Spinning Atoms with the Orbital Angular Momentum of Light

L. Allen, M. Babiker, W. L. Power

Sonja Franke‐Arnold

Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'.

Xiong-Jun Liu, Xin Liu, L. C. Kwek +1 more

Daisuke Akamatsu, Mikio Kozuma

We generated orbital angular momentum in atoms with a spin degree of freedom and coherently transferred it to a light field, which resulted in the generation of a Laguerre-Gaussian (LG) beam. In this method, atoms obtain orbital angular momentum through Larmor precession around the quadrupole field. Successive operations of quadrupole and homogeneous magnetic fields lead to a change of sign in the LG beam or even generation of superposition states of the LG beam with different indexes in real time. Possible applications to control orbital angular momentum of arbitrary photons are also discussed.

Gordon R. M. Robb, Padma Kant Shukla, José Tito Mendonça +2 more

Alex Schimmoller, Spencer Walker, Alexandra S. Landsman

Light contains both spin and orbital angular momentum. Despite contributing equally to the total photonic angular momentum, these components derive from quite different parts of the electromagnetic field profile, namely its polarization and spatial variation, respectively, and therefore do not always share equal influence in light–matter interactions. With the growing interest in utilizing light’s orbital angular momentum to practice added control in the study of atomic systems, it becomes increasingly important for students and researchers to understand the subtlety involved in these interactions. In this article, we present a review of the fundamental concepts and recent experiments related to the interaction of beams containing orbital angular momentum with atoms. An emphasis is placed on understanding light’s angular momentum from the perspective of both classical waves and individual photons. We then review the application of these beams in recent experiments, namely single- and few-photon transitions, strong-field ionization, and high-harmonic generation, highlighting the role of light’s orbital angular momentum and the atom’s location within the beam profile within each case.