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arXiv:2610.12511

Spinodal-controlled freeze-out and nucleation at the first-order superfluid-supersolid transition of a dipolar gas

Wai Kui Wong

Published Oct 7, 2026• 0 citations
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Abstract

Dipolar quantum gases in elongated traps become supersolid through a transition that is continuous at intermediate density but first order at low and high density; at the continuous point, ramps of the scattering length follow Kibble-Zurek scaling. We study ramps across the first-order superfluid-supersolid transition of $^{164}$Dy in an infinite tube using the 3D extended Gross-Pitaevskii equation with truncated-Wigner noise. With quantum noise only, the uniform superfluid survives the metastable window and transforms after its spinodal, where the roton softens. For onsets occurring during the linear ramp, the delay measured from this spinodal has a fitted exponent $ζ= 0.36 \pm 0.02$, close to the continuous-transition result and the mean-field value $1/3$. Reverse ramps show a comparable delay beyond the fold of the crystal branch, producing dynamical hysteresis. Initial thermal noise with nominal temperatures of 2.5-10 nK produces crystalline regions inside the metastable window during holds, with faster nucleation closer to the spinodal and at higher initial temperature. In ramps at 5 nK, thermal fluctuations make the superfluid fraction $f_s$ cross onset thresholds near $f_s = 1$ early, whereas the bulk of the crystal still forms after the zero-temperature spinodal with a similar scaling. Without a heat bath these effective rates depend on preparation: ramps crossing the window at the same rate nucleate early in 2 of 32 or 11 of 16 realizations depending on their starting point. At low density, slower ramps select larger spacings in a crystal of separated droplets, and droplets survive far above the transition on reverse ramps. A Maxwell construction gives a coexistence window $0.037 a_0$ wide around the first-order transition point, in which localized states exist; in the simulated tube they lie above the homogeneous states. At the continuous point there is no coexistence.

DOI
10.48550/arxiv.2610.12511

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Dipolar quantum gases in elongated traps become supersolid through a transition that is continuous at intermediate density but first order at low and high density; at the continuous point, ramps of the scattering length follow Kibble-Zurek scaling. We study ramps across the first-order superfluid-supersolid transition of 164^{164}164Dy in an infinite tube using the 3D extended Gross-Pitaevskii equation with truncated-Wigner noise. With quantum noise only, the uniform superfluid survives the metastable window and transforms after its spinodal, where the roton softens. For onsets occurring during the linear ramp, the delay measured from this spinodal has a fitted exponent ζ=0.36±0.02ζ= 0.36 \pm 0.02ζ=0.36±0.02, close to the continuous-transition result and the mean-field value 1/31/31/3. Reverse ramps show a comparable delay beyond the fold of the crystal branch, producing dynamical hysteresis. Initial thermal noise with nominal temperatures of 2.5-10 nK produces crystalline regions inside the metastable window during holds, with faster nucleation closer to the spinodal and at higher initial temperature. In ramps at 5 nK, thermal fluctuations make the superfluid fraction fsf_sfs​ cross onset thresholds near fs=1f_s = 1fs​=1 early, whereas the bulk of the crystal still forms after the zero-temperature spinodal with a similar scaling. Without a heat bath these effective rates depend on preparation: ramps crossing the window at the same rate nucleate early in 2 of 32 or 11 of 16 realizations depending on their starting point. At low density, slower ramps select larger spacings in a crystal of separated droplets, and droplets survive far above the transition on reverse ramps. A Maxwell construction gives a coexistence window 0.037a00.037 a_00.037a0​ wide around the first-order transition point, in which localized states exist; in the simulated tube they lie above the homogeneous states. At the continuous point there is no coexistence.
We simulate interaction quenches crossing from a superfluid to a supersolid state in a dipolar quantum gas of Dy 164 atoms, trapped in an elongated tube with periodic boundary conditions, via the extended Gross-Pitaevskii equation. A freeze-out time is observed through a delay in supersolid formation after crossing the critical point. We compute the density-density correlations at the freeze-out time and extract the frozen correlation length for the solid order. An analysis of the freeze-out time and correlation length versus the interaction quench rate allows us to extract universal exponents corresponding to the relaxation time and correlation length based on predictions of the Kibble-Zurek mechanism. Over several orders of magnitude, clear power-law scaling is observed for both the freeze-out time and the correlation length, and the corresponding exponents are compatible with predictions based on the excitation spectrum calculated via Bogoliubov theory. Defects due to independent local breaking of translational symmetry, contributing to globally incommensurate supersolid order, are identified, and their number at the freeze-out time is found to also scale as a power law. Our results support the hypothesis of a continuous transition whose universality class remains to be determined but appears to differ from that of the (1 + 1)-dimensional model.
We provide a theoretical characterization of the dynamical crossing of the superfluid-supersolid phase transition for a dipolar condensate confined in an elongated trap, as observed in the recent experiment by Biagioni et al. [G. Biagioni, N. Antolini, A. Ala\~na, M. Modugno, A. Fioretti, C. Gabbanini, L. Tanzi, and G. Modugno, Phys. Rev. X 12, 021019 (2022)]. By means of the extended Gross-Pitaevskii theory, which includes the Lee-Huang-Yang quantum fluctuation correction, we first analyze the ground-state configurations of the system as a function of the interparticle scattering length, for both trap configurations employed in the experiment. Then, we discuss the effects of the ramp velocity, by which the scattering length is tuned across the transition, on the collective excitations of the system in both the superfluid and supersolid phases. We find that, when the transverse confinement is sufficiently strong and the transition has a smooth (continuous) character, the system essentially displays a (quasi) one-dimensional behavior, its excitation dynamics being dominated by the axial breathing modes. Instead, for shallower transverse trapping, when the transition becomes discontinuous, the collective excitations of the supersolid display a coupling with the transverse modes, signaling the onset of a dimensional crossover.
We investigate the excitation spectrum and compressibility of a dipolar Bose-Einstein condensate in an infinite tube potential in the parameter regime where the transition between superfluid and supersolid phases occurs. Our study focuses on the density range in which crystalline order develops continuously across the transition. Above the transition the superfluid shows a single gapless excitation band, phononic at small momenta and with a roton at a finite momentum. Below the transition, two gapless excitations branches (three at the transition point) emerge in the supersolid. We examine the two gapless excitation bands and their associated speeds of sound in the supersolid phase. Our results show that the speeds of sound and the compressibility are discontinuous at the transition, indicating a second-order phase transition. These results provide valuable insights into the identification of supersolid phenomena in dipolar quantum gases and the relationship to supersolidity in spin-orbit coupled gases.
We characterize the role of roton instability in the formation of a supersolid state of an elongated dipolar condensate, following a quench of the contact interactions across the superfluid-supersolid transition, as observed in recent experiments. We perform dynamical simulations by means of the extended Gross-Pitaevskii equation including quantum corrections, for different final values of the $s\text{\ensuremath{-}}\mathrm{wave}$ scattering length. The corresponding excitation spectrum is computed using an effective one-dimensional description, which provides a reasonably accurate prediction for the growth rate of the most unstable mode observed in the simulations. To analyze the behavior of the system, we employ the inverse participation ratio, which conveniently characterizes the different degree of localization in the superfluid and supersolid phases. By means of a suitable effective ansatz for the density, we derive a simple yet effective expression for the formation time of the supersolid. This expression provides valuable insights regarding its scaling behavior with respect to the sss-wave scattering length.
Motivated by a recent experimental work arXiv:2608.20327, we theoretically investigate the nature of phase transitions in a trapped dipolar quantum gas upon tuning the contact interaction strength and dipole orientation. Using extended Gross-Pitaevskii simulations including thermal and quantum effects, we map the phase diagram comprising unmodulated superfluids, triangular droplet arrays, and stripe states. We further characterize the order of the transitions separating them through imaginary-time hysteresis analysis. The unmodulated-to-modulated transition evolves from discontinuous to continuous with increasing dipole tilt before becoming discontinuous again at large tilts. The degree of continuity is further affected by particle number, temperature, and confinement. While continuous behavior generally correlates with the emergence of stripe states, this correspondence is not systematic, and finite-size effects also influence the continuity of the transition. The triangular-to-stripe transition is found to be discontinuous at small contact interaction strengths and becomes increasingly continuous upon approaching the unmodulated-to-modulated phase boundary. Our results reveal a tunable transition order in finite dipolar quantum gases and provide guidance for its experimental investigation.
We consider a binary magnetic gas and develop an extended Gross-Pitaevskii theory to study the system. We apply this theory to the regime where the two- body interactions are attractive for some arrangements of the atoms, and mean- field theory predicts mechanical collapse. In this regime quantum droplets of the binary magnetic gas can emerge, stabilised by quantum fluctuations. These quantum droplets can exist in miscible and immiscible regimes, and we characterise their properties over a broad parameter space. Simplified theories are developed to describe the droplets, and benchmarked against the full numerical calculations. The system dynamics are simulated for scenarios involving droplet formation and crossing the miscible-immiscible transition. Three-body loss is modelled in the dynamical simulations to account for the dominant loss process expected in experiments. We also study the supersolidity of a single-component dipolar gas in an infinite tube potential. An accurate computational algorithm is developed to calculate the ground state of the system in a unit cell. This algorithm is used to determine the phase diagram by characterising the crystalline order and superfluid fraction. Our results reveal that a system confined in a radially harmonic trap has a continuous transition for a range of density values, but is discontinuous for densities above and below this range. The theory is used to calculate the crystalline and supersolid states of a binary magnetic gas in a tube potential.