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Chinese Optics Letters

Study on three level system population transfer

杨山, 旷冶

Published Jan 1, 2003• 1 citation
OpenAlex

Abstract

Stimulated-Raman-adiabatic-passage (STIRAP) process provides an effective technique to transfer electronpopulation from an initial state (e.g. ground state) to excited final state for both atoms and molecules. Inthis paper, we present the results of the study on electron population transfer in three level system. Wehave analyzed the effects of various conditions on the transfer process, such as the time delay of the twolaser beams, two-photon off-resonance, one-photon off-resonance and the change of relative laser intensity.The numerical result is compared with experiment, and the reasons for the effects are also given.

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Stimulated-Raman-adiabatic-passage (STIRAP) process provides an effective technique to transfer electronpopulation from an initial state (e.g. ground state) to excited final state for both atoms and molecules. Inthis paper, we present the results of the study on electron population transfer in three level system. Wehave analyzed the effects of various conditions on the transfer process, such as the time delay of the twolaser beams, two-photon off-resonance, one-photon off-resonance and the change of relative laser intensity.The numerical result is compared with experiment, and the reasons for the effects are also given.
It is possible to prepare atoms or molecules in a selected excited state, one efficient way is to transfer population by stimulated-Raman-adiabatic-passage, but must understand off-resonant effects in coherent excitation in order to improve the efficient of transfer. Here, consider the transfer of population in a three-level system of stimulated-Raman- adiabatic-passage with computer analysis. The transfer efficiency of two-photon resonant is worked out and the outcome demonstrates the possibility of complete transfer. Also analysis the effect of two-photon off-resonant, single-photon off-resonant and difference of laser's intension.
Abstract The population transfer of a NaH molecule from the ground state X 1 Σ + to the target state A 1 Σ + via stimulated Raman adiabatic passage (STIRAP) is investigated. The results show that the intensity, delay time and detuning have a significant effect on population transfer. A large population transfer is observed with increased pump and Stokes intensity, especially when the pump and Stokes intensity match. Population transfer also depends on the delay time between the pump laser pulse and the Stokes laser pulse. The detuning of the two pulses influences the population transfer. Efficient population transfer can be realized under the resonant or two-photon resonant condition.
It introduced several methods to transfer population,including two-level system and three-level system, and gave some comparisons on transfer efficiency and transfer velocity of them in theory. It is shown that population transfer by coherent pulse sequence is better than incoherence one. Numerical simulation results showed that when using Stimulated Raman Adiabatic Rapid Passage (STIRAP), in which the pump laser pulse fully overlaps the Stokes pulse with the Stokes preceding the pump, population can be transferred completely and rapidly. Robust control of population transfer among Zeeman sublevels in the ground states of three-level system is investigated using adiabatic rapid passage in theory. The laser pulse widths are supposed to be short compared to the lifetime of the excited level, which means adiabatic. We demonstrated that techniques of STIRAP can be found to optimize population transfer in the ground states of three-level Λ system.
Stimulated Raman scattering involving adiabatic passage (STIRAP) is a proven technique for population transfer in three-level systems with strong oscillator strengths. We show that the STIRAP process should also yield high transfer efficiencies when the densities of states near the intermediate and final levels are high, provided certain criteria for the experimentally controllable parameters are met. We also show that high transfer efficiencies may even be possible when the pump and Stokes lasers can access levels outside of the three-level system. The criteria are derived with an approach that emphasizes the adiabatic nature of the transfer process in an eigenvector of the interaction Hamiltonian that resembles a trapped state. The results are compared to density matrix calculations.
The technique of stimulated Raman adiabatic passage (STIRAP) is used to transfer potassium atoms from the 22p state to the 21p Rydberg state through the intermediate state 22s. The results show that complete population transfer is related to pulse duration and overlap, and occurs when the pulse duration and overlap have adequate values. At the same time, population trapping is also formed. Complete population transfer can also occurs when the two-photon resonance condition ( Δ s = Δ p ) is met.
We consider a five-level atomic system (M-system) driven by four near-resonant laser pulses and study the possibilities of population transfer via different combinations of Stimulated Raman Adiabatic Passage (STIRAP) and bright-STIRAP (b-STIRAP) processes. We examine these combinations analytically and numerically from the point of view of efficiency of population transfer. It is shown, in particular, that the combination of the processes above enhances the efficiency. Analytical expressions are obtained for the quasienergies of the system in two regimes differing by conditions imposed on resonance detunings. Interaction adiabaticity conditions are analyzed. We also study the necessary successions of turning on and off of pulses which ensure efficient transfer of atomic populations. The obtained analytical results agree well with direct numerical calculations.