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Cross-correlations and Entanglement in Cavity QED

Matthew L. Terraciano

Published Jun 30, 2006• 0 citations
OpenAlex

Abstract

Every quantum system subjected to measurements is an open quantum system. The cavity QED system is elegant in that it probes the interaction between two quantum systems, the atom and the field, while its loss mechanisms are well understood and can be externally monitored. The study of cross-correlations in cavity QED is important for understanding how entanglement evolves in open quantum systems. As quantum information science grows we need to learn more about entanglement and how it can be quantified and measured. Correlation functions have been used to compare an electromagnetic field (intensity) of one mode with the electromagnetic field (intensity) of the same mode at a later time or different spatial location. In quantum optics, correlation functions have been calculated and measured to probe the nonclassical field that results from the interaction of a single mode of the electromagnetic field and an ensemble of two-level atoms (the canonical cavity QED system). This field can exhibit antibunching, squeezing, and can violate inequalities required for a classical field. Entanglement in the steady state of a cavity QED system cannot be measured directly with traditional correlation functions (Hanbury-Brown and Twiss type experiments). Cross-correlations, however, interrogate directly both modes of the entangled pair, the transmitted (cavity) and the fluorescent (atom) intensities, and can act as an entanglement witness. This thesis presents the implementation of a cross-correlation measurement in a cavity QED system. The work has required the construction of an apparatus that incorporates laser cooling and trapping with quantum optics to carefully control both the external (center of mass motion) and internal (atomic state) degrees of freedom of a collection of atoms that interact with a single mode of a high finesse Fabry-Perot cavity. We examine theoretically and experimentally a new intensity cross-correlation function which probes the evolution of the cavity field conditioned on the detection of a fluorescent photon from an atom in the cavity. The results open the possibility to generalize the dynamics of entanglement as a physical resource necessary for the nascent quantum information science.

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Every quantum system subjected to measurements is an open quantum system. The cavity QED system is elegant in that it probes the interaction between two quantum systems, the atom and the field, while its loss mechanisms are well understood and can be externally monitored. The study of cross-correlations in cavity QED is important for understanding how entanglement evolves in open quantum systems. As quantum information science grows we need to learn more about entanglement and how it can be quantified and measured. Correlation functions have been used to compare an electromagnetic field (intensity) of one mode with the electromagnetic field (intensity) of the same mode at a later time or different spatial location. In quantum optics, correlation functions have been calculated and measured to probe the nonclassical field that results from the interaction of a single mode of the electromagnetic field and an ensemble of two-level atoms (the canonical cavity QED system). This field can exhibit antibunching, squeezing, and can violate inequalities required for a classical field. Entanglement in the steady state of a cavity QED system cannot be measured directly with traditional correlation functions (Hanbury-Brown and Twiss type experiments). Cross-correlations, however, interrogate directly both modes of the entangled pair, the transmitted (cavity) and the fluorescent (atom) intensities, and can act as an entanglement witness. This thesis presents the implementation of a cross-correlation measurement in a cavity QED system. The work has required the construction of an apparatus that incorporates laser cooling and trapping with quantum optics to carefully control both the external (center of mass motion) and internal (atomic state) degrees of freedom of a collection of atoms that interact with a single mode of a high finesse Fabry-Perot cavity. We examine theoretically and experimentally a new intensity cross-correlation function which probes the evolution of the cavity field conditioned on the detection of a fluorescent photon from an atom in the cavity. The results open the possibility to generalize the dynamics of entanglement as a physical resource necessary for the nascent quantum information science.
We investigate steady state entanglement in an open quantum system, specifically a single atom in a driven optical cavity with cavity loss and spontaneous emission. The system reaches a steady pure state when driven very weakly. Under these conditions, there is an optimal value for atom-field coupling to maximize entanglement, as larger coupling favors a loss port due to the cavity enhanced spontaneous emission. We address ways to implement measurements of the entanglement and find that normalized cross-correlation functions are indicators of the entanglement in the system. The equal time intensity-field cross correlation between the transmitted field of the cavity and the fluorescence intensity is proportional to the entanglement of formation for weak driving fields.
Cavity quantum electrodynamics (QED) in the strong-coupling regime provides the opportunity to monitor and control the dynamics of a simple quantum system. A single Cesium atom interacts strongly with single-photon fields in the mode of a high-finesse optical cavity. When the resulting coherent coupling rate dominates dissipation in the system, strong coupling is realized and the system displays distinctively quantum behavior. The coupling between atomic internal states and the quantized cavity field allows for diverse protocols in quantum state preparation, quantum communication, and quantum logic. However, the atom's external or motional state must also be taken into account. My research develops cavity QED in the limit where the coherent atom-field coupling dominates the atomic kinetic energy and thus significantly affects the atomic center-of-mass motion. In this regime, the interaction of the atom with the cavity field provides both a means of controlling atomic motion and a signal for detecting that motion in real time with high signal-to-noise. The sensing capability of the ``atom-cavity microscope" is exploited to trap single atoms with single-photon fields and to monitor their orbits in real time as they are bound in the cavity. Such real-time position sensing is the basis for a detailed strategy and ongoing experiment to actively stabilize select aspects of an atom's motion within the cavity. As the cavity-enabled position measurement approaches the standard quantum limit, this work begins to realize a quantum servo for atomic position and to address questions of optimal state estimation and state preparation. In combination with other progress in cavity QED, it furthers the goal of controlled atom-field interactions for quantum information science.
In order to study quantum effects such as state superposition and entanglement, one would like to construct simple systems for which the damping rates are slow relative to the rate of coherent evolution. One such system is strong-coupling cavity quantum electrodynamics (QED), in which a single atom is coupled to a single mode of a high finesse optical cavity. In recent years, optical trapping techniques have been applied to the cavity QED system, allowing an individual atom to remain coupled to the cavity for long periods of time. For the purpose of future cavity QED experiments, one would like to gain as much control over the trapped atom as possible; in particular, one would like to cool the center of mass motion of the atom, to measure the magnetic field at the location of the atom, and to be able to prepare the atom in a given internal state. In the first part of this thesis, I present a scheme for driving Raman transitions inside the cavity that can be used to achieve these goals. After giving a detailed theoretical treatment of the Raman scheme, I describe how it can be implemented in the lab and discuss some preliminary experimental results. In the second part of this thesis, I present a number of simple field theory models. These models were developed in an attempt to understand some of the central ideas of theoretical physics by looking at how the ideas work in a highly simplified context. The hope is that by reducing the mathematical complexity of an actual theory, the underlying physical concepts can be more easily understood.
The experiments discussed in this thesis focus on the interaction of a single trapped atom with the single mode of a high-finesse optical cavity, in the regime of strong coupling. Chapter 1 gives a brief introduction, after which Chapter 2 describes our recent measurements of the transmission spectrum of the atom-cavity system. The spectrum exhibits a clearly resolved vacuum-Rabi splitting, in good quantitative agreement with theoretical predictions. A new Raman scheme for cooling atomic motion along the cavity axis enables a complete spectrum to be recorded for an individual atom trapped within the cavity mode, in contrast to all previous measurements of this type that have required averaging over 10^3-10^5 atoms. Chapter 3 discusses our observations of photon blockade for the transmitted light in the presence of one trapped atom. Excitation of the atom-cavity system by a first photon blocks the transmission of a second one, thereby converting an incident Poissonian stream of photons into a sub-Poissonian, anti-bunched stream, as confirmed by measurements of the photon statistics of the transmitted field. The intensity correlations of the cavity transmission also reveal the energy distribution for oscillatory motion of the trapped atom. Chapter 4 details a set of simple but necessary measurements of relevant experimental parameters such as cavity geometry, linewidth, mirror properties, birefringence, and detection efficiency. The thesis concludes with Appendix A, describing the efficient laser setup we use for our magneto-optical traps.
We consider two systems in the weak driving field limit. The first is an optical parametric oscillator, the transmitted field of which is highly bunched. We discuss a conditioned measurement of the second order intensity correlation function that yields antibunching. The second system we consider is a single two level atom inside a weakly driven cavity. Here we consider cross correlations between the transmitted and fluorescent fields. A strong asymmetry in delay time has been noted by Denisov et. al., here we find strong violations of a classical inequality for the cross correlation.