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Soviet Journal of Quantum Electronics

Boundary-value problems in nonlinear optics of resonant media

V. I. Rupasov, Vladimir I. Yudson

Published Nov 30, 1982• 26 citations
Publisher

Abstract

A study is made of the problem of transmission of light pulses by a boundary of a nonlinear medium under conditions of coherent interaction with matter. It is shown that in the case of a semiinfinite nonlinear medium the reflection coefficient is governed by the linear characteristics of the media in contact so that the boundary-value problem reduces to the Cauchy problem. In another case, when a nonlinear medium is a thin film at the interface between two linear media, it is found that such a film is an almost perfect mirror reflecting weak pulses but it becomes transparent to pulses of sufficiently high intensity and the mirror then modulates the amplitude of such pulses.

DOI
10.1070/qe1982v012n11abeh006090

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A study is made of the problem of transmission of light pulses by a boundary of a nonlinear medium under conditions of coherent interaction with matter. It is shown that in the case of a semiinfinite nonlinear medium the reflection coefficient is governed by the linear characteristics of the media in contact so that the boundary-value problem reduces to the Cauchy problem. In another case, when a nonlinear medium is a thin film at the interface between two linear media, it is found that such a film is an almost perfect mirror reflecting weak pulses but it becomes transparent to pulses of sufficiently high intensity and the mirror then modulates the amplitude of such pulses.
A linear response of a resonant medium to a weak electromagnetic field is studied in the case when a medium is a gas of three-level atoms subjected to a strong saturating pulse. A noncoherent intense pulse and a coherent 2π pulse (of the kind encountered in the theory of self-induced transparency) are considered. The expressions obtained are used to study the problem of the spectrum of the reflection of light by a pulse moving in a medium. An analysis is made of the possibility of using the Doppler effect, which occurs when light is reflected by a moving pulse, in an investigation of the characteristics of pulse propagation, determination of its parameters, and study of the nonlinear characteristics of the medium itself. Possibilities of experimental observation of the predicted effects are discussed, particularly the possibility of conversion of an electromagnetic radiation spectrum.
In a recent paper1 I formulated a method for calculating propagation through nonlinear media for a number of nonlinear optical phenomena. This method does not use the SVEA and can therefore solve nonlinear propagation problems when refraction and reflection at the boundary interfaces are important. Here, I report the first calculation using this exact (albeit numerical) method. For this first test of the utility of the method, I have chosen to study optical bistability in a thin film whose index of refraction is intensity dependent.
A theoretical investigation is reported of the coherent nonlinear response of excitons and biexcitons in a thin semiconductor film subjected to resonant laser radiation. It is shown that saturation of an exciton transition results in an abrupt qualitative change in the nature of film transmission from total reflection of the incident pulse at low pump amplitudes to oscillatory reflection at high amplitudes. A new area theorem is derived for ultrashort pulses: it establishes a correspondence between the areas of the incident, transmitted, and reflected pulses. Anomalous transmission and reflection (area 'quantisation') is predicted for large values of the nonlinear parameter. The equations of state, describing bistable behaviour of the amplitudes of the fields of the transmitted and reflected radiation, are derived for quasi-cw operation.