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Journal of the Optical Society of America B

Polarization photon-gated persistent spectral hole burning

Zhao Lizeng, Xiaomei Zhang, Yong Hua Qin, Zhenzhong Lu, Yuxin Nie, Duoyuan Wang, Minxue Hu, Lingzhi Hu

Published Jul 1, 1997• 0 citations
Publisher

Abstract

Polarization photon-gated persistent spectral hole burning (PSHB) was performed for the meso-phenyl-tetrabenzoporphyrinato-zinc–aromatic cyanide system. Excellent signal-to-noise ratio was obtained. The polarization dependence of the gating effect was observed and studied. Hole filling was investigated in the polarization photon-gated PSHB. Over 100 photon-gated holes have been burned and detected for this system by polarization spectroscopy.

DOI
10.1364/josab.14.001591

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Polarization photon-gated persistent spectral hole burning (PSHB) was performed for the meso-phenyl-tetrabenzoporphyrinato-zinc–aromatic cyanide system. Excellent signal-to-noise ratio was obtained. The polarization dependence of the gating effect was observed and studied. Hole filling was investigated in the polarization photon-gated PSHB. Over 100 photon-gated holes have been burned and detected for this system by polarization spectroscopy.
We introduce a method of polarization spectroscopy into photon-gated persistent spectral hole burning, which results in considerable improvement in the signal-to-background ratio. Fifty multiple spectral holes burnt into meso-phenyl-tetrabenzoporphyrinato-zinc/aromatic cyanide/poly(methyl methacrylate) were clearly detected by this measurement technique. We developed a simplified model to account for the hole shapes. Background birefringence combined with refractive dispersion is thought to play a key role in the generation of asymmetric line shapes.