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Memoirs of the Faculty of Science Kyoto University Series of physics astrophysics geophysics and chemistry

Stark Structure and Field Ionization Characteristics of Highly Excited Rydberg Atoms

Yasuhiro Kishimoto

Published Mar 1, 2002• 0 citations
Publisher

Abstract

The Stark structure and time evolution of highly excited 85Rb Rydberg states in a pulsed eiectr!c fieid have been studied experimentally as weil as theoretically.The Rydberg states in 85Rb with the principal quantum number n ranging from 110 to 140 have been excited with the two step laser excitation scheme and field ionization spectra under the pulsed eiectric field were observed with the ionlzed e!ectron iis: sit non-adiabatic t ' ' '

DOI
10.17983/257659

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Acta Physica Sinica•Jan 1, 2010•10 citations
The Stark structure and time evolution of highly excited 85Rb Rydberg states in a pulsed eiectr!c fieid have been studied experimentally as weil as theoretically.The Rydberg states in 85Rb with the principal quantum number n ranging from 110 to 140 have been excited with the two step laser excitation scheme and field ionization spectra under the pulsed eiectric field were observed with the ionlzed e!ectron iis: sit non-adiabatic t ' ' '
The outer electron of a Rydberg atom is so weakly bound to the atomic core that a relatively small electric field may cause the electron to be stripped from the atom. The field strength at which this ionization happens is strongly dependent on the state of the Rydberg atom. Pulsed electric field ionization serves, therefore, not only as a means by which a Rydberg atom may be efficiently detected, but also a means by which the state of the Rydberg atom may be analyzed.\nThe first observation of predominantly diabatic passage to field ionization of a non-hydrogenic Rydberg atom has resulted in an improved understanding of the adiabatic and diabatic ionization processes. The magnitudes of the various field ionization features have been measured and found to agree with theory, and by detailed analysis, it is now possible to label the various field ionization signal features with the appropriate (VBAR)m(,l)(VBAR) quantum numbers. A much better understanding of the laser excitation process, the Rydberg state production, and the response of the excited state to an increasing electric field has enabled measurement of some Rydberg fine-structure intervals, through observation of field ionization quantum beats.
Field ionization of high Rydberg manifold states (n=112–137)(n=112\text{--}137)(n=112–137) of rubidium-85 under a rotating electric field has been investigated experimentally and theoretically. Applying a rapidly reversed electric field with a small static perpendicular field to rotate the total electric field around zero, we have observed substantial increase of the fraction of the tunneling field-ionization process and a profound broadening of its ionization peak over a wide range of field strengths with increasing transverse electric field. The observed tunneling field-ionization fraction is almost independent of the slew rate of the applied electric field, and also on the principal quantum number nnn over the range investigated. To compare with these experimental results, theoretical calculations have been performed with a successive two-step regime. As the first step we calculated the redistributions of magnetic quantum number ${m}_{\ensuremath{\ell}}$ and parabolic quantum number ${n}_{1}\ensuremath{-}{n}_{2}$ of the states under the rotating electric field. Then the following time evolution of the manifold states with $\ensuremath{\mid}{m}_{\ensuremath{\ell}}\ensuremath{\mid}\ensuremath{\leqslant}3$ was traced on the Stark map in a coherent as well as an incoherent model. The calculated results are generally in good agreement with the experimental ones. The increase of the tunneling field-ionization fraction under a rotating electric field plays an essential role in achieving the high efficiency in the recently proposed selective-field-ionization scheme for high Rydberg atoms.
The high-l Rydberg Stark states are populated by the state transfer from initial prepared nS Rydberg state via avoided crossings induced by a weak electric-field pulse, and investigated by the state selective field ionization method in a cesium standard magneto-optical trap. The dependences of the transfer rate, given by the ratio of the number of high-l Stark states to all atoms, on the strength and holding time of electric-field pulse are investigated and compared with those with additional ions. The results show that the time evolution of high-l Stark states strongly depends on the electric-field strength, and is affected by the additional ions at relatively weaker field (1.51 V/cm here). The density of Rydberg atoms has a minor effect on the characteristic time of evolution process.
In this paper, we investigate the Stark effect of ultra-cold 39D cesium Rydberg atoms in low-field. The Stark structure of 39D Rydberg states is calculated numerically. The cold cesium atoms are excited to Rydberg states via two-step process and the Stark spectra are obtained by field-ionization method. The scalar and tenson polarizabilities of 39D cesium Rydberg atoms are measured to be α5/22=62(7) MHz·V-2cm2，α5/20=－146(13) MHz·V-2cm2, α3/22=73(6) MHz·V-2cm2，α3/20=－106(20) MHz·V-2cm2 respectively. The experimental values are in agreement with the theoretical results.