Beyond traditional nonlinear optics with large numbers of atoms and photons, qualitatively new phenomena arise in a quantum regime of strong interactions between single atoms and photons. By using a microscopic optical resonator, we achieved such interactions and demonstrated a robust, efficient mechanism for the regulated transport of photons one by one. With critical coupling of the input light, a single atom within the resonator dynamically controls the cavity output conditioned on the photon number at the input, thereby functioning as a photon turnstile. We verified the transformation from a Poissonian to a sub-Poissonian photon stream by photon counting measurements of the input and output fields. The results have applications in quantum information science, including for controlled interactions of single light quanta and for scalable quantum processing on atom chips.
Beyond traditional nonlinear optics with large numbers of atoms and photons, qualitatively new phenomena arise in a quantum regime of strong interactions between single atoms and photons. By using a microscopic optical resonator, we achieved such interactions and demonstrated a robust, efficient mechanism for the regulated transport of photons one by one. With critical coupling of the input light, a single atom within the resonator dynamically controls the cavity output conditioned on the photon number at the input, thereby functioning as a photon turnstile. We verified the transformation from a Poissonian to a sub-Poissonian photon stream by photon counting measurements of the input and output fields. The results have applications in quantum information science, including for controlled interactions of single light quanta and for scalable quantum processing on atom chips.
This research program investigated the dynamics of open quantum systems in manifestly quantum or nonclassical domains. The research program exploited recently discovered possibilities in the microscopic realm of quantum mechanics to accomplish tasks that would otherwise be impossible by traditional classical means, including new capabilities for precision measurement and for the processing and distribution of information. Within this setting, the particular investigations related to strong coupling in optical physics whereby nonlinear interactions require only single atoms and photons. The research achieved capabilities beyond traditional nonlinear optics and laser physics and moved into a new regime with dynamical processes involving atoms and photons taken one by one. The research program addressed fundamental issues related to quantum metrology, to quantum communications, and to the general development of quantum information sciences. The most important accomplishments of this work have been the following: (1) The first demonstration of a laser that operates with a single atom; (2) The first realization of a deterministic source for single photons that generates single photons "on demand" from one atom trapped in a cavity; (3) The development of a protocol for the real-time determination of the number of trapped atoms inside an optical cavity in a regime of strong coupling, with N = 0,1,2,3...atoms; and (4) The first experiment to achieve manifestly quantum or nonclassical photon correlations suitable for the implementation of scalable quantum communications networks.
Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.
Although conventional lasers operate with a large number of intracavity atoms, the lasing properties of a single atom in a resonant cavity have been theoretically investigated for more than a decade. Here we report the experimental realization of such a one-atom laser operated in a regime of strong coupling. Our experiment exploits recent advances in cavity quantum electrodynamics that allow one atom to be isolated in an optical cavity in a regime for which one photon is sufficient to saturate the atomic transition. In this regime the observed characteristics of the atom-cavity system are qualitatively different from those of the familiar many atom case. Specifically, we present measurements of intracavity photon number versus pump intensity that exhibit "thresholdless" behavior, and infer that the output flux from the cavity mode exceeds that from atomic fluorescence by more than tenfold. Observations of the second-order intensity correlation function demonstrate that our one-atom laser generates manifestly nonclassical light that exhibits both photon antibunching and sub-Poissonian photon statistics.
We consider the dynamics of single photons in a nonlinear optical cavity. When the Kerr nonlinearities of atomic dark resonances are utilized, the cavity mode is well described by a spin- 1/2 Hamiltonian. We show that it is possible to achieve coherent control of the cavity-mode wave function using $\ensuremath{\pi}$ pulses for single photons that switch the state of the cavity with very high accuracy. The underlying physics is best understood as the nonlinearity induced anticorrelation between single-photon injection/emission events, which we refer to as photon blockade. We also propose a method which uses these strong dispersive interactions to realize a single-photon turnstile device.
In this thesis, we study a system consisting of qubits—two-level quantum systems— interacting in the strong-coupling regime for a finite amount of time with a mode of the electromagnetic field inside a resonator. In particular, we are interested in the dynamics of the photon number and the possibility of controlling its statistics to produce sub-Poissonian light. To describe the system we use quantum trajectory theory where the time evolution of the state vector consists of both a continuous part and jumps, which account for the resonator losses. We also incorporate a variable number of qubits (changing in time) interacting with the mode. A computer simulation was developed and optimised to calculate the quantum trajectories. When one sets the qubits initially to the excited state and fixes the interaction time accordingly, so-called “trapping states” (photon numbers which block the addition of a photon by a single qubit) appear. These states are instrumental in the generation of sub-Poisson fields, for some cases even when the number of interacting qubits follow a Poisson process. We take advantage of the existence of trapping states to implement control protocols based on the measurement of the output field of the resonator, with the objective of lowering the uncertainty in the number of photons. Furthermore, we explore the possibility of creating a source of sub-Poissonian pulses by first using a random interaction time (which bypasses the trapping states) and then utilising the control protocols developed. We are able to achieve fields with a Mandel Q parameter of QM = −0.98 and a photon number of n 68.
Quantum opto-mechanics is a fast moving, broad research field which aims to investigate and control the interaction of light and the quantized motion of mechanical objects and the coupling between them. This allows one to engineer the mechanical quantum state by controlling and measuring the electromagnetic field, and conversely, to control the dynamical evolution of the optical field via its interaction with a mechanical system. Mechanical resonators are accessible in many different shapes and sizes, from kilogram scales in experiments that test gravitational theories to micro- and nano-scales in resolved sideband regime, where the frequency of the mechanical resonator is larger than the bandwidth of the optical cavity. In this regime, it is possible to cool the mechanical object to the ground state which allows a high degree of control and the ability to prepare interesting non-classical states, states that could aid in investigating the quantum dynamics of macroscopic objects. The field of quantum opto-mechanics is a promising testbed for quantum control technologies, such as fundamental tests of quantum mechanics, ultra-sensitive quantum sensors for precise measurements, phonon lasing, mechanical memories with long lifetime and quantum information processing. Furthermore, experiments are progressing toward strong opto-mechanical coupling regimes with single photons. This creates a platform that can take advantage of the nonlinear optical interactions to generate highly non-classical states in such light-matter interfaces. Photonic systems working in the single photon regime will be promising for low power applications and also for implementations of quantum information and computation. Motivated by these applications, this thesis consists of theoretical studies in the context of single photonics. This includes investigating non-classical mechanical state generation and mechanically controlling the dynamical evolution of optical fields in the strong coupling regime single photon opto-mechanics and furthermore, proposing a quantum sensor using single photonics. In this regard, we employ three important formalisms to treat and measure open quantum systems with non-Gaussian input fields: the conditional and unconditional cascaded master equations, Fock-state master equations and input-output Langevin equations. In the context of opto-mechanics, the system to be investigated is composed of two optical cavities with a coupling modulated via a mechanical resonator. In one case, a sequence of single photons are irreversibly sent to one of the optical cavities. After photons go through the opto-mechanical interaction, photon counting measurements are performed on the cavity output, conditionally steering the mechanical state to a highly non-classical Fock state. Numerical calculations are performed to predict the experimental parameters needed to generate a mechanical Fock state before the mechanical object is thermalized. In another case, the same opto-mechanical scheme is employed to conversely modify the state of the optical mode by engineering the state of the mechanical degree of freedom. In this case, it is shown that the opto-mechanical system operates as an effective beam splitter for the input single photons, with a transmission that can be controlled by tuning the number of excitations in the bulk mechanical resonator. When the mechanical resonator has a small coherent amplitude it acts as a quantum control, entangling the optical and mechanical degrees of freedom. As the coherent amplitude of the resonator increases, it acts as a classical control for the input photons. Finally, we propose a novel multi-purpose sensor architecture that can be used for force, refractive index and possibly local temperature detection. In this scheme, two coupled cavities behave as an effective beam splitter. This sensor is based on fourth order interference (the Hong-Ou-Mandel effect) and requires a sequence of single photon pulses and consequently has low pulse power. Changes in the parameter to be measured induce variations in the effective beam splitter reflectivity and result in changes to the visibility of interference. We propose that this generic scheme could be implemented with coupled L3 photonic crystal cavities and find that this system, which only relies on photon coincidence detection and does not need any spectral resolution, can estimate forces as small as 10-7 Newtons and can measure one part per million change in refractive index using a very low input power of 10-10 W.