The recent discovery of efficient quantum algorithms for factoring and database search has shown that quantum computing would allow to solve important problems which are intractable with conventional computers. In contrast to the very demanding task of building a large-scale quantum computer, there are quantum communication protocols, e.g. quantum key distribution for cryptography, which—though still difficult—require much less effort and can be implemented with current technology. Apart from the technological motivation, the study of quantum information offers (at least) two additional benefits. First, new insight into fundamental questions on quantum mechanics, e.g. concerning non-locality and entanglement, are gained from an information-theoretical approach. And second, investigating a particular physical implementation of quantum information can give rise to independent physical results. Spintronics, the use of spin as opposed to charge in (classical) electronics is a new field for which some results presented here could be relevant. In this dissertation we investigate several theoretical aspects of the physical implementation of quantum computation and communication in which the fundamental unit of quantum information, the qubit, is represented by the spin of electrons in semiconductor quantum dots. The required coupling between the spins can be obtained by allowing for tunneling of electrons between adjacent dots, leading to a Heisenberg exchange coupling J S1 · S2 between the spins, a scenario which we study for laterally coupled quantum dots in a two-dimensional electron system, and for a three-dimensional setup with vertically coupled quantum dots. Furthermore, an alternative scheme to couple the spins via the interaction with an optical cavity mode is presented. Quantum error correction represents one of the important ingredients for the physical implementation of a quantum computer by protecting \nit from the e�ects of a noisy environment. As a �rst test for errorcorrection \nin a solid-state device using spins, we propose an optimized \nimplementation of the most primitive error correction scheme (the threebit \ncode). In this context, we introduce parallel switching, allowing \nto operate a quantum computer more e�ciently than the usual serial \nswitching. \nCoupling spins with the exchange interaction J S1 �S2 is not su�cient \nfor quantum computation; the spins also have to be addressed individually \nusing controllable local magnetic �elds or g-factors giBi �Si in order \nto allow for single-qubit operations. On the one hand, we discuss several \nschemes for overcoming the di�culty of applying local magnetic �elds \n(requiring large gradients), e.g. g-factor engineering, which allows for \nall-electric operation of the device. On the other hand, we show that \nat the expense of additional devices (spins) and switching operations, \nsingle-spin rotations can be dispensed with completely. \nAddressing the feasibility of quantum communication with entangled \nelectrons in mesoscopic wires, i.e. interacting many-body environments, \nwe propose an interference experiment using a scattering set-up with an \nentangler and a beam splitter. The current noise for electronic singlet \nstates turns out to be enhanced (bunching), while it is reduced for triplets \n(antibunching). Due to interactions, the �delity of the entangled singlet \nand triplet states is reduced by z4F \nin a conductor described by Fermi \nliquid theory, zF being the quasiparticle weight factor. \nFinally, we study the related but more general problem of the noise of \nthe cotunneling current through one or several tunnel-coupled quantum \ndots in the Coulomb blockade regime. The various regimes of weak and \nstrong, elastic and inelastic cotunneling are analyzed for quantum-dot \nsystems (QDS) with few-level, nearly-degenerate, and continuous electronic \nspectra. In contrast to sequential tunneling, the noise in inelastic \ncotunneling can be super-Poissonian. In order to investigate strong cotunneling \nwe develop a microscopic theory of cotunneling based on the \ndensity-operator formalism and using the projection operator technique. \nWe have derived the master equation for the QDS and the current and \nnoise in cotunneling in terms of the stationary state of the QDS. These \nresults are then applied to QDS with a nearly degenerate and continuous \nspectrum.
The recent discovery of efficient quantum algorithms for factoring and database search has shown that quantum computing would allow to solve important problems which are intractable with conventional computers. In contrast to the very demanding task of building a large-scale quantum computer, there are quantum communication protocols, e.g. quantum key distribution for cryptography, which—though still difficult—require much less effort and can be implemented with current technology. Apart from the technological motivation, the study of quantum information offers (at least) two additional benefits. First, new insight into fundamental questions on quantum mechanics, e.g. concerning non-locality and entanglement, are gained from an information-theoretical approach. And second, investigating a particular physical implementation of quantum information can give rise to independent physical results. Spintronics, the use of spin as opposed to charge in (classical) electronics is a new field for which some results presented here could be relevant. In this dissertation we investigate several theoretical aspects of the physical implementation of quantum computation and communication in which the fundamental unit of quantum information, the qubit, is represented by the spin of electrons in semiconductor quantum dots. The required coupling between the spins can be obtained by allowing for tunneling of electrons between adjacent dots, leading to a Heisenberg exchange coupling J S1 · S2 between the spins, a scenario which we study for laterally coupled quantum dots in a two-dimensional electron system, and for a three-dimensional setup with vertically coupled quantum dots. Furthermore, an alternative scheme to couple the spins via the interaction with an optical cavity mode is presented. Quantum error correction represents one of the important ingredients for the physical implementation of a quantum computer by protecting \nit from the e�ects of a noisy environment. As a �rst test for errorcorrection \nin a solid-state device using spins, we propose an optimized \nimplementation of the most primitive error correction scheme (the threebit \ncode). In this context, we introduce parallel switching, allowing \nto operate a quantum computer more e�ciently than the usual serial \nswitching. \nCoupling spins with the exchange interaction J S1 �S2 is not su�cient \nfor quantum computation; the spins also have to be addressed individually \nusing controllable local magnetic �elds or g-factors giBi �Si in order \nto allow for single-qubit operations. On the one hand, we discuss several \nschemes for overcoming the di�culty of applying local magnetic �elds \n(requiring large gradients), e.g. g-factor engineering, which allows for \nall-electric operation of the device. On the other hand, we show that \nat the expense of additional devices (spins) and switching operations, \nsingle-spin rotations can be dispensed with completely. \nAddressing the feasibility of quantum communication with entangled \nelectrons in mesoscopic wires, i.e. interacting many-body environments, \nwe propose an interference experiment using a scattering set-up with an \nentangler and a beam splitter. The current noise for electronic singlet \nstates turns out to be enhanced (bunching), while it is reduced for triplets \n(antibunching). Due to interactions, the �delity of the entangled singlet \nand triplet states is reduced by z4F \nin a conductor described by Fermi \nliquid theory, zF being the quasiparticle weight factor. \nFinally, we study the related but more general problem of the noise of \nthe cotunneling current through one or several tunnel-coupled quantum \ndots in the Coulomb blockade regime. The various regimes of weak and \nstrong, elastic and inelastic cotunneling are analyzed for quantum-dot \nsystems (QDS) with few-level, nearly-degenerate, and continuous electronic \nspectra. In contrast to sequential tunneling, the noise in inelastic \ncotunneling can be super-Poissonian. In order to investigate strong cotunneling \nwe develop a microscopic theory of cotunneling based on the \ndensity-operator formalism and using the projection operator technique. \nWe have derived the master equation for the QDS and the current and \nnoise in cotunneling in terms of the stationary state of the QDS. These \nresults are then applied to QDS with a nearly degenerate and continuous \nspectrum.
Quantum information processing in semiconductor quantum dots using single and multi-spin qubitsThe idea of a quantum computer, a device capable of processing information using quantum bits (qubit) instead of classical bits that outperforms classical computer in terms of computation speed, is still science ction. However, recent advances in quantum information processing showed that this ction may come true faster than anticipated. A promising platform for the physical realization of a qubit are spin qubits where the information is encoded in the quantum mechanical spin of an electron con ned in a semiconductor quantum dot. There are a variety of di erent implementations how the logical qubit is physically encoded, the use of a single electron spin or the use of the spins of multi electrons. This thesis focuses on the implementation of the spin- 1/2 qubit using the spin of a single electron in a single quantum dot, the exchangeonly (EO) qubit using three electron spins distributed in three quantum dots, and the novel quadrupolar exchange-only (QUEX) qubit using four electron spins distributed in three quantum dots. In this thesis we investigate several theoretical aspects of the physical implementation of the aforementioned qubit encodings. Since all three qubit encodings are allelectric controlled these implementations su er decoherence, the loss of information, from electric uctuations of the environment commonly called charge noise. Typically, the use of more quantum dots increases the decoherence due to charge noise while it decreases the decoherence due to magnetic noise. The rst main aspect investigated in this thesis is the protection of the quantum information encoded in the di erent qubit implementations against charge noise. Special attention is paid to the multi-electron spin implementations where high-symmetry points of operation are discovered which are less sensitive to the charge noise. Protection against charge noise is even better by increasing the number of electrons while keeping the number of quantum dots making the QUEX qubit superior to the EO qubit. So far the main direction in this thesis is the reduction of the qubit sensitivity to electric uctuations. However, coherent electromagnetic elds in form of microwaves v can be used to interconnect qubits. In this thesis also a high-performance coupling between two spin-1/2 is investigated. The use of a resonator, subsequently, allows for a coupling of qubits over macroscopic distances as well as to extract valuable information about the physical system. Because of the larger susceptibility of multi-spin qubits to the electric eld of the resonator, this thesis focuses on the coupling between an EO or a QUEX qubit and a microwave resonator. Points of operations are discovered for both qubit implementations which o er a strong coupling towards a microwave resonator while maintaining their protection against charge noise. Subsequently, a series of measurements are proposed to extract information about the microscopic structure of the quantum dots. Finally, a promising high-performance protocol for coupling two qubits remotely via the resonator is investigated in detail.
A two-level quantum system is the building block of a quantum computer. This pair of quantum states defines the computational unit of a quantum computer, and it is called a quantum bit or qubit in analogy to the bit that is the binary unit of a classical computer. The spin of a single electron naturally defines such a two-level quantum system. A quantum dot can be tuned to the single-electron regime, and an array of singly occupied quantum dots provides a multi-qubit register. This thesis describes the multielectron encoding of a spin qubit using a pair or a trio of quantum dots, and it analyzes the coherence properties and manipulation protocols of this system. The singlet-triplet qubit, coded using the singlet state and the spinless triplet state of a pair of singly occupied quantum dots, can be controlled all electrically when applying voltages to gates close to the quantum dot structure. Rapid, subnanosecond modifications of the double quantum dot's charge configuration have been realized successfully. A small magnetic field gradient across the double quantum dot enables universal qubit control. Two modifications of the normal singlet-triplet encoding are introduced. (1) The six-electron configuration of a double quantum dot encodes a singlet-triplet qubit in the same way as for the two-electron double quantum dot. Two electrons at each quantum dot are irrelevant for the qubit manipulations because they are paired in a singlet state; the remaining two electrons encode the qubit. The qubit's wave function is immune to charge noise at moderate out-of-plane magnetic fields. (2) A singlet-triplet qubit encoded using two quantum dots of different sizes has an orbital state degeneracy of the singlet state and the spinless triplet state at finite out-of-plane magnetic fields. Spin-orbit interactions lift this state degeneracy, while the magnitude of the state coupling is determined by the size difference of the QDs. This setup enables the manipulations of singlet-triplet qubits without the need for magnetic field gradients. Finally, two-qubit gates between singlet-triplet qubits are proposed that use mediated exchange interactions via one quantum state. These operations are well controlled and highly noise insensitive. Orbital interactions alone can control spin qubits coded in a three electron Hilbert space. For example, the exchange-only qubit is encoded using three singly occupied quantum dots. The exchange interactions of two quantum dot pairs need to be modified to manipulate this qubit. The noise sensitivity of the exchange-only qubit is discussed. Alternatively, a three-electron qubit at a double quantum dot can be operated when single electrons are transferred between the quantum dots. Fast, subnanosecond manipulations of the double quantum dot's charge configuration are required to realize single-qubit gates. A novel two-qubit pulse gate for the three-electron double quantum dot qubit is proposed.
If the states of spins in solids can be created, manipulated, and measured at the single-quantum level, an entirely new form of information processing, quantum computing and quantum communication, will be possible. We review our proposed spin-quantum dot architecture for a quantum computer and review some recent results on a deterministic source of entanglement generated by coupling quantum dots. Addressing the feasibility of quantum communication with entangled electrons we consider a scattering set-up with an entangler and beam splitter where the current noise exhibits bunching behavior for electronic singlet states and antibunching behavior for triplet states. We show that spin currents can produce noise even in the absence of any charge currents.
This thesis addresses the concept of quantum computing with semiconductor quantum dots. The basic unit of a quantum computer is a quantum mechanical two-level system, the so-called quantum bit (qubit). The qubit can be defined as the spin of an electron confined in a quantum dot or as a two-dimensional subspace of the Hilbert space for several spins. Some semiconductors have several minima in their conduction band, socalled valleys. A two-dimensional valley degree of freedom can also be considered as a qubit. In this thesis, quantum registers storing spin as well as valley qubits are described theoretically. Virtual hopping yields an exchange interaction between neighboring quantum dots, which reduces the energy of antisymmetric spin-valley states according to the Pauli principle. Considering the spin and the valley degrees of freedom of two electrons in neighboring quantum dots as qubits, the exchange interaction is a four-qubit interaction. In this thesis, it will be shown that it is, nevertheless, possible to generate a universal two-qubit gate for spin qubits or for valley qubits by combining the exchange interaction and individual single-qubit gates. The exchange interaction in this two-electron double quantum dot directly provides a universal two-qubit gate for one spin and one valley qubit as well. For this, the qubits are defined as suitable subspaces, spanned by the singlet and one triplet state of the spin and the valley states, respectively, Using those gates, arbitrary quantum operations can be performed for single-spin and single-valley qubits in the same quantum register, where in one double quantum dot the quantum states are restricted to the singlet-triplet subspace. While in this register single-spin and single-valley rotations are required, these gates are dispensable in a quantum register storing spin and valley singlet-triplet qubits. The single-qubit operations, in this case, can be provided by the exchange interaction and a gradient in the energy splitting of spin and valley states when the spin qubit is stored in a double quantum dot with spin degrees of freedom only and when the spin states in the double quantum dot which stores the valley qubit are polarized. For providing the two-qubit gate, the spin and the valley qubits need to be stored in the same double quantum dot. The crucial task for this register is to interchange the spin of a spin-only and a spin-valley quantum dot in order to switch between the single-qubit and the two-qubit operation mode. This interchanging of the spin can be achieved by a valley-depending virtual hopping between the quantum dots. Furthermore, echo sequences for a so-called exchange-only qubit are considered. An exchange-only qubit is defined as a subspace in a system of three electron spins in a triple quantum dot. An inhomogeneous magnetic field, which may be caused by nuclear spins in the semiconductor, can lead to decoherence and leakage, i.e., the state might leave the qubit subspace. Suppressing this effect by an echo sequence which consists of pulses interchanging neighboring spin states, so-called SWAP gates, was proposed. Controllability over these quantum operations is provided via the exchange interaction. In this thesis, the performance of different such sequences is investigated. The analysis shows that optimization strategies developed for single spin echoes can be adapted for the three spin system. The echo sequences can be different in their order of applied SWAP gates interchanging the spins in the first and second dots or in the second and third dots. The noise suppression performance depends slightly on this order of SWAP gates. For two spins in a double quantum dot a scheme for quantum state tomography is presented. The corresponding measurement operators are constructed from a set of mutually unbiased bases of the four-dimensional two-qubit Hilbert space. These measurements are represented by short sequences of no more than three elementary quantum gates and projective measurements by the well-established spin-to-charge conversion.
Quantum physics describes the universe on a microscopic scale. Even though this scale is not accessible without complex experimental setups, quantum effects are respon- sible for the properties of matter and in some instances we have learned to exploit them technologically. A modern computer constituted of transistors passively utilizes the quantum nature of charge carriers in the band structure of semiconductors to encode and process information. Although such a classical computer is a formidable tool already, what could be achieved with active control over the quantum states in the computer is an intriguing question. This is the idea of the quantum computer, which offers an entirely new paradigm of computing by encoding information in quantum binary digits (qubits). Indeed, for several applications it has been shown that a quantum computer is superior to its classical counterpart, even though its realization remains elusive up to date. One candidate to host qubits are gate-defined semiconductor quantum dots, confin- ing single or few charge carriers with spin. The spin of a single confined electron is a quantum two-level system which can be manipulated and measured, allowing the storage and processing of quantum information. This thesis can be viewed as part of the endeavor to give birth to quantum computers based on semiconductor spin qubits. It primarily focuses on the challenge to enable scalable architectures of well-characterized qubits. In the first part, spin shuttling is investigated. This denotes the coherent transport of a single spin between spatially separate nodes of a quantum processor, driven by a time-dependent electric potential. The object of study is a minimal version of a bucket- brigade-like spin shuttling between two quantum dots. The probability of maintaining the spin state is identified as figure of merit and the effect of spin-orbit interaction and the Zeeman effect in an inhomogeneous magnetic field is explored with analytical and numerical methods. Special attention is paid to the repercussions of near-degenerate valleys. The second part of the thesis addresses the challenge to probe the microscopic properties of a quantum dot array, which is a crucial first step before any quantum operation can be performed. The transmission of a microwave resonator coupled to a triple quantum dot occupied by two electrons is investigated, and a scheme to infer the exchange interaction between electrons in adjacent quantum dots is proposed. By means of analytical derivations it is shown that the transmission profile of the resonator directly reveals the value of the exchange coupling strength between two electrons. This holds even if magnetic gradients or a valley splitting comparable to the inter-dot tunnel coupling are included. Subsequently, quantum transport measurements in the Pauli blockade regime are modelled in the presence of a microwave resonator, bringing together two powerful techniques to probe quantum dots. Based on generalized input-output theory, a theoretical framework is derived to investigate how a double quantum dot in a transport setup interacts with a coupled microwave resonator while the current through the double qauntum dot is rectified by Pauli blockade. It is shown that the output field of the resonator can be used to infer the leakage current and thus obtain insight into the blockade mechanisms and to estimate a large number of parameters of the quantum dots. Furthermore, the back-action of the resonator photons on the steady state leakage current is described and quantified. In the context of Pauli blockade, the spin and valley physics of bilayer graphene quantum dots in the few-electron regime is touched upon, describing a situation where spin blockade is observed despite the presence of the valleys. In the final part of the thesis, the attention is shifted towards the readout of the spin qubits. A new paradigm of dispersive readout is devised, which is performed while the qubit dephases, implementing a measurement in the x-basis. Laplace transforming the time dependent cavity response allows a separation of contributions from multiple qubits coupled to the same resonator. Thus, they can be read out simultaneously in a single shot. Modelling silicon spin qubits, as an example, results in in a readout time that compares favourably to conventional dispersive readout with comparable fidelity, even for a single qubit. With an auxiliary qubit the readout scheme can be extended to a quantum non-demolition measurement.
Quantum error-correcting codes have been developed to protect a quantum computer from decoherence due to a noisy environment. In this paper, we present two methods for optimizing the physical implementation of such error correction schemes. First, we discuss an optimal quantum circuit implementation of the smallest error-correcting code (the three bit code). Quantum circuits are physically implemented by serial pulses, i.e., by switching on and off external parameters in the Hamiltonian one after another. In contrast to this, we introduce a parallel switching method which allows faster gate operation by switching all external parameters simultaneously, and which has potential applications for arbitrary quantum computer architectures. We apply both serial and parallel switching to electron spins in coupled quantum dots subject to a Heisenberg coupling $H=J(t){\mathbf{S}}_{1}\ensuremath{\cdot}{\mathbf{S}}_{2}.$ We provide a list of steps that can be implemented experimentally and used as a test for the functionality of quantum error correction.