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Review of Scientific Instruments

In situ magnetic compensation for potassium spin-exchange relaxation-free magnetometer considering probe beam pumping effect

Jiancheng Fang, Tao Wang, Wei Quan, Heng Yuan, Hong Zhang, Yang Li, Sheng Zou

Published Jun 1, 2014• 69 citations
Publisher

Abstract

A novel method to compensate the residual magnetic field for an atomic magnetometer consisting of two perpendicular beams of polarizations was demonstrated in this paper. The method can realize magnetic compensation in the case where the pumping rate of the probe beam cannot be ignored. In the experiment, the probe beam is always linearly polarized, whereas, the probe beam contains a residual circular component due to the imperfection of the polarizer, which leads to the pumping effect of the probe beam. A simulation of the probe beam's optical rotation and pumping rate was demonstrated. At the optimized points, the wavelength of the probe beam was optimized to achieve the largest optical rotation. Although, there is a small circular component in the linearly polarized probe beam, the pumping rate of the probe beam was non-negligible at the optimized wavelength which if ignored would lead to inaccuracies in the magnetic field compensation. Therefore, the dynamic equation of spin evolution was solved by considering the pumping effect of the probe beam. Based on the quasi-static solution, a novel magnetic compensation method was proposed, which contains two main steps: (1) the non-pumping compensation and (2) the sequence compensation with a very specific sequence. After these two main steps, a three-axis in situ magnetic compensation was achieved. The compensation method was suitable to design closed-loop spin-exchange relaxation-free magnetometer. By a combination of the magnetic compensation and the optimization, the magnetic field sensitivity was approximately 4 fT/Hz(1/2), which was mainly dominated by the noise of the magnetic shield.

DOI
10.1063/1.4881685

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IEEE Access•Jan 1, 2019•20 citations
A novel method to compensate the residual magnetic field for an atomic magnetometer consisting of two perpendicular beams of polarizations was demonstrated in this paper. The method can realize magnetic compensation in the case where the pumping rate of the probe beam cannot be ignored. In the experiment, the probe beam is always linearly polarized, whereas, the probe beam contains a residual circular component due to the imperfection of the polarizer, which leads to the pumping effect of the probe beam. A simulation of the probe beam's optical rotation and pumping rate was demonstrated. At the optimized points, the wavelength of the probe beam was optimized to achieve the largest optical rotation. Although, there is a small circular component in the linearly polarized probe beam, the pumping rate of the probe beam was non-negligible at the optimized wavelength which if ignored would lead to inaccuracies in the magnetic field compensation. Therefore, the dynamic equation of spin evolution was solved by considering the pumping effect of the probe beam. Based on the quasi-static solution, a novel magnetic compensation method was proposed, which contains two main steps: (1) the non-pumping compensation and (2) the sequence compensation with a very specific sequence. After these two main steps, a three-axis in situ magnetic compensation was achieved. The compensation method was suitable to design closed-loop spin-exchange relaxation-free magnetometer. By a combination of the magnetic compensation and the optimization, the magnetic field sensitivity was approximately 4 fT/Hz(1/2), which was mainly dominated by the noise of the magnetic shield.
Maintaining a near-zero magnetic field condition is a requisite for atomic magnetometer under the spin-exchange relaxation-free (SERF) regime. Therefore, the precise determination of the residual magnetic fields is of great significance. Herein, we proposed an in-situ measurement method of residual magnetic fields in a dual-beam atomic magnetometer based on a transient response of the transverse polarization along the probe beam direction after switching off the pump beam. Proceeding from the Bloch equation, we established a complete evolution expression of the polarization vector under any static residual magnetic field with the pump beam switched off. On this basis, we analyzed the transient response of the transverse polarization by numerical simulation under different situations of residual magnetic fields. Besides, we also considered two possible conditions when the residual magnetic fields are relatively large or small, respectively. Accordingly, we presented an efficient and convenient estimation method of the residual magnetic fields based on certain time characteristics of the transient response. We verified the feasibility of our method by experiment and achieved a triaxial residual magnetic fields measurement within 0.5 s. This method can realize an in situ and real-time measurement of the residual magnetic fields in a fast and convenient way. Furthermore, this method can evaluate the effectiveness of different magnetic field compensation methods without introducing any modulation or extra devices.
The spin-exchange-relaxation-free (SERF) atomic magnetometer is an ultra-high sensitivity magnetometer, but it must be operated in a magnetic field with strength less than about 10 nT. Magnetic field compensation is an effective way to shield the magnetic field, and this paper demonstrates an in situ triaxial magnetic field compensation system for operating the SERF atomic magnetometer. The proposed hardware is based on optical pumping, which uses some part of the SERF atomic magnetometer itself, and the compensation method is implemented by analyzing the dynamics of the atomic spin. The experimental setup for this compensation system is described, and with this configuration, a residual magnetic field of strength less than 2 nT (±0.38 nT in the x axis, ±0.43 nT in the y axis, and ±1.62 nT in the z axis) has been achieved after compensation. The SERF atomic magnetometer was then used to verify that the residual triaxial magnetic fields were coincident with what were achieved by the compensation system.
The most efficient way to improve the sensitivity of an optically pumped magnetometer (OPM) is to maximize the spin-polarization lifetime of the atoms. The spin exchange relaxation-free (SERF) OPM that operates in zero field environment is one of the most sensitive magnetic sensors. This paper proposes a new three-axis magnetic field compensation method for the single-beam OPM, which zeroes the magnetic field around the sensor to make it work in SERF regime. The method simultaneously employs two modulation magnetic fields and two low-frequency sweeping magnetic fields along two directions perpendicular to the laser beam during the compensation process. The output signal of the photodiode is demodulated at different frequencies, resulting in two outputs that reflect the three components of the magnetic field. This method does not require iterate to tune the three-axis field, which increases the speed of the compensation process significantly. The magnetic field resolutions of the method for the x-axis, y-axis and z-axis are 0.6 pT, 0.6 pT and 5 pt, respectively. A compact OPM with noise density about 20 fT / Hz1/2@10 Hz is developed and tested, demonstrating the feasibility of the method.
A method of measuring in-situ magnetic field gradient is proposed in this paper. The magnetic shield is widely used in the atomic magnetometer. However, there is magnetic field gradient in the magnetic shield, which would lead to additional gradient broadening. It is impossible to use an ex-situ magnetometer to measure magnetic field gradient in the region of a cell, whose length of side is several centimeters. The method demonstrated in this paper can realize the in-situ measurement of the magnetic field gradient inside the cell, which is significant for the spin relaxation study. The magnetic field gradients along the longitudinal axis of the magnetic shield are measured by a spin-exchange relaxation-free (SERF) magnetometer by adding a magnetic field modulation in the probe beam’s direction. The transmissivity of the cell for the probe beam is always inhomogeneous along the pump beam direction, and the method proposed in this paper is independent of the intensity of the probe beam, which means that the method is independent of the cell’s transmissivity. This feature makes the method more practical experimentally. Moreover, the AC-Stark shift can seriously degrade and affect the precision of the magnetic field gradient measurement. The AC-Stark shift is suppressed by locking the pump beam to the resonance of potassium’s D1 line. Furthermore, the residual magnetic fields are measured with σ + - and σ – -polarized pump beams, which can further suppress the effect of the AC-Stark shift. The method of measuring in-situ magnetic field gradient has achieved a magnetic field gradient precision of better than 30 pT/mm.
In this article, we analyze the amplitude-frequency and phase-frequency responses of a spin-exchange relaxation-free (SERF) atomic magnetometer with the nonorthogonal angle between the pump and probe beam. The optical nonorthogonality leads to a change in the photon spin direction of circularly polarized pump light, which decides the polarization direction of the atomic ensemble, causing significant differences in dynamic responses to the magnetic field. We theoretically analyze relationships between dynamic response solutions of the Bloch equation with different pump lights and magnetic field directions based on which the equations are linearized. The equations are solved with the Fourier transform method, and three-axis dynamic responses are obtained under the influences of optical nonorthogonality and residual static magnetic field. In the experiment, we verify the linear superposition characteristics between different response components. According to the results, we propose a novel method to quickly calibrate the nonorthogonal angle, which could reduce the optical nonorthogonal angle by 20 times, reaching 0.54°, and effectively enhance the dynamic magnetic field response signal in atomic magnetometers.
In this study, we demonstrate a non-modulated triaxial magnetic field compensation method for spin-exchange relaxation-free (SERF) atomic magnetometers. We realize simultaneous compensation of the magnetic field along the pump and probe directions by maximizing the first order differential value of the zero-field resonance signal. The magnetic field perpendicular to the pump-probe plane is compensated by zeroing the DC response of the magnetometer. The zero-field resonance is obtained by applying a linearly changed magnetic field along the direction perpendicular to that of the pump-probe plane. The first order differential of the zero-field resonance is acquired using the second order central difference method in real time. Compared with the conventional compensation methods, this method does not involve modulation and demodulation. Therefore, it requires no lock-in amplifier, thus making it more applicable in miniature atomic devices. Moreover, this method compensates the magnetic field along the pump and probe directions using only one criterion. It avoids the cross-talk effect between the pump and probe directions in the presence of non-orthogonal coils. The experiment results show that the compensation resolution is 9 pT, 7 pT and 0.05 pT for the probe, pump, and direction perpendicular to the pump-probe plane, respectively.