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Applied Physics Letters

Efficient broadband frequency conversion via simultaneous adiabatic three wave mixing processes

Gil Porat, Ady Arie

Published Apr 15, 2013• 15 citations
Publisher

Abstract

Two frequency-cascaded and spatially simultaneous three-wave-mixing processes, each pumped by a different frequency, are studied in a quasi-phase-matching crystal with chirped poling. Theory, numerical simulation, and experiment all show that efficient two-process adiabatic frequency conversion takes place over a broad range of input wavelengths. Experimentally, up to five process cascades are obtained. Furthermore, it is demonstrated that reversing the chirp sign results in a different conversion for the same input wavelength. This method can be applied to generation of an all-optically tunable frequency comb.

DOI
10.1063/1.4802597

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Two frequency-cascaded and spatially simultaneous three-wave-mixing processes, each pumped by a different frequency, are studied in a quasi-phase-matching crystal with chirped poling. Theory, numerical simulation, and experiment all show that efficient two-process adiabatic frequency conversion takes place over a broad range of input wavelengths. Experimentally, up to five process cascades are obtained. Furthermore, it is demonstrated that reversing the chirp sign results in a different conversion for the same input wavelength. This method can be applied to generation of an all-optically tunable frequency comb.
In the field of nonlinear frequency conversion, the cascaded frequency conversion scheme is an effective means to obtain new wavelengths. In this paper, we demonstrate efficient frequency conversion through three cascaded three-wave mixing processes based on Stark-chirped rapid adiabatic passage, which are different from previous cascaded wavelength conversion processes based on stimulated Raman adiabatic passage. Further, by analyzing the relevant parameters in the three-process cascaded frequency conversion models we have established, we find that the new scheme increases the conversion range and has lower restrictions on the conversion conditions while maintaining extremely low intermediate frequency intensity. These advantages allow our work to be applied to the acquisition of a mid-infrared or visible laser.
We propose an efficient broadband frequency generation technique for two collinear optical parametric processes ω3=ω1+ω2ω_3=ω_1+ω_2ω3​=ω1​+ω2​ and ω4=ω1−ω2ω_4=ω_1-ω_2ω4​=ω1​−ω2​. It exploits chirped quasi-phase-matched gratings, which in the undepleted pump approximation regime perform population transfer that is analogous to adiabatic population transfer in a three-state ``vee'' quantum system. The energy of the input fields is transferred adiabatically either into ω3ω_3ω3​ or ω4ω_4ω4​ field, depending on which of the two phase matchings occurs first by the local modulation period in the crystal. One can switch the output between ω3ω_3ω3​ and ω4ω_4ω4​ by inverting the direction of the local modulation sweep, which corresponds to a rotation of the crystal by angle πππ
We propose an adiabatic scheme for cascaded fourth-harmonic generation (FHG) in chirped dual-period quasi-phase-matched (QPM) crystals, where adiabatic evolution is introduced into the multi-step frequency conversion process. By engineering two chirped QPM gratings for the fundamental-to-second-harmonic ( FF → SH ) and second-to-fourth-harmonic ( SH → FH ) interactions, efficient harmonic generation is achieved through a continuous adiabatic passage in phase-mismatch space, rather than discrete phase-matching conditions in conventional QPM schemes. This approach enables robust and tunable energy transfer among harmonics, allowing controllable generation of second- and fourth-harmonic signals. Numerical results show a maximum FHG efficiency of 94% and a tunable bandwidth of ∼13 nm under realistic conditions. The tunability originates from the controlled shift of QPM resonances along the propagation direction.
An efficient broadband sum-frequency generation (SFG) technique using the two cascaded optical parametric processes ${\ensuremath{\omega}}_{3}={\ensuremath{\omega}}_{1}+{\ensuremath{\omega}}_{2}$ and ${\ensuremath{\omega}}_{4}={\ensuremath{\omega}}_{1}+{\ensuremath{\omega}}_{3}$ is proposed. The technique uses chirped quasi-phase-matched gratings, which, in the undepleted pump approximation, make SFG analogous to adiabatic population transfer in three-state systems with crossing energies in quantum physics. If the local modulation period first makes the phase match occur for ${\ensuremath{\omega}}_{3}$ and then for ${\ensuremath{\omega}}_{4}$ SFG processes then the energy is converted adiabatically to the ${\ensuremath{\omega}}_{4}$ field. Efficient SFG of the ${\ensuremath{\omega}}_{4}$ field is also possible by the opposite direction of the local modulation sweep; then transient SFG of the ${\ensuremath{\omega}}_{3}$ field is strongly reduced. Most of these features remain valid in the nonlinear regime of depleted pump.
Abstract The method of adiabatic frequency conversion, in analogy with a two‐level atomic system, has been put forward recently and verified experimentally to achieve robust frequency mixing processes such as sum and difference frequency generation. Here a comparative study of efficient frequency mixing using various techniques of shortcuts to adiabaticity such as counter‐diabatic driving and invariant‐based inverse engineering is presented. It is shown here that it is possible to perform sum frequency generation by properly designing the poling structure of a periodically poled crystal and the coupling between the input lights and the crystal. The required crystal length for frequency conversion significantly decreases beyond the adiabatic limit. This approach significantly improves the robustness of the process against the variation in temperature as well as the signal frequency. By introducing a single parameter control technique with constant coupling and combining with the inverse engineering, perturbation theory, and optimal control, it is shown that the phase mismatch can be further optimized with respect to the fluctuations of input wavelength and crystal temperature that results into a novel experimentally realizable mixing scheme.
We demonstrate that the frequency conversion in the cascaded processes can be mapped uniquely to an associated three-wave mixing processes in adiabatic evolution. After solving the coupling wave equations of three-wave mixing processes, we immediately find the solutions of the corresponding cascaded coupled equations. Furthermore, we introduce a rather simple model, which displays the main features of the optical stimulated Raman adiabatic passage (STIRAP) but allows for analytic evaluation of all quantities. It performs two simultaneous three-wave mixing processes efficiently and without significant generation of an intermediate frequency. At last, we consider in detail the effects of the phase mismatch to the optical STIRAP efficiency, which show that the analytic bounds are seen to describe the transfer region very accurately.