Quantum criticality and nonequilibrium dynamics on a Lieb lattice of Rydberg atoms
Mark R. Hirsbrunner, Milan Kornjača, Rhine Samajdar, Siva Darbha, Majd Hamdan, J. T. Balewski, Ermal Rrapaj, Sheng-Tao Wang, Daan Camps, Fangli Liu, Pedro L. S. Lopes, Katherine Klymko
Neutral-atom quantum simulators offer a promising approach to the exploration of strongly interacting many-body systems, with applications spanning condensed matter, statistical mechanics, and high-energy physics. Through a combination of quantum experiments, numerical calculations, and analytical methods, we demonstrate a rich set of phenomena accessible on such quantum simulators by studying an array of Rydberg atoms placed on the Lieb lattice. First, we map out the ground states and phase diagram of the system, identifying a range of density-wave-ordered phases -- including a collinear phase stabilized purely by quantum fluctuations -- and find good agreement between theory and experiment. Allowing for local control of the detuning field thereafter, we discover a quantum analog of the classical liquid-vapor transition between two density-wave phases distinguished by sublattice occupation, and probe its underlying hysteretic dynamics. Furthermore, we study out-of-equilibrium quantum quenches and observe anomalously slow relaxation dynamics consistent with the kinetic constraints of an emergent string phase. These results highlight how geometric control offered by neutral-atom simulators can extend the frontiers of programmable quantum matter, enabling access to complex phases, metastability, and thermalization dynamics in many-body quantum systems.
Neutral-atom quantum simulators offer a promising approach to the exploration of strongly interacting many-body systems, with applications spanning condensed matter, statistical mechanics, and high-energy physics. Through a combination of quantum experiments, numerical calculations, and analytical methods, we demonstrate a rich set of phenomena accessible on such quantum simulators by studying an array of Rydberg atoms placed on the Lieb lattice. First, we map out the ground states and phase diagram of the system, identifying a range of density-wave-ordered phases -- including a collinear phase stabilized purely by quantum fluctuations -- and find good agreement between theory and experiment. Allowing for local control of the detuning field thereafter, we discover a quantum analog of the classical liquid-vapor transition between two density-wave phases distinguished by sublattice occupation, and probe its underlying hysteretic dynamics. Furthermore, we study out-of-equilibrium quantum quenches and observe anomalously slow relaxation dynamics consistent with the kinetic constraints of an emergent string phase. These results highlight how geometric control offered by neutral-atom simulators can extend the frontiers of programmable quantum matter, enabling access to complex phases, metastability, and thermalization dynamics in many-body quantum systems.
We describe the zero-temperature phase diagram of a model of a two-dimensional square-lattice array of neutral atoms, excited into Rydberg states and interacting via strong van der Waals interactions. Using the density-matrix renormalization group algorithm, we map out the phase diagram and obtain a rich variety of phases featuring complex density wave orderings, upon varying lattice spacing and laser detuning. While some of these phases result from the classical optimization of the van der Waals energy, we also find intrinsically quantum-ordered phases stabilized by quantum fluctuations. These phases are surrounded by novel quantum phase transitions, which we analyze by finite-size scaling numerics and Landau theories. Our work highlights Rydberg quantum simulators in higher dimensions as promising platforms to realize exotic many-body phenomena.
Understanding emergent phenomena in out-of-equilibrium interacting many-body systems is an exciting frontier in physical science. While quantum simulators represent a promising approach to this long-standing problem, in practice it can be challenging to directly realize the required interactions, measure arbitrary observables, and mitigate errors. Here we use coherent mapping between the Rydberg and hyperfine qubits in a neutral atom array simulator to engineer and probe complex quantum dynamics. We combine efficient analog dynamics with fully programmable state preparation and measurement, leverage non-destructive readout for loss information and atomic qubit reuse, and use an atom reservoir for replacing lost atoms. With this analog-digital approach, we first demonstrate dynamical engineering of ring-exchange and particle hopping dynamics via Floquet driving and measure the spectral function of single excitations by evolving initial superposition states. Extending these techniques to a 271-site kagome lattice, we employ closed-loop optimization to target an out-of-equilibrium critical quantum spin liquid of the Rokhsar-Kivelson type. We observe the key features of such a state, including the absence of local order, many-body coherences between nearly equal-amplitude dimer configurations over up to 18 sites, and universal correlations consistent with predictions from field theory. Together, these results pave the way for using dynamical control in analog-digital quantum simulators to study complex quantum many-body systems.
The dynamics of isolated quantum systems following a sudden quench plays a central role in many areas of material science, high-energy physics, and quantum chemistry. Featuring complex phenomena with implications for thermalization, non-equilibrium phase transitions, and Floquet phase engineering, such far-from-equilibrium quantum dynamics is challenging to study numerically, in particular, in high-dimensional systems. Here, we use a programmable neutral atom quantum simulator to systematically explore quench dynamics in spin models with up to 180 qubits. By initializing the system in a product state and performing quenches across a broad parameter space, we discover several stable, qualitatively distinct dynamical regimes. We trace their robustness to Floquet-like prethermal steady states that are stabilized over long emergent timescales by strong dynamical constraints. In addition, we observe sharp peaks in the dynamical response that are quantitatively explained by the structured melting of prethermalization through resonances. In two dimensions, we uncover a sharp dynamical response change that converges with increased system size, that is linked to the proliferation of Néel-order defects and indicative of a dynamical phase transition with no equilibrium analogs. Uncovering an intricate interplay between quantum prethermalization and emergent dynamical phases, our results demonstrate the use of quantum simulators for revealing complex non-equilibrium quantum many-body phenomena.
Programmable arrays of neutral Rydberg atoms are one of the leading platforms today for scalable quantum simulation and computation. In these systems, the dipole-dipole interactions between the individual atoms, or qubits, typically result in binary -- i.e., two-body -- couplings. In this work, we develop an experimentally accessible scheme for engineering three-body interactions in Rydberg lattices. Such strong three-body couplings can fundamentally modify the underlying physics compared to systems with only two-body interactions: we demonstrate this, in particular, by systematically investigating the effective many-body Hamiltonian and its emergent quantum phases. This capability paves the way for the quantum simulation of a broader class of correlated models of condensed matter and high-energy physics.
Programmable quantum systems provide insights into many-body quantum phenomena and enable new methods for computation and metrology. The frontier challenge for these systems is scaling up in the number of quantum particles while retaining a high degree of quantum control. In recent years arrays of neutral atoms have emerged as a scalable and powerful platform for tackling these challenges, thanks to their large number of qubits, flexible geometry, and a well-established toolbox for preparation, detection, coherent control. At the forefront of quantum science and engineering, these systems have been used for quantum simulation of various spin models and have also demonstrated building blocks of quantum computation. In this thesis I will present advances in development of large two-dimensional atom arrays, where hundreds of individual atoms are trapped, rearranged, and initialized in various defect-free arrangements in one or two dimensions. Afterwards, interactions between atoms is controlled via coherent excitation to highly excited Rydberg states, resulting in strong long-range van der Waals forces. We utilize these interaction for quantum simulation of many-body spin Hamiltonians by demonstrating preparation of several exotic phases of matter, study phase transitions, and probe non-equilibrium dynamics. Further, we study the quantum speedup in solving a hard combinatorial optimization problem via efficiently mapping the problem onto the Rydberg atom array. We also utilize Rydberg interactions to demonstrate high-fidelity two-qubit gate operations in a reconfigurable atom array architecture. Lastly I will demonstrate recent technical improvements that have enabled larger system sizes, higher fidelity rydberg excitations, and local control of individual atoms, paving the way for novel approaches for studying quantum many-body phenomena.
Abstract Lattice gauge theories (LGTs) describe a broad range of phenomena in condensed matter and par11 ticle physics. A prominent example is confinement, responsible for bounding quarks inside hadrons such as protons or neutrons [1]. When quark-antiquark pairs are separated, the energy stored in the string of gluon fields connecting them grows linearly with their distance, until there is enough energy to create new pairs from the vacuum and break the string. While such phenomena are ubiquitous in LGTs, simulating the resulting dynamics is a challenging task [2]. Here, we report the observation of string breaking in synthetic quantum matter using a programmable quantum simulator based on neutral atom arrays [3–5]. We show that a (2+1)D LGT with dynamical matter can be efficiently implemented when the atoms are placed on a Kagome geometry [6], with a local U(1) symmetry emerging from the Rydberg blockade [7], while long-range Rydberg interactions naturally give rise to a linear confining potential for a pair of charges, allowing us to tune both their masses as well as the string tension. We experimentally map out the corresponding phase diagram by adiabatically preparing the ground state of the atom array in the presence of defects, and observe substructure of the confined phase, distinguishing regions dominated by fluctuating strings or by broken string con24 figurations. Finally, by harnessing local control over the atomic detuning, we quench string states and observe string breaking dynamics exhibiting a many-body resonance phenomenon. Our work paves a way to explore phenomena in high-energy physics using programmable quantum simulators.