A frequency-doubled diode laser spectrometer in the blue-wavelength region with a continuous-frequency tuning range of up to ∼7 GHz has been developed, comprising a powerful fundamental light source based on a master/slave laser combination coupled with a KNbO3 crystal for second-harmonic generation in a power-enhancement cavity. It has been employed for the observation of saturated absorption spectra in 52S1/2–62P1/2 hyperfine transitions of atomic rubidium with the aid of a modulation transfer spectroscopic technique, and also the frequency stabilization to one of them has been demonstrated, suggesting the possibility of the establishment of a precision optical frequency marker in the blue range. A relative stability of better than 2.8×10−10 is estimated based on the locked error signal in the preliminary stabilization. With a further study of the frequency instability and uncertainty, in addition to supplementary improvements of apparatus, one may expect a realization of a stabilized laser in the blue-spectral domain. Details of the developed blue-light source are described and the demonstrated results of the rubidium spectroscopy are also described and discussed.
Using modulation transfer spectroscopy, we achieve the frequency stabilization of a high-power 3-W blue laser at the wavelength of 420 nm to the
Rb 5S1/2--
6P3/2 transition. The in-loop frequency stability of this laser is $1.8\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}11}/\sqrt{\ensuremath{\tau}}$, reaching $1.7\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}12}$ at 100 s and $7\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}13}$ at 1000 s. An external power feedback loop is established using an acousto-optic modulator, employing the zeroth-order diffracted light for power stabilization, achieving an in-loop power stability of $1.0\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$ at 1 s. Moreover, the continuous mode-hop free interval of this high-power laser can simultaneously cover the
5S1/2--
6P3/2 transitions of
85Rb and
87Rb, with successful locking achieved for both isotopes, providing a comprehensive analysis of the
Rb atomic transitions in the blue spectral region. As an application, this 3-W 420-nm laser with excellent power and frequency stabilities is used as a repumping source for diffuse laser cooling of
87Rb atoms, realizing a one-meter-long cold-atom cloud. This paves the way for using blue-light cooling to realize a cold-
Rb-atom active optical clock. In addition, the ultrahigh-stability 420-nm laser also finds applications in various fields such as the Rydberg atom experiment, Bose-Einstein condensation, ultranarrow-bandwidth Faraday atomic filter, and so on.
Frequency-modulation (FM) spectroscopy has been performed on the D(2) transitions of rubidium atoms with an AlGaAs diode laser at 780 nm. Doppler-broadened hyperfine-structure transitions of (85)Rb and (87)Rb were resolved with no residual amplitude-modulation-induced background signal by modulating the injection current of the laser diode at a low frequency (20-50 MHz) compared with the Doppler width. To obtain Doppler-free spectra, we combined FM spectroscopy with saturation spectroscopy. The results show that the FM spectroscopy technique is sensitive and should be useful for high-resolution spectroscopy, although the resolution was instrument limited and unusual double peaks were observed.
The modulation transfer spectroscopy (MTS) technique used to stabilize two different transition lines of rubidium, required for laser cooling of atoms, is investigated. The laser source is based on a 1560 nm semiconductor laser diode that is amplified by an erbium doped fiber amplifier (EDFA). The laser output is frequency doubled with a fiber coupled periodically poled Lithium Niobate (PPLN) crystal to 780 nm. To address the weak spectral features of repumping laser, a theoretical study is conducted followed by experimental verification. The 87Rb D2 line F = 1 → F' = 0 transition temperature-enhanced MTS signal is observed, which provides a choice to stabilize the repumping laser frquency on the F = 1 → F ' = 2 transition using frequency shifting with acousto-optic modulators (AOMs). Compared with the orignal MTS signal, this method is shown to be more stable and accurate for laser frequency locking. Laer frequency locking is realized by controlling the driving current of the seed laser using digital PID feedback. After locking, the laser linewidth is 35.36 kHz.
In this work, we address the issue of the suitability of blue fluorescent light as a frequency offset reference during the ladder-level excitation 5S1/2→5P3/2→5D3/2 of Rb85 atoms. A simple pump–probe spectroscopy experiment is performed to generate non-degenerate blue light emission produced by the spontaneous decay route 5D3/2→6P3/2→5S1/2. By varying the relative intensity of the pump–probe combination, we can hover between regimes dominated by mechanisms such as double resonance optical pumping (DROP) and Autler–Townes splitting. The efficacy of the blue fluorescence (420 nm) as a frequency offset reference is pronounced under the DROP regime due to its narrow (∼natural) linewidth. To provide further insight into the stability performance, the pump laser connecting the 5P3/2→5D3/2 transition is stabilized to the peak of the blue light with the help of a probe stabilized to the saturation absorption signal of the 5S1/2→5P3/2 transition. For this purpose, we used the coherence-induced modulation transfer technique. The error frequency noise power spectra and the subsequent Allan variance calculation clearly show that probe fluctuations are transferred to the pump laser because of an existing two-photon coherent coupling.
This is a progress report on the realization of a compact and transportable frequency standard at 1556 nm based on a two-photon transition in rubidium at 778 nm. These hyperfine transitions present great metrological interest. They have a narrow theoretical linewidth of 150 kHz when observed with a 1556 nm laser, and their absolute frequency is known with an uncertainty of 5.2 X 10-12. In this experiment, we use a high power 1556 nm DFB laser and reduce its linewidth to the 10 kHz level using optical feedback from a confocal cavity. We generate its second harmonic in a periodically poled LiNbO3 crystal and use this signal to injection-lock a Fabry-Perot laser emitting 42 mW at 778 nm. The slave laser is used to observe the Doppler-free two- photon transitions: two counter-propagating beams excite rubidium atoms which emit a blue fluorescence on resonance. This 420 nm light is detected on the side of the Rb cell with a photomultiplier. Such an optical frequency standard at 1556 nm, standing in the multiwavelength telecommunications systems window, becomes an attractive source for absolute frequency calibration of WDM components, optical spectrum analyzers and wavemeters.
We have performed high resolution spectroscopy of rubidium with a single mode continuous wave distributed feedback (DFB) laser diode. The saturation spectrum of the D 2 -line of 85 Rb and 87 Rb was recorded with a resolution close to the natural line width. The emission frequency was actively stabilized to Doppler-free transitions with a relative accuracy of better than 7 parts in 10 9 using commercially available servo devices only. An output power of 80 mW was sufficient to allow for two-photon spectroscopy of the 5S-5D-transition of 87 Rb. Further, we report on the spectral properties of the DFB diode, its tuning range and its frequency modulation properties. The line width of the diode laser, determined with high resolution Doppler free two photon spectroscopy, was 4 MHz without applying any active stabilization techniques. For time scales below 5 μs the line width drops below 2 MHz.