purpose of single-electron spin resonance, we study different types of single quantum dot devices that are designed for the generation of a local ac magnetic field in the vicinity of the dot. We observe photon-assisted tunnelling as well as pumping due to the ac voltage induced by the ac current driven through a wire in the vicinity of the dot, but no evidence for ESR so far. Analogue concepts for a double quantum dot and the hydrogen molecule are discussed in detail. Our experimental results in laterally coupled vertical double quantum dot device show that the Heitler–London model forms a good approximation of the two-electron wavefunction. The exchange coupling constant J is estimated. The relevance of this system for two-qubit gates, in particular the SWAP operation, is discussed. Density functional calculations reveal the importance of the gate electrode geometry in lateral quantum dots for the tunability of J in realistic two-qubit gates.