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arXiv:2610.12800

Analog quantum simulation of Shastry-Sutherland Ising materials

Vahagn Mkhitaryan, Milan Kornjača, Mao Lin, Alexander Schuckert, Majd Hamdan, Sergio H. Cantú, Ammar Ali, Tommaso Macrí, Nathan Gemelke, Alexander Keesling, Peter Komar, Travis S. Humble, Alexei Bylinski, Pedro L. S. Lopes, Fangli Liu, Alexandra Boltasseva, Mikhail D. Lukin, Arnab Banerjee, Vladimir M. Shalaev, Sheng-Tao Wang

quant-phcond-mat.str-elSubmitted Oct 8, 2026• Announced Oct 12, 2026• 0 citations
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Abstract

Frustrated magnets host rich emergent behavior because competing interactions generate dense manifolds of low-energy states. The Ising Shastry-Sutherland model is a paradigmatic setting, motivated experimentally by Ising-like rare-earth tetraborides such as TmB$_4$ and ErB$_4$, whose field-induced magnetization plateaus have motivated extensive microscopic modeling. Yet how tunable quantum fluctuations reorganize this material-motivated phase diagram remains largely unexplored. Here, we realize a transverse- and longitudinal-field Ising model on the Shastry-Sutherland lattice using a programmable Rydberg-atom array. We map its quantum phase diagram using density matrix renormalization group calculations and probe corresponding signatures experimentally in arrays containing more than 110 atoms. Beyond the established classical phases, the calculations identify two regimes absent in the classical limit and stabilized at finite transverse field: a $2/5$ filling plateau whose finite stability region emerges from a classically degenerate phase boundary and a symmetry-preserving quantum-dimer regime replacing classically selected collinear order. Experiments on finite open arrays reveal signatures consistent with these regimes across three boundary-pinning conditions, with the resulting response maps agreeing qualitatively with the calculated phase diagram. Our results establish programmable Rydberg-atom arrays as tools for exploring frustrated, material-motivated Hamiltonians and motivate searches for new, quantum-driven magnetization plateaus and quantum-dimer behavior in ErB$_4$ under a transverse field or in strain-tuned TmB$_4$.

Comments
24 pages, 13 figures

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Frustrated magnets host rich emergent behavior because competing interactions generate dense manifolds of low-energy states. The Ising Shastry-Sutherland model is a paradigmatic setting, motivated experimentally by Ising-like rare-earth tetraborides such as TmB4_44​ and ErB4_44​, whose field-induced magnetization plateaus have motivated extensive microscopic modeling. Yet how tunable quantum fluctuations reorganize this material-motivated phase diagram remains largely unexplored. Here, we realize a transverse- and longitudinal-field Ising model on the Shastry-Sutherland lattice using a programmable Rydberg-atom array. We map its quantum phase diagram using density matrix renormalization group calculations and probe corresponding signatures experimentally in arrays containing more than 110 atoms. Beyond the established classical phases, the calculations identify two regimes absent in the classical limit and stabilized at finite transverse field: a 2/52/52/5 filling plateau whose finite stability region emerges from a classically degenerate phase boundary and a symmetry-preserving quantum-dimer regime replacing classically selected collinear order. Experiments on finite open arrays reveal signatures consistent with these regimes across three boundary-pinning conditions, with the resulting response maps agreeing qualitatively with the calculated phase diagram. Our results establish programmable Rydberg-atom arrays as tools for exploring frustrated, material-motivated Hamiltonians and motivate searches for new, quantum-driven magnetization plateaus and quantum-dimer behavior in ErB4_44​ under a transverse field or in strain-tuned TmB4_44​.
A core concept in condensed matter physics is geometric frustration that leads to emergent spin phases in magnetic materials.These distinct phases, which depart from the conventional ferromagnet or the antiferromagnet, require unique computational techniques to decipher.In this study, we use the canonical Ising Shastry-Sutherland lattice to demonstrate new techniques for solving frustrated Hamiltonians using a quantum annealer of programmable superconducting qubits.This Hamiltonian can be tuned to produce a variety of intriguing ground states ranging from short-and long-range orders and fractional order parameters.We show that a large-scale finite-field quantum annealing experiment is possible on 468 logical spins of this model embedded into the quantum hardware.We determine microscopic spin configurations using an iterative quantum annealing protocol and develop mean-field boundary conditions to attenuate finitesize effects and defects.We not only recover all phases of the Shastry-Sutherland Ising model-including the well-known fractional magnetization plateau in a longitudinal field-but also predict the spin behavior at the critical points with significant ground-state degeneracy and in the presence of defects.The results lead us to establish the connection to the diffuse neutron scattering experiments by calculation of the static structure factors.
Exact results in frustrated quantum many-body systems are rare, especially in dimensions higher than one. The Shastry-Sutherland (SS) model stands out as a rare example of a two-dimensional spin system with an exactly solvable dimer singlet ground state. In this work, we introduce a three-dimensional analogue of the SS lattice, constructed by deforming the pyrochlore lattice to preserve the local SS geometry. Despite the dimensional increase and altered topology, the ground-state phase diagrams of classical Ising and Heisenberg spins, remain analytically tractable and closely follow their 2D counterparts, including the existence of a 1/3 magnetization plateau and umbrella states. Most notably, for quantum spins S = 1/2, the dimer singlet state survives as an exact ground state over a finite region of the phase diagram. We argue, using exact diagonalization, that the singlet phase is stabilized beyond its 2D counterpart, suggesting enhanced robustness in three dimensions. These results offer a rare, controlled platform to explore the impact of dimensionality on quantum frustration, exact solvability, and potential spin liquid behavior in 3D, with relevance to emergent topological and magnetic phases.
Using density matrix renormalization group (DMRG) and perturbative continuous unitary transformations (PCUTs), we study the magnetization process in a magnetic field for all coupling strengths of a quasi-1D version of the 2D Shastry-Sutherland lattice, a frustrated spin tube made of two orthogonal dimer chains. At small inter-dimer coupling, plateaus in the magnetization appear at 1/6, 1/4, 1/3, 3/8, and 1/2. As in 2D, they correspond to a Wigner crystal of triplons. However, close to the boundary of the product singlet phase, plateaus of a new type appear at 1/5 and 3/4. They are stabilized by the localization of bound states of triplons. Their magnetization profile differs significantly from that of single-triplon plateaus and leads to specific NMR signatures. We address the possibility to stabilize such plateaus in further geometries by analyzing small finite clusters using exact diagonalizations and the PCUTs.
We explore the field-induced magnetic phases of an S=1S=1S=1 XXZXXZXXZ model with single-ion anisotropy and large Ising-like anisotropy on a Shastry-Sutherland lattice over a wide range of Hamiltonian parameters and applied magnetic field. The multitude of ground-state phases are characterized in detail in terms of their thermodynamic properties, and the underlying classical (Ising limit) spin arrangements for the plateau phases are identified by calculating the static structure factors. The enlarged local Hilbert space of the S=1S=1S=1 spins results in several ground state phases that are not realized for S=1/2S=1/2S=1/2 spins. These include the quantum paramagnetic state that is ubiquitous to S=1S=1S=1 spins with single-ion anisotropy, two different spin supersolid phases (with distinct longitudinal ordering), and a magnetization plateau that arises as a direct descendant of the 1/3 plateau due to quantum fluctuations that are not possible for S=1/2S=1/2S=1/2 spins. We predict the same mechanism will lead to plateaus at smaller fractions of 1/3 for higher spins. The full momentum dependence of the longitudinal and transverse components of the static structure factor is calculated in the spin supersolid phase to demonstrate the simultaneous existence of diagonal and off-diagonal long-range order as well as the different longitudinal orderings.
Shastry-Sutherland magnet is a typical frustrated spin system hosting rich phases. While the Heisenberg limit has been extensively studied, the role of spin-orbit coupling is not well explored. Motivated by newly discovered rare-earth Shastry-Sutherland magnets, we construct a generic effective-spin model that describes the interactions between Kramers doublet local moments on a Shastry-Sutherland lattice. Due to the strong spin-orbit coupling, the model takes the form of extended XYZ interactions on both intra- and inter-dimer bonds. We show that, in addition to the conventional “singlet” dimer phase, strong spin-orbit coupling can stabilize peculiar “triplet” dimer phases. These “triplet” dimer phases, though fully gapped, respond immediately to magnetic fields and evolve smoothly into the fully polarized phase. We present that the recently discovered Shastry-Sutherland magnet Yb 2 Be 2 GeO 7 belongs to the “triplet” dimer phase, and discuss the implication of our results to a broad class of quantum magnets in general.
Neutral-atom quantum simulators offer a promising approach to the exploration of strongly interacting many-body systems, with applications spanning condensed matter, statistical mechanics, and high-energy physics. Through a combination of quantum experiments, numerical calculations, and analytical methods, we demonstrate a rich set of phenomena accessible on such quantum simulators by studying an array of Rydberg atoms placed on the Lieb lattice. First, we map out the ground states and phase diagram of the system, identifying a range of density-wave-ordered phases -- including a collinear phase stabilized purely by quantum fluctuations -- and find good agreement between theory and experiment. Allowing for local control of the detuning field thereafter, we discover a quantum analog of the classical liquid-vapor transition between two density-wave phases distinguished by sublattice occupation, and probe its underlying hysteretic dynamics. Furthermore, we study out-of-equilibrium quantum quenches and observe anomalously slow relaxation dynamics consistent with the kinetic constraints of an emergent string phase. These results highlight how geometric control offered by neutral-atom simulators can extend the frontiers of programmable quantum matter, enabling access to complex phases, metastability, and thermalization dynamics in many-body quantum systems.