Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Quantum Electronics and Laser Science Conference

Frequency modulation two-photon spectroscopy with a modelocked laser in laser-cooled Rb

Michael J. Snadden, A.S. Bell, Roger B. M. Clarke, Erling Riis

Published Jun 2, 1996• 0 citations
OpenAlex

Abstract

Summary form only given. We have previously demonstrated two-photon spectroscopy using a modelocked laser in samples of laser-cooled /sup 85/Rb and /sup 87/Rb. In this paper we present a mechanism with which to frequency stabilize the probe laser in resonance with the two-photon transition. We show that frequency modulation spectroscopy provides an ideal signal to frequency stabilize the laser to the line center. By modulating at a high frequency one can also work where technical noise in the laser is very low.

Related papers

Laser frequency stabilization on 5 P → 5 D transition by double resonance optical pumping and two-photon transition spectroscopy in rubidium

Jinpeng Yuan, Shichao Dong, Lirong Wang +2 more

Abstract We present a laser frequency locking scheme for the high excited transition of rubidium, which cannot be directly referenced by atomic absorption spectroscopy. Double resonance optical pumping spectroscopy and two-photon transition spectroscopy of a 5 S → 5 P → 5 D transition are obtained in a room temperature vapor cell and employed as the reference sources. An Allan deviation of 1.71 × 10 −12 at an averaging time of 2048 s with a residual frequency fluctuation of ±0.2 MHz over 7000 s is obtained by two-photon transition spectroscopy. The case of double resonance optical pumping spectroscopy presents an Allan deviation of 4.86 × 10 −12 at an averaging time of 2048 s with a residual frequency fluctuation of ±0.4 MHz over 7000 s. One distinct advantage of two-photon transition spectroscopy method is demonstrated by the analysis of the fast Fourier transform of error signal. A narrower full width at half-maximum of two-photon transition spectroscopy and a higher zero crossing slope by using a frequency modulation method lead to a better frequency stabilization. This work provides a technical basis for the laser frequency stabilization based on atomic and molecular transition spectroscopy, and it also supplies a new frequency standard for optical telecommunication applications.

Laser Physics•Dec 20, 2019•1 citation

Laser frequency stabilization and shifting by using modulation transfer spectroscopy

Bing Cheng, Zhaoying Wang, Bin Wu +4 more

The stabilizing and shifting of laser frequency are very important for the interaction between the laser and atoms. The modulation transfer spectroscopy for the 87 Rb atom with D2 line transition F = 2 → F′ = 3 is used for stabilizing and shifting the frequency of the external cavity grating feedback diode laser. The resonant phase modulator with electro—optical effect is used to generate frequency sideband to lock the laser frequency. In the locking scheme, circularly polarized pump- and probe-beams are used. By optimizing the temperature of the vapor, the pump- and probe-beam intensity, the laser linewidth of 280 kHz is obtained. Furthermore, the magnetic field generated by a solenoid is added into the system. Therefore the system can achieve the frequency locking at any point in a range of hundreds of megahertz frequency shifting with very low power loss.

Chinese Physics B•Oct 1, 2014•25 citations

FM spectroscopy in fluorescence in laser-cooled rubidium

Michael J. Snadden, Roger B. M. Clarke, Erling Riis

A novel variation of the technique of two-photon frequency modulation (FM) spectroscopy has been developed, which allows signals to be obtained from small (∼105 atoms) and dilute (∼1010 cm−3) samples – in this case laser-cooled rubidium atoms. This was possible by detecting and demodulating the fluorescence signal rather than the transmission through the sample. Data are presented demonstrating the dependence of the signal on phase and frequency of the imposed modulation. Initially the atoms were held in a magneto-optic trap but, in order to eliminate line broadening due to the presence of the trapping fields, data were taken with the atoms in free fall. A similar signal, slightly shifted and broadened by the trapping fields, was obtained while the trap was on and used for long-term stabilisation of the probe laser.

Optics Communications•Jul 1, 1998•8 citations

Modulation transfer spectroscopy in atomic rubidium

Daniel McCarron, S. A. King, Simon L. Cornish

We report modulation transfer spectroscopy on the D2 transitions in 85 Rb and 87 Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87 Rb F = 2 → F ' = 3 and the 85 Rb F = 3 → F ' = 4 transitions, can be significantly enhanced by expanding the beams, improving the signals for laser frequency stabilization. The signal gradient for these transitions is increased by a factor of 3 and the peak to peak amplitude was increased by a factor of 2. The modulation transfer signal for the 85 Rb F = 2 → F ' transitions is also presented to highlight how this technique can generate a single, clear line for laser frequency stabilization even in cases where there are a number of closely spaced hyperfine transitions.

arXiv:0805.2708•Measurement Science and Technology•Aug 19, 2008•209 citations

Frequency stabilization of a GaAs semiconductor laser by use of the optical-optical double-resonance effect of the Doppler-free spectrum of Rb D/sub 1/ line

Masao Suzuki, S. Yamaguchi

The frequency of a GaAs semiconductor laser was locked to the hyperfine spectrum of the Rb D/sub 1/ line by saturation spectroscopy. A first GaAs laser was locked to one of the Doppler-free hyperfine lines using a source modulation method. The burnt hole modulated by the stabilized laser beam was detected by a second laser beam irradicated from the same or the opposite direction and was used as a frequency discriminator to stabilize the second laser. The characteristics of the double-resonance spectrum were measured. The frequency stability of the second laser, which was free from frequency modulation, was estimated to be on the order of 10/sup -9/.>

IEEE Journal of Quantum Electronics•Dec 1, 1988•12 citations

Laser frequency stabilization in the 10 −14 range via optimized modulation transfer spectroscopy on the 87 Rb D 2 line

Sanglok Lee, Geol Moon, Sang Eon Park +5 more

We present a high-performance laser frequency stabilization method using modulation transfer spectroscopy (MTS) on the rubidium 87 D 2 transition line. A substantial improvement of the laser frequency stability was achieved by searching for the optimal diameter and intensity settings of the probe and pump beam. The frequency instability measured from the beat frequency of two locked external cavity diode lasers (ECDLs) reached a short-term stability of 4.5 × 10 − 14 / τ and did not exceed 2 × 10 −12 until 10 5 s, which is the best performance reported thus far with a D 2 transition. The long-term stability is limited by the offset fluctuations of the baseline induced by the residual amplitude modulation (RAM), which can be further improved by reducing the current temperature variation of about 0.2 K by means of temperature stabilization or through a further reduction of the RAM.

Optics Letters•Jan 17, 2023•47 citations
Summary form only given. We have previously demonstrated two-photon spectroscopy using a modelocked laser in samples of laser-cooled /sup 85/Rb and /sup 87/Rb. In this paper we present a mechanism with which to frequency stabilize the probe laser in resonance with the two-photon transition. We show that frequency modulation spectroscopy provides an ideal signal to frequency stabilize the laser to the line center. By modulating at a high frequency one can also work where technical noise in the laser is very low.
Abstract We present a laser frequency locking scheme for the high excited transition of rubidium, which cannot be directly referenced by atomic absorption spectroscopy. Double resonance optical pumping spectroscopy and two-photon transition spectroscopy of a 5 S → 5 P → 5 D transition are obtained in a room temperature vapor cell and employed as the reference sources. An Allan deviation of 1.71 × 10 −12 at an averaging time of 2048 s with a residual frequency fluctuation of ±0.2 MHz over 7000 s is obtained by two-photon transition spectroscopy. The case of double resonance optical pumping spectroscopy presents an Allan deviation of 4.86 × 10 −12 at an averaging time of 2048 s with a residual frequency fluctuation of ±0.4 MHz over 7000 s. One distinct advantage of two-photon transition spectroscopy method is demonstrated by the analysis of the fast Fourier transform of error signal. A narrower full width at half-maximum of two-photon transition spectroscopy and a higher zero crossing slope by using a frequency modulation method lead to a better frequency stabilization. This work provides a technical basis for the laser frequency stabilization based on atomic and molecular transition spectroscopy, and it also supplies a new frequency standard for optical telecommunication applications.
The stabilizing and shifting of laser frequency are very important for the interaction between the laser and atoms. The modulation transfer spectroscopy for the 87 Rb atom with D2 line transition F = 2 → F′ = 3 is used for stabilizing and shifting the frequency of the external cavity grating feedback diode laser. The resonant phase modulator with electro—optical effect is used to generate frequency sideband to lock the laser frequency. In the locking scheme, circularly polarized pump- and probe-beams are used. By optimizing the temperature of the vapor, the pump- and probe-beam intensity, the laser linewidth of 280 kHz is obtained. Furthermore, the magnetic field generated by a solenoid is added into the system. Therefore the system can achieve the frequency locking at any point in a range of hundreds of megahertz frequency shifting with very low power loss.
A novel variation of the technique of two-photon frequency modulation (FM) spectroscopy has been developed, which allows signals to be obtained from small (∼105 atoms) and dilute (∼1010 cm−3) samples – in this case laser-cooled rubidium atoms. This was possible by detecting and demodulating the fluorescence signal rather than the transmission through the sample. Data are presented demonstrating the dependence of the signal on phase and frequency of the imposed modulation. Initially the atoms were held in a magneto-optic trap but, in order to eliminate line broadening due to the presence of the trapping fields, data were taken with the atoms in free fall. A similar signal, slightly shifted and broadened by the trapping fields, was obtained while the trap was on and used for long-term stabilisation of the probe laser.
We report modulation transfer spectroscopy on the D2 transitions in 85 Rb and 87 Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87 Rb F = 2 → F ' = 3 and the 85 Rb F = 3 → F ' = 4 transitions, can be significantly enhanced by expanding the beams, improving the signals for laser frequency stabilization. The signal gradient for these transitions is increased by a factor of 3 and the peak to peak amplitude was increased by a factor of 2. The modulation transfer signal for the 85 Rb F = 2 → F ' transitions is also presented to highlight how this technique can generate a single, clear line for laser frequency stabilization even in cases where there are a number of closely spaced hyperfine transitions.
The frequency of a GaAs semiconductor laser was locked to the hyperfine spectrum of the Rb D/sub 1/ line by saturation spectroscopy. A first GaAs laser was locked to one of the Doppler-free hyperfine lines using a source modulation method. The burnt hole modulated by the stabilized laser beam was detected by a second laser beam irradicated from the same or the opposite direction and was used as a frequency discriminator to stabilize the second laser. The characteristics of the double-resonance spectrum were measured. The frequency stability of the second laser, which was free from frequency modulation, was estimated to be on the order of 10/sup -9/.>
We present a high-performance laser frequency stabilization method using modulation transfer spectroscopy (MTS) on the rubidium 87 D 2 transition line. A substantial improvement of the laser frequency stability was achieved by searching for the optimal diameter and intensity settings of the probe and pump beam. The frequency instability measured from the beat frequency of two locked external cavity diode lasers (ECDLs) reached a short-term stability of 4.5 × 10 − 14 / τ and did not exceed 2 × 10 −12 until 10 5 s, which is the best performance reported thus far with a D 2 transition. The long-term stability is limited by the offset fluctuations of the baseline induced by the residual amplitude modulation (RAM), which can be further improved by reducing the current temperature variation of about 0.2 K by means of temperature stabilization or through a further reduction of the RAM.