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Soviet Journal of Quantum Electronics

Scattering of light by an intense saturating pulse in a resonance medium

V. I. Rupasov

Published Nov 30, 1982• 2 citations
Publisher

Abstract

A linear response of a resonant medium to a weak electromagnetic field is studied in the case when a medium is a gas of three-level atoms subjected to a strong saturating pulse. A noncoherent intense pulse and a coherent 2π pulse (of the kind encountered in the theory of self-induced transparency) are considered. The expressions obtained are used to study the problem of the spectrum of the reflection of light by a pulse moving in a medium. An analysis is made of the possibility of using the Doppler effect, which occurs when light is reflected by a moving pulse, in an investigation of the characteristics of pulse propagation, determination of its parameters, and study of the nonlinear characteristics of the medium itself. Possibilities of experimental observation of the predicted effects are discussed, particularly the possibility of conversion of an electromagnetic radiation spectrum.

DOI
10.1070/qe1982v012n11abeh006079

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A linear response of a resonant medium to a weak electromagnetic field is studied in the case when a medium is a gas of three-level atoms subjected to a strong saturating pulse. A noncoherent intense pulse and a coherent 2π pulse (of the kind encountered in the theory of self-induced transparency) are considered. The expressions obtained are used to study the problem of the spectrum of the reflection of light by a pulse moving in a medium. An analysis is made of the possibility of using the Doppler effect, which occurs when light is reflected by a moving pulse, in an investigation of the characteristics of pulse propagation, determination of its parameters, and study of the nonlinear characteristics of the medium itself. Possibilities of experimental observation of the predicted effects are discussed, particularly the possibility of conversion of an electromagnetic radiation spectrum.
An analysis is made of the evolution of a light pulse in a two-level resonant medium as a function of the degree of preliminary excitation by another pulse. It is shown that, in addition to self-induced transparancy observed under certain conditions associated with the degree of excitation of the atomic system, resonance scattering is also found due to the existence of macroscopic polarization of the medium. This scattering is not observed when the medium is in a noncoherent state. The transverse reversible relaxation time T * 2 can be determined from the variation of the scattering intensity.
An analysis is made of the propagation of a short coherent optical pulse in a three-level resonant medium with an essentially nonequidistant spectrum as a function of the degree of preexcitation of the medium. It is found that in addition to self-induced transparency and resonance scattering, stimulated Raman scattering (Stokes or anti-Stokes) should be observed under certain spatial phase-matching conditions. The area theorem is formulated for all radiation components. An analysis is made of the case of propagation of a resonant electromagnetic pulse of frequency ω in a system of three-level atoms having an equidistant spectrum. Under conditions of preexcitation of the medium at the frequency 2ω by longitudinal acoustic pulses, a scattered transverse acoustic wave at the frequency ω may be observed.
A study is made of the problem of transmission of light pulses by a boundary of a nonlinear medium under conditions of coherent interaction with matter. It is shown that in the case of a semiinfinite nonlinear medium the reflection coefficient is governed by the linear characteristics of the media in contact so that the boundary-value problem reduces to the Cauchy problem. In another case, when a nonlinear medium is a thin film at the interface between two linear media, it is found that such a film is an almost perfect mirror reflecting weak pulses but it becomes transparent to pulses of sufficiently high intensity and the mirror then modulates the amplitude of such pulses.
A review is given of the investigations of the coherent interaction of light pulses with resonantly absorbing two-level media. An analysis is made of the self-induced transparency discovered by McCall and Hahn and of its importance in quantum electronics. Bleached states associated with the phase modulation are considered in detail. A comparison is made with the theory of nonlinear waves of different physical origin. A review is given of some possible physical applications associated with the discriminatory nature of the transmission and delay of light in the self-induced transparency effect.
An expression is obtained for the nonlinear susceptibility governing the addition of frequencies under resonance conditions. Allowance is made for the Stark shift, changes in populations, and transient response of the medium. Analysis is made of the stimulated emission of the third harmonic as a result of two-photon resonance in parallel and focused beams. It is shown that the saturation effect limits seriously the conversion coefficient of a nonlinear medium of fixed length. Optimal intensities of the fundamental-frequency radiation are found. It is shown that when a beam is focused sharply in a nonlinear medium, the saturation effect and Stark shift make it possible to add frequencies in media with normal dispersion. The relationship between four-photon parametric effects and coherent resonant processes such as self-induced transparency is established for ultrashort pulses.