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arXiv:0811.0264 · Physical Review Letters

Two-Photon Gateway in One-Atom Cavity Quantum Electrodynamics

Alexander Kubanek, Alexei Ourjoumtsev, I. Schuster, M. Koch, Pepijn W. H. Pinkse, Karim Murr, Gerhard Rempe

Published Nov 13, 2008• 132 citations
arXivHTMLPDF

Abstract

Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.

DOI
10.1103/physrevlett.101.203602

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Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.
Atoms absorb and emit resonant light photon by photon. However, an atom strongly coupled to the light field of a high-finesse optical resonator forms a new system with new characteristics, enabling the emission and absorption of photon pairs. The energy eigenstates of the coupled system form an anharmonic ladder of doublets, the so-called Jaynes-Cummings ladder. The first doublet, consisting of the two so-called normal modes, has been observed in various cavity QED systems. It can be explained classically using Maxwell equations as arising from the coupling of a classical dipole to a classical electromagnetic field. In contrast, the higher-order doublet has so far no classical analogue. It requires both the quantization of the atomic internal state as well as the quantization of light.
This thesis reports on experiments with single atoms strongly coupled to a single mode of a high-finesse optical cavity. In the first part, it is shown that the motion of the atom in an intracavity dipole trap can be observed with high spatial and temporal resolution. Depending on the atom's current position, the dipole trap is switched to control the motion of the atom. The feedback acts in real time, faster than one oscillation period of the atom in the trap. In the second part the anharmonic energy level structure of the system is investigated. This anharmonicity allows one to selectively populate states containing two energy quanta in a two-photon process, resulting in a nonlinear response of the system with respect to the drive laser intensity. The photon statistics of the light transmitted through the cavity shows photon bunching and super-Poissonian fluctuations, indicating the transmission of photon pairs typical for a two-photon gateway.
A tutorial review is given on recent experiments performed with 1 ⩽ N ⩽ 110 atoms in a microscopic high-finesse optical cavity. The resonator has length 1 mm and finesse 80 000. The radiative properties of the strongly coupled atom-cavity system differ from those of the individual components. For example, spontaneous emission is reversible, the first excited state of the composite system splits into two levels and the intensity fluctuations of the light transmitted by the resonator are nonclassical. We observe photon-antibunching and sub-Poissonian photon statistics. In terms of practical applications, the system renders possible ( i ) the detection of single atoms with high sensitivity and ( ii ) optical bistability for a few atoms and photons only.
We propose and analyze a scheme for photon trapping in an optical resonator coupled with two-level atoms. We show that when the cavity is excited by two identical light fields, one from each end of the cavity, the output light from the cavity is suppressed while the intracavity light field is nearmaximum due to the excitation of the polariton state of the coupled cavity and atom system. We also present methods for the direct probing of the trapped polariton state. The photon trapping is manifested by the destructive interference of the transmitted light and the incident light, which is conditioned on the presence of incoherent processes such as spontaneous decay of the atomic excitation of the polariton state. Such photon trapping is quite generic and should be observable experimentally in a variety of cavity quantum electrodynamics systems.
Although conventional lasers operate with a large number of intracavity atoms, the lasing properties of a single atom in a resonant cavity have been theoretically investigated for more than a decade. Here we report the experimental realization of such a one-atom laser operated in a regime of strong coupling. Our experiment exploits recent advances in cavity quantum electrodynamics that allow one atom to be isolated in an optical cavity in a regime for which one photon is sufficient to saturate the atomic transition. In this regime the observed characteristics of the atom-cavity system are qualitatively different from those of the familiar many atom case. Specifically, we present measurements of intracavity photon number versus pump intensity that exhibit "thresholdless" behavior, and infer that the output flux from the cavity mode exceeds that from atomic fluorescence by more than tenfold. Observations of the second-order intensity correlation function demonstrate that our one-atom laser generates manifestly nonclassical light that exhibits both photon antibunching and sub-Poissonian photon statistics.
A single atom in free space can have a strong influence on a light beam and a single photon can have a strong effect on a single atom in free space. Regarding this interaction, two conceptually different questions can be asked: can a single atom fully absorb a single photon and can a single atom fully reflect a light beam. The conditions for achieving the full effect in either case are different. Here we discuss related questions in the context of an optical resonator. When shaping a laser pulse properly it will be fully absorbed by an optical resonator, i.e., no light will be reflected and all the pulse energy will accumulate inside the resonator before it starts leaking out. We show in detail that in this case the temporal pulse shape has to match the time-reversed pulse obtained by the cavity’s free decay. On the other hand a resonator, made of highly reflecting mirrors which normally reflect a large portion of any incident light, may fully transmit the light, as long as the light is narrow band and resonant with the cavity. The analogy is the single atom—normally letting most of the light pass—which under special conditions may fully reflect the incident light beam. Using this analogy we are able to study the effects of practical experimental limitations in the atom-photon coupling, such as finite pulses, bandwidths, and solid angle coverage, and to use the optical resonator as a test bed for the implementation of the quantum experiment.