In this thesis, we show how an optical microcavity setup can create multiparticle entanglement in an ensemble of neutral atoms by means of quantum Zeno dynamics (QZD).Our setup combines an atom chip with a fibre Fabry-Perot (FFP) resonator and allows us to load an ensemble of Rb87 atoms into a single node of an intracavity dipole trap, coupling the atoms strongly and identically to the cavity light field which enables us to perform a quantum non-destructive measurement of their collective state.We realise QZD by modifying the dynamics of the collective state (encoded in atomic hyperfine states addressed with MW radiation) by means of frequent cavity measurements at optical frequency. This QZD is shown to create multiparticle entanglement in a fast and deterministic scheme. To analyse the created states, we reconstruct the symmetric part of the atomic density matrix from 2d measurements of the ensemble's Husimi Q-distribution. We give a time-resolved account of the creation of states with at least 3-11 entangled atoms and fidelity of up to 0.37 with respect to a W state of 36 atoms. Studying the influence of measurement strength and experimental imperfections, we show that our experiments are well described by simple models with no free parameters.This thesis also presents work towards improved FFP cavities. We discuss the problem of frequency splitting of polarisation eigenmodes in cavities made from two fibres microfabricated with a CO2 laser. We show that this effect depends on the symmetry of the microfabricated structures and demonstrate that it can be controlled both at the level of fabrication and when assembling a cavity.
In this thesis, we show how an optical microcavity setup can create multiparticle entanglement in an ensemble of neutral atoms by means of quantum Zeno dynamics (QZD).Our setup combines an atom chip with a fibre Fabry-Perot (FFP) resonator and allows us to load an ensemble of Rb87 atoms into a single node of an intracavity dipole trap, coupling the atoms strongly and identically to the cavity light field which enables us to perform a quantum non-destructive measurement of their collective state.We realise QZD by modifying the dynamics of the collective state (encoded in atomic hyperfine states addressed with MW radiation) by means of frequent cavity measurements at optical frequency. This QZD is shown to create multiparticle entanglement in a fast and deterministic scheme. To analyse the created states, we reconstruct the symmetric part of the atomic density matrix from 2d measurements of the ensemble's Husimi Q-distribution. We give a time-resolved account of the creation of states with at least 3-11 entangled atoms and fidelity of up to 0.37 with respect to a W state of 36 atoms. Studying the influence of measurement strength and experimental imperfections, we show that our experiments are well described by simple models with no free parameters.This thesis also presents work towards improved FFP cavities. We discuss the problem of frequency splitting of polarisation eigenmodes in cavities made from two fibres microfabricated with a CO2 laser. We show that this effect depends on the symmetry of the microfabricated structures and demonstrate that it can be controlled both at the level of fabrication and when assembling a cavity.
A major focus in modern experimental quantum physics is to create many-particle entangled states with single-particle control. In this Thesis we present a new platform that aims at achieving this purpose by combining two main ingredients: the collective coupling of cold rubidium atoms to an optical cavity and the individual control of the particles via a highresolution microscope. At the heart of our experimental system is a miniaturized fiber Fabry-Perot cavity that allows accessing the strong coupling regime of Cavity Quantum Electrodynamics (CQED). In addition to the CQED probe, a second cavity mode with twice the wavelength creates a lattice potential for identically and maximally coupling the atoms to the cavity. The spatial overlap between the two intra-cavity standing waves plays an essential role and we present methods to characterize and optimize it. We also report a technique for integrating the fiber cavity with a high-numerical aperture objective in a compact and stable setup. For transporting cold atoms from the capture region to the fiber resonator, we developed a system based on a movable optical dipole trap, driven by an acousto-optical deflector, which realizes a fast and efficient loading of the intracavity lattice. The combination of these elements allowed the observation of strong coupling between the cavity mode and the atoms in the 1D lattice via vacuum-Rabi-splitting measurements. This constitutes an important step towards generating many-body entanglement in our system, where the interplay between collective operations (performed via the cavity) and local control on the atomic qubits (provided by the microscope) is a promising approach for new entanglement schemes.
Multiparticle entangled quantum states, a key resource in quantum-enhanced metrology and computing, are usually generated by coherent operations exclusively. However, unusual forms of quantum dynamics can be obtained when environment coupling is used as part of the state generation. In this work, we used quantum Zeno dynamics (QZD), based on nondestructive measurement with an optical microcavity, to deterministically generate different multiparticle entangled states in an ensemble of 36 qubit atoms in less than 5 microseconds. We characterized the resulting states by performing quantum tomography, yielding a time-resolved account of the entanglement generation. In addition, we studied the dependence of quantum states on measurement strength and quantified the depth of entanglement. Our results show that QZD is a versatile tool for fast and deterministic entanglement generation in quantum engineering applications.
One of the most exciting prospects of quantum physics today is to simulate large quantum systems, intractable by classical computation, by connecting many smaller systems together. A cavity-based quantum network of atoms and photons constitutes one such approach, where each cavity interfaces between stationary atomic qubits in a node and photonic qubits travelling along optical fibre channels. For this scheme to work well, the cavity-based interface must be faithful and well-controlled. In this thesis, we construct a fibre-tip Fabry-Pérot cavity by aligning two optical fibre-tips against each other, where each has a concave, mirror-coated surface. Three properties make it highly suitable for interfacing: a small mode volume for strong atom-photon coupling, directly fibre-coupled cavity light, and optical access for trapped atoms. For the latter, we design a scheme that allows for a 2D reconfigurable array of atoms, held in the cavity mode by holographically-generated optical tweezers. Our particular design will allow us to move atoms independently of one another. We find the atom-cavity system parameters for optimal single photon generation, absorption and remote state transfer using V-STIRAP (vacuum-stimulated emission by Raman adiabatic passage). Using master equations and the Nelder-Mead algorithm, we optimise both the parameters and V-STIRAP pulse shapes to do this. We assemble the first fibre cavity formed of two single-mode fibres in ultra-high vacuum. Aligning two single-mode fibres is particularly demanding; we overcome this with an assembly method that gives permanent sub-micron alignment precision, unlike other similar cavities that need realigning using a translation stage. We fully characterise the cavity's parameters, then test it by probabilistically loading atoms from a magneto-optical trap, measuring the Purcell-enhanced fluorescence from the cavity. Altogether, our advances facilitate deterministically controlled, strongly-coupled and networked quantum systems.
A system comprised of a small number of neutral atoms coupled to the mode of a high finesse optical resonator is a model system to study light-matter interaction at the quantum level and to explore fundamental effects like the influence of the measurement process on the atomic state. Promising proposals to generate entangled states in such systems are based on the simultaneous coupling of two atoms to one resonator mode. In chapter 1 of this thesis I shortly summarise the experimental tools to capture, trap, and transport single atoms using a magneto-optical trap and an optical conveyor belt. I discuss theoretical foundations to describe our system and present numerical simulations, the results of which enter the analysis of our experimental data. The average atom-cavity coupling strength is deduced from the measured cavity transmission and compared to a model taking atomic motion into account. The dynamics of the hyperfine spin state of one and two coupled atoms is the focus of chapter 2. I describe a nondestructive cavity-based state detection method, quantify the state detection fidelity, and identify optimum experimental parameters. This method is then used to record random telegraph signals, exhibiting quantum jumps on a timescale of milliseconds. Telegraph signals for two atoms are analysed employing Bayesian statistics, yielding additional information on the evolution of the hyperfine states. A good localisation of the atom is necessary to achieve stable coupling to the cavity mode. In chapter 3, I discuss two different aspects of how the motion of the atom can be controlled. Firstly an intracavity dipole trap is characterised and it is shown that it results in improved confinement of the atom. Secondly I examine the dependence of cavity-cooling forces on our experimental parameters and compare two different cooling regimes.
Generating and manipulating multiparticle quantum entangled states is an exciting challenge of modern physics. Along this line, we have built a platform where cold rubidium atoms are strongly coupled to a fiber-based microcavity, under a quantum gas microscope. The atoms are trapped in a lattice at 1560nm, which allows strong and homogeneous coupling to the commensurate probe lattice at 780nm. First, we observe a coherent interaction between the cavity and the atoms, in the strong coupling regime, in spite of a large frequency inhomogeneity induced by the trap. It is the first report of such cavity protection effect with less than 200 emitters. We measure the growing coupling of the dark states to the cavity as the disorder takes over the collective coupling. In the protected regime we engineer frequency-modulated polaritons through a modulation of the atomic frequency. Then, we setup optical tweezers in the microcavity to obtain and manipulate several single atoms. The cavity enables fast and non demolition detection of a single atom in a tweezer. We measure the vacuum Rabi splitting of this atom, demonstrating its strong coupling with an effective cooperativity of 30. Finally, we obtain single atoms in a chain of 9 tweezers. This work opens to way to manipulating many individual atoms strongly coupled to the cavity, with applications in multiparameter quantum metrology, using spatially distributed and locally measurable entanglement as a resource, and quantum simulation of a chain of addressable spins with cavity-mediated infinite range interactions.
Strong atom-photon interactions in optical cavities are a key resource for quantum information processing, quantum networking, and the exploration of quantum optical effects. Optical tweezer arrays offer scalable, site-resolved control of neutral atoms, but their integration with high-cooperativity cavity QED systems remains challenging. Here we combine a twelve-site 87Rb optical tweezer array with a high-cooperativity fiber Fabry-Pérot microcavity. The array is positioned within the cavity mode and individual sites are controlled with subwavelength precision, enabling continuous tuning of the single-atom coupling strength via deterministic displacement through the standing-wave field. For up to five atoms coupled to the cavity, we measure collectively enhanced vacuum Rabi splitting and implement cavity-based non-destructive readout of the number of coupled atoms. These results establish a scalable architecture for cavity-mediated entanglement generation and many-body cavity QED with single-atom control, and they lay the foundation for fiber-integrated quantum network nodes.