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How to design, optimise and implement a fibre-tip Fabry-Pérot cavity for quantum networks of atoms and photons

Mohammed, Marwan

Published Jan 1, 2021• 0 citations
Publisher

Abstract

One of the most exciting prospects of quantum physics today is to simulate large quantum systems, intractable by classical computation, by connecting many smaller systems together. A cavity-based quantum network of atoms and photons constitutes one such approach, where each cavity interfaces between stationary atomic qubits in a node and photonic qubits travelling along optical fibre channels. For this scheme to work well, the cavity-based interface must be faithful and well-controlled. In this thesis, we construct a fibre-tip Fabry-Pérot cavity by aligning two optical fibre-tips against each other, where each has a concave, mirror-coated surface. Three properties make it highly suitable for interfacing: a small mode volume for strong atom-photon coupling, directly fibre-coupled cavity light, and optical access for trapped atoms. For the latter, we design a scheme that allows for a 2D reconfigurable array of atoms, held in the cavity mode by holographically-generated optical tweezers. Our particular design will allow us to move atoms independently of one another. We find the atom-cavity system parameters for optimal single photon generation, absorption and remote state transfer using V-STIRAP (vacuum-stimulated emission by Raman adiabatic passage). Using master equations and the Nelder-Mead algorithm, we optimise both the parameters and V-STIRAP pulse shapes to do this. We assemble the first fibre cavity formed of two single-mode fibres in ultra-high vacuum. Aligning two single-mode fibres is particularly demanding; we overcome this with an assembly method that gives permanent sub-micron alignment precision, unlike other similar cavities that need realigning using a translation stage. We fully characterise the cavity's parameters, then test it by probabilistically loading atoms from a magneto-optical trap, measuring the Purcell-enhanced fluorescence from the cavity. Altogether, our advances facilitate deterministically controlled, strongly-coupled and networked quantum systems.

DOI
10.5287/ora-eorydqzmo

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One of the most exciting prospects of quantum physics today is to simulate large quantum systems, intractable by classical computation, by connecting many smaller systems together. A cavity-based quantum network of atoms and photons constitutes one such approach, where each cavity interfaces between stationary atomic qubits in a node and photonic qubits travelling along optical fibre channels. For this scheme to work well, the cavity-based interface must be faithful and well-controlled. In this thesis, we construct a fibre-tip Fabry-Pérot cavity by aligning two optical fibre-tips against each other, where each has a concave, mirror-coated surface. Three properties make it highly suitable for interfacing: a small mode volume for strong atom-photon coupling, directly fibre-coupled cavity light, and optical access for trapped atoms. For the latter, we design a scheme that allows for a 2D reconfigurable array of atoms, held in the cavity mode by holographically-generated optical tweezers. Our particular design will allow us to move atoms independently of one another. We find the atom-cavity system parameters for optimal single photon generation, absorption and remote state transfer using V-STIRAP (vacuum-stimulated emission by Raman adiabatic passage). Using master equations and the Nelder-Mead algorithm, we optimise both the parameters and V-STIRAP pulse shapes to do this. We assemble the first fibre cavity formed of two single-mode fibres in ultra-high vacuum. Aligning two single-mode fibres is particularly demanding; we overcome this with an assembly method that gives permanent sub-micron alignment precision, unlike other similar cavities that need realigning using a translation stage. We fully characterise the cavity's parameters, then test it by probabilistically loading atoms from a magneto-optical trap, measuring the Purcell-enhanced fluorescence from the cavity. Altogether, our advances facilitate deterministically controlled, strongly-coupled and networked quantum systems.
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A leading strategy for the creation of a scalable quantum computer is through a networked architecture. This would comprise stationary nodes for quantum information processing and photonic channels for their communication and entanglement distribution. In this scheme a coherent interface between light and matter is a critical component, facilitating the deterministic and reversible transfer of quantum information between stationary and travelling qubits. This requirement may be fulfilled by a high finesse optical cavity, whose radiation field is strongly coupled to a trapped quantised emitter. Neutral atoms are an ideal species for the development of such a device, given their inherent compatibility with dielectric mirror surfaces. However, an outstanding challenge in building an elementary network of neutral atom-cavity systems is in establishing a single atom dipole trap within each cavity mode. This thesis presents the development of an open-access cavity suitable for single atom localisation, whilst maintaining strong atom-cavity coupling, {g0,κ,γ} = {11,2.1,3} × 2πMHz, and the efficient extraction of generated photons, η=0.5. We consider cavity design methodology, deriving a connection between the physical properties of the optical resonator and its intended role in the production of single photons. An experimental platform is developed for the creation of cavity mirrors by laser ablation, with a high degree of geometrical control. This is used to produce a set of pyramidal micro-mirrors, demonstrated to represent a favourable alternative to the widespread adoption of fibre-tip cavities. These pyramidal mirrors are shown to support multi-feature resonators, allowing several atom-cavity interfaces to be formed using a pair of substrates. By developing a novel procedure for mirror alignment, a hybrid mirror cavity is fabricated and integrated into an experimental architecture tailored for atomic trapping. Suitability of the cavity for future experimentation is demonstrated by frequency stabilisation to an atomic resonance of 87Rb.
Scalable quantum information processing requires efficient coupling between stationary qubits (trapped atoms, ions, NV centres, etc.) via “flying” single-photon qubits. Here we investigate the optimisation and integration of fibre-tip microcavities into radiofrequency ion traps to achieve (i) high-fidelity transfer of ion qubits onto single photons, (ii) low-loss coupling of cavity photons into single-mode optical fibre, and (iii) achieving conditions (i) and (ii) without disturbing the ion trap. Our cavities are fabricated by laser micro-machining the ends of optical fibres and subsequent coating with a thin dielectric mirror, giving rise to cavity mirrors with a Gaussian profile. These cavities allow for small mode volume and thus large ion-photon coupling fulfilling requirement (i), while simultaneously providing intrinsic coupling to optical fibres, requirement (ii), as long as mode matching between the cavity mode and the fibre mode can be achieved at the cavity mirror. Using a semi-analytical numerical method, we show that Gaussian-shaped mirrors can in fact be used to enhance ion-photon coupling beyond what is possible with more common spherical cavity mirrors. Ion traps are notoriously sensitive to the presence of dielectric materials such as cavity mirrors near the trap centre, preventing requirement (iii) from being achieved. We performed an extensive numerical study of five different common ion traps to find the optimum configurations for integrating fibre-tip cavities with minimised effects on the trapping potentials. We discuss these results and present simple and effective design rules for realising optimum ion-cavity based quantum networks.
This thesis describes the first experimentally achieved coupling of a single atomic ion to an optical fibre-cavity as well as the first photonic interaction between a single ion and a single semiconductor quantum dot. The newly developed apparatus stores a single Yb+ ion in a radio-frequency Paultrap. There the ion is overlapped in-situ with the field of a miniature Fabry-Perot cavity which is mounted on a 3D-translation stage. The key elements of the setup are the cavity mirrors which are microfabricated onto the front facets of optical fibres. The small size of these mirrors are ideal for integration with an electrode structure of similar dimensions. Moreover these cavities are intrinsically fibre coupled and thereby well suited for distributed networks based on photonic interaction. We focus in our studies of the cavity-ion interaction on the application of the cavity as a converter between atomic and photonic excitations. To this end, we investigate the probability of the ion to emit photons into the cavity mode and find that this rate exceeds the natural spontaneous emission rate of the transition. We confirm that the emitted light field consists of a stream of single photons by measuring the second order correlation function. Furthermore, when prepared in a single Zeeman state, the emission process correlates the polarisation of the photon with the spin state of the ion. Remarkably, swapping the roles of ion and light field does not affect the interaction strength, i.e. we observe strongly enhanced absorption by the ion when a faint probe beam is injected into the cavity mode. The novel cavity-ion geometry advances the prospects to reach the strong-coupling regime with single ions and the feasibility of a distributed ion-based quantum network. Finally we employ the cavity-enhanced absorption to demonstrate photonic coupling between an InAs/GaAs quantum dot and a Yb+ ion. The setups for both systems are spatially separated by 20 m and optically linked by a single mode fibre. Quantum dot photons are guided into the cavity and the absorption by the ion is investigated for various excitation parameters. Our results mark the first steps towards hybrid networks and set the stage for further studies of the interaction between this unequal couple.
In recent years there has been rapid progress into realising a working universal quantum computer, in particular with the development of chip-based radio frequency ion traps. The next significant leap will come with successfully integrating optical cavities into these ion traps to allow for interaction between remote ions via photons as required for more efficient and scalable quantum networking schemes. Fibre-tip cavities are especially interesting for such applications as they enable highly efficient coupling of photons from the cavity into optical fibres for onward transmission. Here we analyse theoretically and numerically the effects of parallel off-axial misalignment in millimetre scale optical Fabry-Perot cavities. While near-concentric cavity configurations produce the smallest mode waist and thus strongest coupling to a trapped ion, their mode is extremely sensitive to misalignment. Shorter cavities exhibit more robust modes, but at the cost of larger mode waists. For example, for typical experimental parameters (mirror radius of curvature 0.7 mm, mirror diameter 0.140 mm, operation wavelength 850 nm) we find that the cavity lifetime is reduced by a factor 1/e for a misalignment of 0.95 nm for a beam waist of 2.91 um (cavity length of 1.397 mm), which increases to 11.0 nm for a waist of 4.33 um (length of 1.386 mm), and 3.12 um for a waist of 7.38 um (length of 1.273 mm). In the parameter regimes of interest, we derive a simple relation between cavity length, mirror radius, and misalignment sensitivity. Finally, we also consider the effect of mode matching of the misaligned cavity mode with the optical mode of the fibre for efficient cavity to fibre coupling. In conclusion, our model allows us to optimise photon-ion coupling in fibre-tip resonators for quantum information processing in the presence of finite fabrication and alignment tolerances.
We investigate the coupling of a single trapped ion to a miniature optical cavity operating in the ultraviolet. Our cavity provides a source of single photons at a high rate into a single spatial mode. Using our apparatus, we have demonstrated the highest atom-cavity coupling rate achieved with a single ion by an order of magnitude. When the ion is continuously excited, we observe phase-sensitive correlations between emission into free-space and into the cavity mode, which can be explained by a cavity induced back-action effect on a driven dipole. We demonstrate coherent manipulation of a hyperfine qubit and ultra-short optical π\piπ rotations, which are essential tools for creation and detection of spin-photon entanglement. To this end, we have developed optical fibre-based Fabry-Perot cavities in the ultraviolet spectral range. These cavities operate near the primary dipole transition of Yb at 370 nm, and allow us to couple a pure atomic two-level system offered by a single trapped ion to the cavity mode. A new Paul trap apparatus in an ultra-high vacuum chamber has been built which allows for the integration of these cavities at very small ion-mirror separations. In order for independent operation of the trap, a compact system of diode lasers has been built which are stabilised to low-drift optical reference cavities. Coherent control of the hyperfine qubit in Yb 171 is achieved through application of microwave radiation, and ultra-short optical π\piπ rotations are performed with resonant light pulses derived from a frequency-doubled mode-locked titanium-sapphire laser. The experiment is controlled through a system of hardware and software which has been developed in a modular fashion and will allow for efficient control on the nanosecond time-scale when several such systems are interconnected. The success of our system opens the door to future experiments with trapped ions which will reach the strong coupling regime with a single ion. Furthermore, when operated in the fast-cavity regime, systems based on our approach will enable high-efficiency collection of photons from the ion into the single mode of an optical fibre. These systems will allow for the generation of distributed entanglement and will prove ideal as nodes in a larger quantum network of trapped ions.