Scalable quantum processors require repeated qubit initialization throughout large arrays. In semiconductor spin qubits, fast initialization commonly relies on local reservoir access or measurement-based feedback, requiring dedicated infrastructure that becomes increasingly difficult to distribute as processors scale. Here, we demonstrate reservoir- and measurement-free initialization of a silicon spin-qubit pair in an industrially fabricated Si/SiGe quantum-dot device using a fixed sequence of microwave and baseband pulses. Odd spin-parity states relax to the singlet charge state, whereas blocked even spin-parity states are microwave-driven through the triplet manifold and subsequently converted to the singlet by singlet-triplet mixing and charge hybridization. Repeated cycles produce the singlet-associated charge outcome with a median probability of 99.4% across the sampled preparation states, while exchange spectroscopy independently verifies mapping to the target $|\uparrow\downarrow\rangle$ operational state. Microwave spectroscopy and time-domain measurements identify the dark-state-limited single-cycle transfer and the subsequent blockade-lifting dynamics that set the initialization time scale. The demonstrated pumping sequence uses approximately $12\,μ\mathrm{s}$ of microwave bursts and mixing dwells, while we project sub-microsecond initialization under improved device conditions. These results establish fixed-sequence microwave initialization as a scalable control primitive for semiconductor spin-qubit processors, based on singlet-triplet physics that can be adapted to platforms with suitable Pauli-blockade transitions.
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27 pages, 5 main figures and 4 extended data figures
Scalable quantum processors require repeated qubit initialization throughout large arrays. In semiconductor spin qubits, fast initialization commonly relies on local reservoir access or measurement-based feedback, requiring dedicated infrastructure that becomes increasingly difficult to distribute as processors scale. Here, we demonstrate reservoir- and measurement-free initialization of a silicon spin-qubit pair in an industrially fabricated Si/SiGe quantum-dot device using a fixed sequence of microwave and baseband pulses. Odd spin-parity states relax to the singlet charge state, whereas blocked even spin-parity states are microwave-driven through the triplet manifold and subsequently converted to the singlet by singlet-triplet mixing and charge hybridization. Repeated cycles produce the singlet-associated charge outcome with a median probability of 99.4% across the sampled preparation states, while exchange spectroscopy independently verifies mapping to the target ∣↑↓⟩ operational state. Microwave spectroscopy and time-domain measurements identify the dark-state-limited single-cycle transfer and the subsequent blockade-lifting dynamics that set the initialization time scale. The demonstrated pumping sequence uses approximately 12μs of microwave bursts and mixing dwells, while we project sub-microsecond initialization under improved device conditions. These results establish fixed-sequence microwave initialization as a scalable control primitive for semiconductor spin-qubit processors, based on singlet-triplet physics that can be adapted to platforms with suitable Pauli-blockade transitions.
We demonstrate rapid high-fidelity state preparation and measurement in exchange-only Si/SiGe triplequantum-dot qubits.Fast measurement integration (980-ns) and initialization (approximately 300-ns) operations are performed with all-electrical baseband control.We emphasize a leakage-sensitive joint initialization and measurement metric, developed in the context of exchange-only qubits but applicable more broadly, and report an infidelity of 2.5 ± 0.5×10 -3 .This result is enabled by a high-valley-splitting heterostructure, initialization at the two-to three-electron charge boundary, and careful assessment and mitigation of T 1 during spin-to-charge conversion.The ultimate fidelity is limited by a number of comparably important factors and we identify clear paths toward further improved fidelity and speed.Along with an observed single-qubit randomized benchmarking error rate of 1.7 × 10 -3 , this work demonstrates initialization, control, and measurement of Si/SiGe triple-dot qubits at fidelities and durations that are promising for scalable quantum information processing.
Quantum physics describes the universe on a microscopic scale. Even though this scale is not accessible without complex experimental setups, quantum effects are respon- sible for the properties of matter and in some instances we have learned to exploit them technologically. A modern computer constituted of transistors passively utilizes the quantum nature of charge carriers in the band structure of semiconductors to encode and process information. Although such a classical computer is a formidable tool already, what could be achieved with active control over the quantum states in the computer is an intriguing question. This is the idea of the quantum computer, which offers an entirely new paradigm of computing by encoding information in quantum binary digits (qubits). Indeed, for several applications it has been shown that a quantum computer is superior to its classical counterpart, even though its realization remains elusive up to date. One candidate to host qubits are gate-defined semiconductor quantum dots, confin- ing single or few charge carriers with spin. The spin of a single confined electron is a quantum two-level system which can be manipulated and measured, allowing the storage and processing of quantum information. This thesis can be viewed as part of the endeavor to give birth to quantum computers based on semiconductor spin qubits. It primarily focuses on the challenge to enable scalable architectures of well-characterized qubits. In the first part, spin shuttling is investigated. This denotes the coherent transport of a single spin between spatially separate nodes of a quantum processor, driven by a time-dependent electric potential. The object of study is a minimal version of a bucket- brigade-like spin shuttling between two quantum dots. The probability of maintaining the spin state is identified as figure of merit and the effect of spin-orbit interaction and the Zeeman effect in an inhomogeneous magnetic field is explored with analytical and numerical methods. Special attention is paid to the repercussions of near-degenerate valleys. The second part of the thesis addresses the challenge to probe the microscopic properties of a quantum dot array, which is a crucial first step before any quantum operation can be performed. The transmission of a microwave resonator coupled to a triple quantum dot occupied by two electrons is investigated, and a scheme to infer the exchange interaction between electrons in adjacent quantum dots is proposed. By means of analytical derivations it is shown that the transmission profile of the resonator directly reveals the value of the exchange coupling strength between two electrons. This holds even if magnetic gradients or a valley splitting comparable to the inter-dot tunnel coupling are included. Subsequently, quantum transport measurements in the Pauli blockade regime are modelled in the presence of a microwave resonator, bringing together two powerful techniques to probe quantum dots. Based on generalized input-output theory, a theoretical framework is derived to investigate how a double quantum dot in a transport setup interacts with a coupled microwave resonator while the current through the double qauntum dot is rectified by Pauli blockade. It is shown that the output field of the resonator can be used to infer the leakage current and thus obtain insight into the blockade mechanisms and to estimate a large number of parameters of the quantum dots. Furthermore, the back-action of the resonator photons on the steady state leakage current is described and quantified. In the context of Pauli blockade, the spin and valley physics of bilayer graphene quantum dots in the few-electron regime is touched upon, describing a situation where spin blockade is observed despite the presence of the valleys. In the final part of the thesis, the attention is shifted towards the readout of the spin qubits. A new paradigm of dispersive readout is devised, which is performed while the qubit dephases, implementing a measurement in the x-basis. Laplace transforming the time dependent cavity response allows a separation of contributions from multiple qubits coupled to the same resonator. Thus, they can be read out simultaneously in a single shot. Modelling silicon spin qubits, as an example, results in in a readout time that compares favourably to conventional dispersive readout with comparable fidelity, even for a single qubit. With an auxiliary qubit the readout scheme can be extended to a quantum non-demolition measurement.
Electron spins confined in semiconductor quantum dots are emerging as a promising system to study quantum information science and to perform sensitive metrology. Their weak interaction with the environment leads to long coherence times and robust storage for quantum information, and the intrinsic tunability of semiconductors allows for controllable operations, initialization, and readout of their quantum state. These spin qubits are also promising candidates for the building block for a scalable quantum information processor due to their prospects for scalability and miniaturization. owever, several obstacles limit the performance of quantum information experiments in these systems. For example, the weak coupling to the environment makes inter-qubit operations challenging, and a fluctuating nuclear magnetic field limits the performance of single-qubit operations.\n\n\n\nThe focus of this thesis will be several experiments which address some of the outstanding problems in semiconductor spin qubits, in particular, singlet-triplet (S-T0) qubits. We use these qubits to probe both the electric field and magnetic field noise that limit the performance of these qubits. The magnetic noise bath is probed with high bandwidth and precision using novel techniques borrowed from the field of Hamiltonian learning, which are effective due to the rapid control and readout available in S-T0 qubits. These findings allow us to effectively undo the undesired effects of the fluctuating nuclear magnetic field by tracking them in real-time, and we demonstrate a 30-fold improvement in the coherence time T2*.\n\n\n\nWe probe the voltage noise environment of the qubit using coherent qubit oscillations, which is partially enabled by control of the nuclear magnetic field. We find that the voltage noise bath is frequency- dependent, even at frequencies as high as 1MHz, and it shows surprising and, as of yet, unexplained temperature dependence. We leverage this knowledge of the voltage noise environment, the nuclear magnetic field control, as well as new techniques for calibrated measurement of the density matrix in a singlet-triplet qubit to entangle two adjacent single-triplet qubits. We fully characterize the generated entangled states and prove that they are, indeed, entangled.\n\n\n\nThis work opens new opportunities to use qubits as sensors for improved metrological capabilities, as well as for improved quantum information processing. The singlet-triplet qubit is unique in that it can be used to probe two fundamentally different noise baths, which are important for a large variety of solid state qubits. More specifically, this work establishes the singlet-triplet qubit as a viable candidate for the building block of a scalable quantum information processor.
Pauli-spin-blockade (PSB) measurements have so far achieved the highest fidelity of spin readout in semiconductor quantum dots, overcoming the 99% threshold. Moreover, in contrast to energy-selective readout, PSB is less error prone to thermal energy, an important feature for large-scale architectures that could be operated at temperatures above a few hundreds of millikelvins. In this work, we use rf reflectometry on a single-lead quantum dot to perform charge sensing and to probe the spin state of a double quantum dot at 0.5 K. At this relatively elevated temperature, we characterize both singlet-triplet and parity readout, which are complementary measurements to perform a complete readout of a two-spin system. We demonstrate high-fidelity spin readout with an average fidelity above 99.9 % for a readout time of 20 μs and 99 % for 4 μs. Finally, we succeed in initializing a singlet state in a single dot with a fidelity higher than 99 % and separate the two electrons while retaining the same spin state with a 95.6 % fidelity
This dissertation describes a set of experiments with the goal of creating a super-conductor-semiconductor hybrid circuit quantum electrodynamics architecture with single electron spins. Single spins in silicon quantum dots have emerged as attractive qubits for quantum computation. However, how to scale up spin qubit systems remains an open question. The hybrid architecture considered here could provide a route to realizing large networks of quantum dot–based spin qubit registers. The first experiment in this thesis is aimed at achieving strong coupling between a single electron spin and a single microwave photon. The electron is trapped in a gate-defined double quantum dot in a Si/SiGe heterostructure and the photon is stored in an on-chip superconducting high-impedance NbTiN cavity. The photon is coupled directly to the electron charge, and indirectly to the electron spin, mediated through a synthetic spin-orbit field. We observe a vacuum Rabi splitting that depends on the spin-charge hybridization. The ratio of spin-photon coupling strength to decoherence rates of the spin and cavity combined is larger than unity, confirming the strong coupling regime has been reached. In addition, we find an optimal degree of spin-charge hybridization for which this ratio is maximized. The demonstration of strong spin-photon coupling not only opens a new range of physics experiments, but fulfills also a crucial requirement for coupling spin qubits at a distance via a cavity. The second experiment is focused on spin readout with the on-chip cavity. Instead of the direct dispersive readout of a single spin, we use the cavity to detect whether the electron is allowed to tunnel between the two dots or not. We benchmark the charge sensitivity and bandwidth of the detector and find that rapid detection of the electron charge with high SNR is possible. In the two-electron regime, electron tunneling is contingent on the total spin state (Pauli spin blockade). This spin-to-charge conversion scheme enables single-shot detection of singlet states with high-fidelity. The demonstration of single-shot spin readout with a cavity is an essential step towards readout in dense spin qubit arrays, such as the crossbar network, where it is not possible to integrate electrometers and accompanying reservoirs adjacent to the qubit dots. In the third experiment, we develop on-chip microwave filters to suppress microwave photon leakage from the cavity through the gate electrodes that are necessary to form quantum dots. We introduce a new cavity design that is compatible with long-distance connectivity between spins, but is also more susceptible to microwave leakage. We test and compare two low-pass filter variations in terms of performance, footprint and integrability. They use the same nanowire inductor, but different implementations of the capacitor: one with a planar interdigitated capacitor and one novel design with an overlapping thin-film capacitor. We find that both approaches are effective against microwave leakage. However, the large footprint of the interdigitated capacitor makes this solution inconvenient as the number of gate lines increases. The thin-film capacitor, with its much smaller footprint, is better suited for our devices. The final part of this dissertation contains concluding remarks and possible future directions are proposed.
Silicon-based spin qubits have emerged as a promising platform for scalable quantum computation due to their compatibility with advanced semiconductor fabrication and integration with classical CMOS electronics. As fabrication capabilities advance toward larger, higher-yield devices, the field is transitioning from academic prototypes toward processors ultimately requiring millions of qubits. This shift places increasing emphasis on developing operating techniques that scale with qubit number. In this thesis, a four qubit SiMOS processor is used to investigate three key aspects of multi-qubit operation for spin-based quantum computing. First, tuning and operation techniques for parallel double-quantum-dot unit cells are developed. Electron loading strategies enable four-qubit operation in an isolated charge configuration, and universal single- and two-qubit control is demonstrated. The native gate set is characterised using gate set tomography. The processor is operated as two unit cells that can be initialised and read out in parallel, providing two independent parity measurements per shot, without increasing operation time or degrading state preparation and measurement fidelity. Second, control techniques for generating multi-qubit entangled states and executing general quantum circuits are established. Three-qubit maximally entangled states, including cluster and Greenberger–Horne–Zeilinger states, are generated and measured with a maximum fidelity of 82.5%. A Mermin value of 3.14 is achieved, certifying genuine tripartite entanglement. A fully symmetric dynamically decoupled gate sequence is developed, extending the entanglement lifetime beyond T2* to a limit set by T2-Hahn. A workflow for compiling, executing, and analysing arbitrary circuits from OpenQASM is also demonstrated. Finally, the first mid-circuit measurements in a silicon spin-qubit system are presented. This capability is extended to feedforward control, including a novel “in-layer” method that performs conditional phase operations without routing information to the classical control layer. This approach leverages measurement-induced backaction as a control mechanism. Both in-layer and FPGA-enabled feedforward strategies are benchmarked, and their dominant error channels are identified.