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Acta Physica Polonica A

Fluorescence Spectra Study in Extremely Thin Cs-Vapor Layers

Kapka Vaseva, P. Todorov, Dimitar G. Slavov, S. Cartaleva, Kaloian Koynov, Solomon M. Saltiel

Published Nov 1, 2007• 0 citations
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Abstract

The high resolution spectroscopy of nanometric-thin alkali-vapor layers was made possible through the development of extremely thin cell.We have investigated the behavior of the extremely thin cell fluorescence spectra both experimentally and theoretically.Experiment is performed on the D 2 line of Cs-vapor-layer with thickness L = mλ, where m = 0.5, 0.75, 1, 1.25.For open optical transitions, the fluorescence spectra shows narrow dip on the top of the sub-Doppler-width fluorescence profile, at L ≥ λ.In case of closed transition, an extremely small feature in the fluorescence slightly shifted from its maximum is observed at L = (5/4)λ.The used theoretical model, based on the optical Bloch equations is in qualitative agreement with the experimental observations.

DOI
10.12693/aphyspola.112.865

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Physical Review A•Jun 25, 2004•110 citations
The high resolution spectroscopy of nanometric-thin alkali-vapor layers was made possible through the development of extremely thin cell.We have investigated the behavior of the extremely thin cell fluorescence spectra both experimentally and theoretically.Experiment is performed on the D 2 line of Cs-vapor-layer with thickness L = mλ, where m = 0.5, 0.75, 1, 1.25.For open optical transitions, the fluorescence spectra shows narrow dip on the top of the sub-Doppler-width fluorescence profile, at L ≥ λ.In case of closed transition, an extremely small feature in the fluorescence slightly shifted from its maximum is observed at L = (5/4)λ.The used theoretical model, based on the optical Bloch equations is in qualitative agreement with the experimental observations.
The high resolution spectroscopy of nanometric alkali-vapor layers has been made possible through the development of extremely thin cell.We present a detailed comparison of the fluorescence profiles amplitude and width, obtained in the extremely thin cell, both theoretically and experimentally.Experiments are performed on the D 2 line of Cs-vapor layer with thickness L = mλ, where m = 0.5, 0.75, 1, 1.25.The enhancement rate of the transition profiles width is not growing monotonously, but it is larger for L varying in the interval from L = 0.75λ to L = λ than that varying in the interval from L = λ to L = 1.25λ.The used theoretical model, based on the optical Bloch equations is in qualitative agreement with the experimental observations.
In this communication we report the first observation of a narrow, reduced fluorescence dip in the profile of the completely closed transition on the D2 line of 133Cs vapor, confined in Extremely Thin Cell with nanometric thickness. The theoretical modeling of the fluorescence based on the Optical Bloch Equation for two-level atomic system, shows that the narrow dip in the fluorescence could be attributed to a very small loss in the excitation process of the examined degenerate transition. While the population in the atomic system remains constant, the depolarization of the excited level can lead to some loss in the efficiency of the optical transition excitation. Under the conditions of our experiment, no dip in the fluorescence is registered for the cell thickness where a well pronounced Dicke peak in the absorption takes place. For the cells with nanometric thickness, the previous investigations demonstrate that the fluorescence profiles of optical transitions differ significantly from the absorption profiles. However, our experiment shows that some traces of the coherent Dicke process contributing to the absorption line still remain in the fluorescence, which is result of non-coherent processes.
The saturation behavior of absorption and fluorescence spectra on the D2 line of Cs is presented, demonstrating a significant difference between open and closed transitions. Cs vapor is confined in an extremely thin cell (ETC) with widely tunable thickness L=(0.5-3)λ, where λ is the light wavelength. In the saturation regime, the closed transition demonstrates enhanced absorption in a narrow spectral interval due to the Dicke effect, while the open one demonstrates only a velocity-selective dip in the absorption. The fluorescence of open transitions shows reduced fluorescence dips, enhancing their contrast with ETC thickness. The closed transition exhibits only a small plateau around the optical transition center. Applying two-level theoretical modeling based on optical Bloch equations, a qualitative agreement with experimental observations is achieved. The rate of contrast enhancement with cell thickness is larger for the theoretical than for the experimental dips. In addition, for the closed transition a tiny peak in the fluorescence is theoretically predicted, with the first experimental confirmation presented. The sub-Doppler spectra of vapor layers with a thickness of several light wavelengths show potential for realization of precise frequency references and photonics sensors.
Saturation effects affecting absorption and fluorescence spectra of an atomic vapor confined in an extremely thin cell (cell thickness $L<1\phantom{\rule{0.3em}{0ex}}\ensuremath{\mu}\mathrm{m}$) are investigated experimentally and theoretically. The study is performed on the D2{D}_{2}D2​ line $(\ensuremath{\lambda}=852\phantom{\rule{0.3em}{0ex}}\mathrm{nm})$ of Cs and concentrates on the two situations $L=\ensuremath{\lambda}∕2$ and $L=\ensuremath{\lambda}$, the most contrasted ones with respect to the length dependence of the coherent Dicke narrowing. For $L=\ensuremath{\lambda}∕2$, the Dicke-narrowed absorption profile simply broadens and saturates in amplitude when increasing the light intensity, while for $L=\ensuremath{\lambda}$, sub-Doppler dips of reduced absorption at the line-center appear on the broad absorption profile. For a fluorescence detection at $L=\ensuremath{\lambda}$, saturation induces narrow dips, but only for hyperfine components undergoing a population loss through optical pumping. These experimental results are interpreted with the help of the various existing models and are compared with numerical calculations based upon a two-level modeling that considers both a closed and an open system.
We present the first experimental observation of narrow dips in the fluorescence profiles of completely closed hyperfine transitions in Rb vapor at high atomic density, which is attributed to the depolarization of the excited state.Moreover, at low atomic density, a narrow peak on the top of the fluorescence profile is demonstrated, centered at the completely closed transition within the D2 line of Cs.Experiments are performed in thin (700 µm) alkali cell by single light beam spectroscopy.The cell is filled with Cs containing a small portion of Rb.
We compare the behavior of absorption and of resonance fluorescence spectra in an extremely thin Rb vapor cell as a function of the ratio of $L∕\ensuremath{\lambda}$, with LLL the cell thickness $(L\ensuremath{\sim}150--1800\phantom{\rule{0.3em}{0ex}}\mathrm{nm})$ and $\ensuremath{\lambda}$ the wavelength of the Rb D2{D}_{2}D2​ line $(\ensuremath{\lambda}=780\phantom{\rule{0.3em}{0ex}}\mathrm{mn})$. The Dicke-type coherent narrowing [G. Dutier et al., Europhys. Lett. 63, 35 (2003)] is observed only in transmission measurements, in the linear regime, with its typical collapse and revival, which reaches a maximum for $L=(2n+1)\ensuremath{\lambda}∕2$ (nnn integer). It is shown not to appear in fluorescence, whose behavior-amplitude, and spectral width, is more monotonic with LLL. Conversely, at high-intensity, the sub-Doppler saturation effects are shown to be the most visible in transmission around $L=n\ensuremath{\lambda}$.