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arXiv:2305.19811 · Physical Review A

Supersolid formation in a dipolar condensate by roton instability

Aitor Alaña, I. L. Egusquiza, Michele Modugno

Published Sep 26, 2023• 12 citations
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Abstract

We characterize the role of roton instability in the formation of a supersolid state of an elongated dipolar condensate, following a quench of the contact interactions across the superfluid-supersolid transition, as observed in recent experiments. We perform dynamical simulations by means of the extended Gross-Pitaevskii equation including quantum corrections, for different final values of the $s\text{\ensuremath{-}}\mathrm{wave}$ scattering length. The corresponding excitation spectrum is computed using an effective one-dimensional description, which provides a reasonably accurate prediction for the growth rate of the most unstable mode observed in the simulations. To analyze the behavior of the system, we employ the inverse participation ratio, which conveniently characterizes the different degree of localization in the superfluid and supersolid phases. By means of a suitable effective ansatz for the density, we derive a simple yet effective expression for the formation time of the supersolid. This expression provides valuable insights regarding its scaling behavior with respect to the $s$-wave scattering length.

DOI
10.1103/physreva.108.033316

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We characterize the role of roton instability in the formation of a supersolid state of an elongated dipolar condensate, following a quench of the contact interactions across the superfluid-supersolid transition, as observed in recent experiments. We perform dynamical simulations by means of the extended Gross-Pitaevskii equation including quantum corrections, for different final values of the s\ensuremath-waves\text{\ensuremath{-}}\mathrm{wave}s\ensuremath-wave scattering length. The corresponding excitation spectrum is computed using an effective one-dimensional description, which provides a reasonably accurate prediction for the growth rate of the most unstable mode observed in the simulations. To analyze the behavior of the system, we employ the inverse participation ratio, which conveniently characterizes the different degree of localization in the superfluid and supersolid phases. By means of a suitable effective ansatz for the density, we derive a simple yet effective expression for the formation time of the supersolid. This expression provides valuable insights regarding its scaling behavior with respect to the sss-wave scattering length.
We provide a theoretical characterization of the dynamical crossing of the superfluid-supersolid phase transition for a dipolar condensate confined in an elongated trap, as observed in the recent experiment by Biagioni et al. [G. Biagioni, N. Antolini, A. Ala\~na, M. Modugno, A. Fioretti, C. Gabbanini, L. Tanzi, and G. Modugno, Phys. Rev. X 12, 021019 (2022)]. By means of the extended Gross-Pitaevskii theory, which includes the Lee-Huang-Yang quantum fluctuation correction, we first analyze the ground-state configurations of the system as a function of the interparticle scattering length, for both trap configurations employed in the experiment. Then, we discuss the effects of the ramp velocity, by which the scattering length is tuned across the transition, on the collective excitations of the system in both the superfluid and supersolid phases. We find that, when the transverse confinement is sufficiently strong and the transition has a smooth (continuous) character, the system essentially displays a (quasi) one-dimensional behavior, its excitation dynamics being dominated by the axial breathing modes. Instead, for shallower transverse trapping, when the transition becomes discontinuous, the collective excitations of the supersolid display a coupling with the transverse modes, signaling the onset of a dimensional crossover.
Dipolar condensates have recently been coaxed into supersolid phases supporting both superfluid and crystal excitations. While one-dimensional (1D) supersolids may be prepared via a roton instability, we find that such a procedure in two dimensions (2D) leads to greater heating. We go on to show that 2D roton modes have little in common with the supersolid configuration: instead, unstable centralized rotons trigger a process of nonlinear crystal growth. By evaporatively cooling directly into the supersolid phase--hence bypassing the first-order roton instability--we experimentally produce a 2D supersolid in a near-circular trap. We develop a stochastic Gross-Pitaevskii theory that includes beyond-meanfield effects to further explore the formation process. We calculate the static structure factor for a 2D supersolid, and compare to a 1D array. These results provide insight into the process of supersolid formation in 2D, and define a realistic path to the formation of large two-dimensional supersolid arrays.
Dipolar condensates have recently been coaxed to form the long-sought supersolid phase. While one-dimensional supersolids may be prepared by triggering a roton instability, we find that such a procedure in two dimensions (2D) leads to a loss of both global phase coherence and crystalline order. Unlike in 1D, the 2D roton modes have little in common with the supersolid configuration. We develop a finite-temperature stochastic Gross-Pitaevskii theory that includes beyond-mean-field effects to explore the formation process in 2D and find that evaporative cooling directly into the supersolid phase-hence bypassing the first-order roton instability-can produce a robust supersolid in a circular trap. Importantly, the resulting supersolid is stable at the final nonzero temperature. We then experimentally produce a 2D supersolid in a near-circular trap through such an evaporative procedure. Our work provides insight into the process of supersolid formation in 2D and defines a realistic path to the formation of large two-dimensional supersolid arrays.
In a recent experiment, it has been found that by tuning the interaction strength of a dipolar Bose-Einstein Condensate confined in a quasi-1D geometry orthogonal to the polarization direction, the roton gap vanishes, while density modulations are induced in the trapped gas. This suggests the possibility of realizing a supersolid in dipolar quantum gases. Inspired by this experiment, we simulate a dipolar BEC in a ring geometry by confining the dipoles in a ”tube” orthogonal to the polarization direction and enforcing periodic boundary conditions. Our calculations are based on a Density Functional approach where the total energy density functional includes the beyond-mean-field correction of Lee-Huang-Yang, which partially accounts for quantum fluctuations. We study the ground state properties of the system by evolving in imaginary time the EulerLagrange equation derived from the variational principle. We also study the excitation spectrum of the system by solving the corresponding Bogoliubov-de Gennes equations. We find that the calculated excitation spectrum shows indeed a roton minimum, and the roton gap can become vanishingly small by reducing the effective scattering length. As the roton gap disappears, we find that the system spontaneously develops in its ground-state a periodic structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. We find that this structure shows the hallmarks of a supersolid system, i.e. (i) a finite non-classical translational inertia and (ii) the appearance, besides the phonon mode, of the Nambu-Goldstone gapless mode corresponding to fluctuations in the phase, and related to the spontaneous breaking of the gauge symmetry.
Motivated by a recent experiment [L. Chomaz et al., Nat. Phys. 14, 442 (2018)], we perform numerical simulations of a dipolar Bose-Einstein condensate (BEC) in a tubular, periodic confinement at T=0T=0T=0 within density functional theory, where the beyond-mean-field correction to the ground-state energy is included in the local density approximation. We study the excitation spectrum of the system by solving the corresponding Bogoliubov--de Gennes equations. The calculated spectrum shows a roton minimum, and the roton gap decreases by reducing the effective scattering length. As the roton gap disappears, the system spontaneously develops a periodic linear structure formed by denser clusters of atomic dipoles immersed in a dilute superfluid background. This structure shows the hallmarks of a supersolid system, i.e., (i) a finite nonclassical translational inertia along the tube axis and (ii) the appearance of two gapless modes, i.e., a phonon mode associated with density fluctuations and resulting from the translational discrete symmetry of the system, and a Nambu-Goldstone gapless mode corresponding to phase fluctuations, resulting from the spontaneous breaking of the gauge symmetry. A further decrease in the scattering length eventually leads to the formation of a periodic linear array of self-bound droplets.
Supersolids are a phase of matter exhibiting both superfluidity and a periodic density modulation typical of crystals. When formed via quantum phase transition from a superfluid, they require a formation time before their density pattern develops. In this paper protocols and schemes are proposed for experimental applications, building on earlier descriptions of the role roton instability plays in the supersolid formation process and the associated formation time. In particular, two protocols are put forward to shorten the formation time and lessen the excitation produced when crossing the phase transition. As a case study of the impact that mechanical fluctuations (noise) can have on the phase transition when conducting an experiment, the impact of a mechanical kick before the transition is also investigated. The proposed schemes achieve a shortening of the formation process for comparable levels of excitation, in the framework of extended Gross-Pitaevskii theory.