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Chinese Optics Letters

Measurement of the wavelength modulation indices with selective reflection spectroscopy

Liantuan Xiao, Jianming Zhao, Wangbao Yin, Yanting Zhao, Bernard A. Journet, Journet, 贾锁堂

Published Jan 1, 2003• 2 citations
OpenAlex

Abstract

The wavelength modulation indices are measured based on harmonic amplitude ratio of 4f_(amp)/6f_(amp) (4f_(amp) and 6f_(amp) are the 4- and 6-th harmonic central peak amplitudes correspondingly) with the Doppler-free selective reflection modulation spectroscopy. The experiments for the 6S_(1/2)(F = 4) ? 6P_(3/2)(F' = 5) transition of cesium D_(2) line with 30-MHz linewidth were carried out. The 4f- and 6f-harmonic signals were detected with two digital lock-in amplifiers separately. The maximum error for modulation indices measurement was ±0.1 within the range of m from 3 to 6. The non-linear modulation behaviour of an external cavity diode laser induced by voltage tuning was studied with this method. The method for modulation indices measurement does not require a solid etalon as usual for measuring the wavelength modulation depth and the absorption linewidth correspondingly.

Related papers

Measurement of Modulation Index with High-order-harmonic Detection

Yin Wang

The modulation indexes have been measured by the harmonics intensity ratios (4f max /6f max ).By use of the numerical analysis,we get the relationship of the modulation index and high harmonics (4f,6f) detection.We also get 4f and 6f harmonic signals about the 6S 1/2 (F=4)→6P 3/2 transition of the cesium D 2 line using the voltage modulation.The experimental results are fairly agreement with theoretical analysis.This method is efficient for the measurements of the modulation depth and line width.

Journal of Optoelectronics·laser•Jan 1, 2002•0 citations

High-resolution Reflection Spectroscopy ofCs D_2 Line Studied byHigh-order-harmonic Detection

Jia Suo-Tang

In this paper, by numerical analysis the relationship of the modulation broaden index with modulation index using high-order-harmonic detection is investigated. Using the voltage modulation the 2f,4f and 6f harmonic signals about the reflection spectroscopy of 6S1/2(F = 4) →6P3/2 transition of the cesium D2 line are also be measured. The experimental results are in good agreement with the theoretical predictions. It is found that narrower line-width can be achieved by higher-harmonic detection than the line-width detected by direct absorption when the modulation index is smaller than 1.81, 2.98 and 4.14 for 2f, 4f, and 6f signals, respectively.

中国激光(英文版)•Jan 1, 2002•0 citations

Experimental investigation of the sub-Doppler transmission spectroscopy in a thin vapour layer at room temperature

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Electromagnetically induced transparency in modulated laser fields

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Abstract We study electromagnetically induced transparency (EIT) in a room-temperature cesium vapor cell using wavelength-modulated probe laser light. In the utilized cascade level scheme, the probe laser drives the lower transition 6 S 1 / 2 ( F = 4) → 6 P 3 / 2 ( F ’ = 5), while the coupling laser drives the Rydberg transition 6 P 3 / 2 → 57 S 1 / 2 . The probe laser has a fixed average frequency and is modulated at a frequency of a few kHz, with a variable modulation amplitude in the range of tens of MHz. The probe transmission is measured as a function of the detuning of the coupling laser from the Rydberg resonance. The first-harmonic demodulated EIT signal has two peaks that are, in the case of large modulation amplitude, separated by the peak-to-peak modulation amplitude of the probe laser times a scaling factor λ p / λ c , where λ p and λ c are the probe- and coupling-laser wavelengths. The scaling factor is due to Doppler shifts in the EIT geometry. Second-harmonic demodulated EIT signals, obtained with small modulation amplitudes, yield spectral lines that are much narrower than corresponding lines in the modulation-free EIT spectra. The resultant spectroscopic resolution enhancement is conducive to improved measurements of radio-frequency (RF) fields based on Rydberg-atom EIT, an approach in which the response of Rydberg atoms to RF fields is exploited to characterize RF fields. Here, we employ wavelength modulation spectroscopy to reduce the uncertainty of atom-based frequency and field measurement of an RF field in the VHF radio band.

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Frequency-modulation spectroscopy with blue diode lasers

Ulf P. Gustafsson, Gabriel Somesfalean, Jānis Alnis +1 more

Frequency-modulation spectroscopy provides ultrasensitive absorption measurements. The technique is especially adaptable to diode lasers, which can be modulated easily, and has been used extensively in the near-infrared and infrared spectral regions. The availability of blue diode lasers now means that the accessible wavelength region can be increased. We successfully demonstrate wavelength-modulation spectroscopy and two-tone frequency-modulation spectroscopy for the weak second resonance line of potassium at 404.8 nm and for the transition at 405.8 nm in lead, starting from the thermally populated 6(p)(2 3)P(2) metastable level. Information on the modulation parameters is obtained with a fitting procedure. Experimental signal-to-noise ratios at different absorption levels are compared with theoretical signal-to-noise ratios and show good agreement. Detection sensitivities of 2 x 10(-6) and 5 x 10(-6) for wavelength and two-tone frequency-modulation spectroscopy, respectively, for a 120-Hz bandwidth are demonstrated.

Applied Optics•Jul 20, 2000•29 citations
The wavelength modulation indices are measured based on harmonic amplitude ratio of 4f_(amp)/6f_(amp) (4f_(amp) and 6f_(amp) are the 4- and 6-th harmonic central peak amplitudes correspondingly) with the Doppler-free selective reflection modulation spectroscopy. The experiments for the 6S_(1/2)(F = 4) ? 6P_(3/2)(F' = 5) transition of cesium D_(2) line with 30-MHz linewidth were carried out. The 4f- and 6f-harmonic signals were detected with two digital lock-in amplifiers separately. The maximum error for modulation indices measurement was ±0.1 within the range of m from 3 to 6. The non-linear modulation behaviour of an external cavity diode laser induced by voltage tuning was studied with this method. The method for modulation indices measurement does not require a solid etalon as usual for measuring the wavelength modulation depth and the absorption linewidth correspondingly.
The modulation indexes have been measured by the harmonics intensity ratios (4f max /6f max ).By use of the numerical analysis,we get the relationship of the modulation index and high harmonics (4f,6f) detection.We also get 4f and 6f harmonic signals about the 6S 1/2 (F=4)→6P 3/2 transition of the cesium D 2 line using the voltage modulation.The experimental results are fairly agreement with theoretical analysis.This method is efficient for the measurements of the modulation depth and line width.
In this paper, by numerical analysis the relationship of the modulation broaden index with modulation index using high-order-harmonic detection is investigated. Using the voltage modulation the 2f,4f and 6f harmonic signals about the reflection spectroscopy of 6S1/2(F = 4) →6P3/2 transition of the cesium D2 line are also be measured. The experimental results are in good agreement with the theoretical predictions. It is found that narrower line-width can be achieved by higher-harmonic detection than the line-width detected by direct absorption when the modulation index is smaller than 1.81, 2.98 and 4.14 for 2f, 4f, and 6f signals, respectively.
Photon counting has been widely used in weak light even to single photon detection.However,the Shot noise of photon-counting N for Poisson statistics seriously affects the sensitivity.A method using wavelength modulation spectroscopy technique to improve signal-to-noise ratio of photon-counting is presented.The light from an external cavity diode laser is wavelength modulated and then chopped to a series of laser pulses by using a acoustic-optical modulator,the counts of fluorescence photon are recorded and then converted to an analog signal.The analog signal is added to a lock-in amplifier for harmonic demodulation using lock-in method.The fluorescence spectrum is the 6S_1/2(F=4)→6P_3/2 transition of Cs D_2 line and the detected probability of photon is 35%.The experimental demonstration has achieved a 51 dB signal-to-noise improvement factor in 2f harmonic detection.The minimum detectable count here is 3×10-4 with the residual noise 7.54 μV.The results show a potential application in fluorescence detection of cold molecules or single molecule.
Abstract We study electromagnetically induced transparency (EIT) in a room-temperature cesium vapor cell using wavelength-modulated probe laser light. In the utilized cascade level scheme, the probe laser drives the lower transition 6 S 1 / 2 ( F = 4) → 6 P 3 / 2 ( F ’ = 5), while the coupling laser drives the Rydberg transition 6 P 3 / 2 → 57 S 1 / 2 . The probe laser has a fixed average frequency and is modulated at a frequency of a few kHz, with a variable modulation amplitude in the range of tens of MHz. The probe transmission is measured as a function of the detuning of the coupling laser from the Rydberg resonance. The first-harmonic demodulated EIT signal has two peaks that are, in the case of large modulation amplitude, separated by the peak-to-peak modulation amplitude of the probe laser times a scaling factor λ p / λ c , where λ p and λ c are the probe- and coupling-laser wavelengths. The scaling factor is due to Doppler shifts in the EIT geometry. Second-harmonic demodulated EIT signals, obtained with small modulation amplitudes, yield spectral lines that are much narrower than corresponding lines in the modulation-free EIT spectra. The resultant spectroscopic resolution enhancement is conducive to improved measurements of radio-frequency (RF) fields based on Rydberg-atom EIT, an approach in which the response of Rydberg atoms to RF fields is exploited to characterize RF fields. Here, we employ wavelength modulation spectroscopy to reduce the uncertainty of atom-based frequency and field measurement of an RF field in the VHF radio band.
Frequency-modulation spectroscopy provides ultrasensitive absorption measurements. The technique is especially adaptable to diode lasers, which can be modulated easily, and has been used extensively in the near-infrared and infrared spectral regions. The availability of blue diode lasers now means that the accessible wavelength region can be increased. We successfully demonstrate wavelength-modulation spectroscopy and two-tone frequency-modulation spectroscopy for the weak second resonance line of potassium at 404.8 nm and for the transition at 405.8 nm in lead, starting from the thermally populated 6(p)(2 3)P(2) metastable level. Information on the modulation parameters is obtained with a fitting procedure. Experimental signal-to-noise ratios at different absorption levels are compared with theoretical signal-to-noise ratios and show good agreement. Detection sensitivities of 2 x 10(-6) and 5 x 10(-6) for wavelength and two-tone frequency-modulation spectroscopy, respectively, for a 120-Hz bandwidth are demonstrated.